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唑类含能离子化合物的合成研究进展 被引量：45

Progress of Study on the Synthesis of Azole Energetic Ionic Compounds
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摘要 综述了以咪唑、三唑、四唑以及五唑等唑类化合物为母体的一些含能盐的合成,系统总结了这类新型含能材料的熔点、密度、生成焓等理化性能以及爆轰性能,并分析了分子结构及取代基对含能盐性能的影响。对唑类含能盐在火炸药和推进剂等方面的应用进行了展望。附36篇参考文献。 The synthesis of energetic salts comprising imidazole, triazole, tetrazole and pentazole as precursors are reviewed with 36 references. The physiochemical properties of these new energetic salts, such as melting point, density, enthalpy of formation and detonation performance, as well as the effect of molecular structure and substituted groups on properties are summarized. The applications of these compounds in explosives and propellants are discussed.
作者 刘晓建 张慧娟 林秋汉 李玉川 李亚裕 庞思平
机构地区 北京理工大学生命学院 北京航天试验技术研究所
出处 《火炸药学报》 EI CAS CSCD 北大核心 2010年第1期6-10,共5页 Chinese Journal of Explosives & Propellants
基金 国家自然科学基金资助(20772011 20903011)
关键词 有机化学 富氮杂环 含能材料 离子盐 唑类 合成 organic chemistry nitrogen-rich heterocycles energetic material ionic salts azole synthesis
分类号 O641.2 [理学—物理化学] TQ254 [化学工程—有机化工]
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参考文献36

  • 1Ogihara W, Yoshizawa M, Ohto H. Novel ionic liquids composed of only azole ions [J]. Chem Lett, 2004.. 33,1022.
  • 2Katritzky A R,Singh S, Kirichemko K,et al. 1-butyl- 3-methylimidazolium3, 5-dinitro-1, 2, 4-triazolate: a novel ionic liquid containing a rigid, planar energetic anion[J]. Chem Commun, 2005,7 : 868-870.
  • 3Xue H, Gao Y, Shreeve J M, et al. New energetic salts based on nitrogen-containing heterocycles [J].Chem Mater,2005,17:191- 198.
  • 4Gao H X, Ye C F, Shreeve J M. 2,4,5-Trinitro- imidazole-based energetic salts [J]. Chem Eur J, 2007,13:3853-3860.
  • 5Drake G W, Hawkins T,Brand A,et al. Energetic, low melting salts of simple heteroeycles[J]. Propell, Explos, Pyroteeh, 2003,28 (4) : 174-180.
  • 6Schmidt M W, Gordon M S, Boatz J A. Triazolium- based energetic ionic liquids [J]. J Phys Chem A, 2005,109 : 7285-7295.
  • 7Xue H, Gao Y, Shreeve J M, et al. Energetic azo lium azolate salts [J]. Inorganic Chemistry, 2005,44 : 5068 5072.
  • 8Xue H, Twamley B, Shreeve J M. The first 1-alkyl- 3-perfluoroalkyl-4, 5-dimethyl 1,2,4-triazolium salts [J]. J Org Chem, 2004,69:1397-1400.
  • 9Mirzaei Y R, Xue H, Shreeve J M. Low melting N-4- functionalized-1-alkyl or polyfluoroalkyl-1, 2, 4- triazolium salts [J]. Inorg Chem, 2004,43 : 361-367.
  • 10Mirzaei Y R, Twamley B, Shreeve J M. Syntheses of 1-alkyl-1, 2, 4-triazoles and the formation of quaternary 1-alkyl-4-polyfluoroalkyl-1,2,4-triazolium salts leading to ionic liquids[J]. J Org Chem, 2002, 67:9340-9345.

二级参考文献6

  • 1Hiskey M, Chavez D. Progress in high-nitrogen chemistry in explosives, propellants and pyrotechnics[A]. Proc 27th International Pyrotechnics Seminar[C]. Colorado:IPS,2000: 3-14.
  • 2Bucerius Klaus. Stable nitrogen-rich composition[P]. US:5198046, 1993.
  • 3Hiskey M, Goldman N, Stine J. High-nitrogen energetic materials derived from azotetrazolate[J]. Energetic Materials, 1998,(16):119-127.
  • 4张丙辰译.起爆药中四唑类的潜力[J].火工品,1988,(1):42-47.
  • 5Peng Yu-Lin,Wong Chi-Wung . Preparation guanidinium 5′,5-azotetrazolate[P]. US:5877300, 1999.
  • 6Gerhard Holl,Manfred Kaiser,Kaiser,et al.[N2H5]+2[N4C-N=N-CN4]2-:A new high-nitrogen highenergetic materials[J]. Inorg Chem,2001,(40):3570-3575.)

共引文献39

同被引文献543

引证文献45

二级引证文献164

火炸药学报
2010年 第1期

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