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自蔓延高温合成氮化硅镁粉体 被引量：1

Self-propagating high-temperature synthesis of MgSiN2 powder
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摘要 研究了不同起始反应物体系(Mg+Si,Mg2Si和Mg+Si3N4)对氮气中燃烧合成氮化硅镁(MgSiN2)粉体的影响,结果显示,不同反应物体系的燃烧产物不同.Mg2Si和Mg+Si3N4能获得单一相的MgSiN2,而且氧含量低至0.356%(质量分数),而Mg+Si体系燃烧产物除主相MgSiN2外,还含有少量Si和MgO及一些未知相.
作者 彭桂花 江国健 李文兰 庄汉锐
机构地区 中国科学院
出处 《功能材料》 EI CAS CSCD 北大核心 2004年第z1期3051-3053,共3页 Journal of Functional Materials
关键词 自蔓延高温合成 氮化硅镁
分类号 TQ174.75+8.12 [化学工程—陶瓷工业]
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参考文献8

  • 1[1]Groen W A, Kraan M J, Preparation, microstructure and properties of MgSiN2 ceramics [J]. J Eur Ceram Soc, 1993,12:413.
  • 2[2]Hintzen H T, Swaanen P, Metselaar R, Hot-pressing of MgSiN2 Ceramics [J]. J Mater Sci Lett, 1994, 13: 1314.
  • 3[3]Hayashi H, Hirao K, Toriyama M, et al. MgSiN2 addition as a means of increasing the thermal conductivity of β-Si3N4[J]. J Am Ceram Soc, 2001, 12: 3060.
  • 4[4]Uchida H, Itatani K, Aizawa M, et al. Synthesis of magnesium silicon nitride by the nitridation of powders in the magnesium-silicon system [J]. J Ceram Soc Jpn, 1997,105(11): 934.
  • 5[5]Bruls R J, Hintzen H T, Metselaar R. Preparation and characterization of MgSiN2 powders [J]. J Mater Sci, 1999,34: 4519.
  • 6[6]Leno e s Z, Hirao K, Yamauchi Y, et al. Reaction synthesis of magnesium silicon nitride powder.[J]. J Am. Ceram. Soc.,2003, 86(7): 1088.
  • 7[7]Uchida H, Itatani K, Aizawa M, et al. Synthesis of magnesium silicon nitride powder by the carbothermal reduction technique [J]. Adv Powder Technol, 1999, 10(2): 133.
  • 8[8]Munir Z A. Synthesis of high temperature materials by self-propagating combustion [J]. Am Ceram Soc Bull, 1988,67: 342.

同被引文献18

  • 1BLAIR R G, KUDYBA-JANSEN A A, et al. Preparation, characterization and properties of MgSiN2 ceramics [J]. J Mater Sci: Mater Electron, 2002, 13: 63-75.
  • 2FANG C M, GROOT R A DE, BRULS R J, et al. Ab initio band structure calculations of Mg3N2 and MgSiN2 [J]. J Phys: Condens Matter, 1999, 11: 4833-4842.
  • 3TANAKA S, ITATANI K, HINTZEN H T. Effect of silicon nitride addition on the thermal and mechanical properties of magnesium silicon nitride ceramics [J]. J Eur Ceram Soc, 2004, 24: 2163-2168.
  • 4GROEN W A, KRAAN M J. Preparation, microstructure and properties of MgSiN2 ceramics [J]. J Eur Ceram Soc, 1993, 12: 413-420.
  • 5PENG G H, LIANG M, LIANG Z H, et al. Spark plasma sintered silicon nitride ceramics with high thermal conductivity using MgSiN2 as additives [J]. J Am Ceram Soc, 2009, 92(9): 2122-2124.
  • 6UCHIDA H, ITATANI K, AIZAWA M, et al. Synthesis of magnesium silicon nitride by the nitridation of powders in the magnesium-silicon system [J]. J Ceram Soc Jpn, 1997, 105(11): 934-939.
  • 7PENG G H, JIANG G J, ZHUANG H R, et al. Fabrication of β-Si3N4 whiskers by combustion synthesis with MgSiN2 as additives [J]. Mater Res Bull, 2005, 40: 2139-2143.
  • 8PENG L, XU L Q, JU Z C, et al. Large-scale synthesis of magnesium silicon nitride powders at low temperature [J]. J Am Ceram Soc, 2008, 91(1): 333-336.
  • 9LENOES Z, HIRAO K, YAMAUCHI Y, et al. Reaction synthesis of magnesium silicon nitride powder [J]. J Am Ceram Soc, 2003, 86: 1088-1093.
  • 10GREKOV F F, CHERNOVETS B V. Methods for MgSiN2 synthesis [J]. Russ J Appl Chem, 2004, 77: 1223-1226.

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功能材料
2004年 第z1期

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