摘要
以乙二胺为溶剂,以介孔分子筛SBA-15为载体,采用低温溶剂热法成功地合成出V和N元素共修饰的V—TiO2-xNX/SBA-15整体式可见光催化剂。将其用于光催化降解亚甲基兰的反应,较单-V或N改性的催化剂具有更强的可见光吸收能力,表现出更好的催化降解亚甲基兰的性能。结果也表明,采用金属、非金属双元素改性及“一锅法”整体合成方法是提高二氧化钛催化活性和实用性的有效方法。
Visible-light-responsive V-TiO2-xNx/SBA-15 was triumphantly synthesized by ' one pot' method at low- temperature with ethylenediamine as solvent. The evaluation of catalytic activity showed that the V-TiO2-x Nx/SBA-15 sample had much superior performance with respect to the single V or N modified TiO2/SBA-15 in the visible-light photoeatalytic purification of methyene. It was indicated that visible-light absorption of the V-TiO2-x Nx/SBA-15 samples were enhanced by co-modification of V and N and 'one pot' synthesis.
出处
《石油学报(石油加工)》
EI
CAS
CSCD
北大核心
2008年第B10期256-259,共4页
Acta Petrolei Sinica(Petroleum Processing Section)
基金
国家自然科学基金(20573059,20777039)和国家重点基础研究发展计划(973计划,2003CB615801)项目资助