摘要
The formation of the Nail molecule from unaligned ultracoM atoms via photoassociation （PA） is theoretically investigated by numerically solving the time-dependent Schrodinger equation including the vibrational and rotational degrees of freedom. The PA processes via one- and two-photon excitations are described. The calculated results show that the associated molecule can be prepared to a desired rovibrational state of the ground electronic state for Nail. Compared with the one-pfloton association probability, the two-photon association probability is obviously enhanced.
The formation of the Nail molecule from unaligned ultracoM atoms via photoassociation （PA） is theoretically investigated by numerically solving the time-dependent Schrodinger equation including the vibrational and rotational degrees of freedom. The PA processes via one- and two-photon excitations are described. The calculated results show that the associated molecule can be prepared to a desired rovibrational state of the ground electronic state for Nail. Compared with the one-pfloton association probability, the two-photon association probability is obviously enhanced.
基金
Supported by the National Natural Science Foundation of China under Grant Nos 10974024 and 20633070.
