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Concentrations and Sources of Polycyclic Aromatic Hydrocarbons in Topsoil of Benxi City, Northeast China 被引量:1

Concentrations and Sources of Polycyclic Aromatic Hydrocarbons in Topsoil of Benxi City, Northeast China
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摘要 Polycyclic aromatic hydrocarbons (PAHs) contamination of topsoil in Benxi City, Northeast China was investigated in this study, and sampling sites were located in industrial area and residential area. Results demonstrate that there is high variability in the total PAHs concentrations, ranging from 783.00 ng/g to 729 076.29 ng/g dry weight in the topsoil of Benxi City and the pollution in industrial area is the most serious. The results also present that higher molecular weight PAHs (4–6 rings) contribute substantially (79.03%) to the overall content of PAHs. The PAHs sources were determined with factor analysis by nonnegative constraints, and the results show that PAHs originating from traffic tunnel, power plant, coke oven and residential emission sources, account for 27.10%, 40.81%, 20.11% and 11.98%, respectively, of the total. The PAHs pollution is the most serious around Benxi Iron and Steel Group Corporation, and the PAHs mainly originate from coke oven and traffic tunnel, with the average contribution rate of 57.40% and 42.60%, respectively. The source apportionment results are basically consistent with the industry distribution, and the geographical and climatic characteristics of the study area. Polycyclic aromatic hydrocarbons (PAHs) contamination of topsoil in Benxi City, Northeast China was investigated in this study, and sampling sites were located in industrial area and residential area. Results demonstrate that there is high variability in the total PAHs concentrations, ranging from 783.00 ng/g to 729 076.29 ng/g dry weight in the topsoil of Benxi City and the pollution in industrial area is the most serious. The results also present that higher molecular weight PAHs (4-6 rings) contribute substantially (79.03%) to the overall content of PAHs. The PAHs sources were determined with factor analysis by nonnegative constraints, and the results show that PAHs originating from traffic tunnel, power plant, coke oven and residential emission sources, account for 27.10%, 40.81%, 20.11% and 11.98%, respectively, of the total. The PAHs pollution is the most serious around Benxi Iron and Steel Group Corporation, and the PAHs mainly originate from coke oven and traffic tunnel, with the average contribution rate of 57.40% and 42.60%, respectively. The source apportionment results are basically consistent with the industry distribution, and the geographical and climatic characteristics of the study area.
出处 《Chinese Geographical Science》 SCIE CSCD 2011年第2期185-194,共10页 中国地理科学(英文版)
基金 Under the auspices of Program of National Soil Pollution Survey (No. 6HBZJ1002)
关键词 polycyclic aromatic hydrocarbons concentration characteristics source apportionment factor analysis 中国东北地区 多环芳烃 本溪市 表层土壤 本溪钢铁集团公司 浓度 交通隧道 碳氢化合物
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  • 1Aichner B, Glaser B, Zech W, 2007. Polycyclic aromatic hydrocarbons and polychlorinated biphenyls in urban soils from Kathmandu, Nepal. Organic Geochemistry, 38(4): 700-715. doi: 10.1016/j.orggeochem.2006.11.002.
  • 2Amit M, Ajay T, 2006. Polycyclic aromatic hydrocarbons (PAHs) concentrations and related carcinogenic potencies in soil at a semi-arid region of India. Chemosphere, 65(3): 449-456. doi: 10.1016/J.chemosohere.2006.01.062.
  • 3Barbara M K, Bozena S, Agnieszka K P, 2009. Concentrations, sources, and spatial distribution of individual polycyclic aromatic hydrocarbons (PAHs) in agricultural soils in the Eastern part of the EU: Poland as a case study. Science of the Total Environment, 407(12): 3746-3753. doi: 10.1016/j.scitotenv.2009.01.010.
  • 4Baumard R Budzinski H, Michon Q et al., 1998. Origin and bioavailability of PAHs in the Mediterranean Sea from mussel and sediment. Estuarine, Coastal and Shelf Science, 47(1): 77-90. doi: 10.1006/ecss. 1998.0337.
  • 5Belkessam L, Lecomte P, Milon V et al., 2005. Influence of pre-treatment step on PAHs analyses in contaminated soils. Chemosphere, 58(3): 321-328. doi: 10.1016/j.chemosphere. 2004.07.040.
  • 6Bucheli T D, Blum F, Desaules A et al., 2004. Polycyclic aromatic hydrocarbons, black carbon, and molecular markers in soils of Switzerland. Chemosphere, 56(11): 1061-1076. doi: 10.1016/j. chemo sphere. 2004.06.002.
  • 7Budzinski H, Jones I, Bellocq Jet al., 1997. Evaluation of sediment contamination by polycyclic aromatic hydrocarbons in the Gironde estuary. Marine Chemistry, 58(1-2): 85-97. doi: 10.1016/S0304-4203(97)00028-5.
  • 8Bzdusek P A, Christensen E R, Li A et al., 2004. Source appor-tionment of sediment PAHs in Lake Calumet, Chicago: Appli- cation of factor analysis with nonnegative constrains. Environmental Science & Technology, 38(1): 97-103. doi: 10.1021/ es034842k.
  • 9Cai Q Y, Mo C H, Li Y H et al., 2007. Occurrence and assessment of polycyclic aromatic hydrocarbons in soils from vegetable fields of the Pearl River Delta, South China. Chemosphere, 68(1): 159-168. doi: 10.1016/i.chemosDhere.2006.1 2.015.
  • 10Chen Y J, Sheng G Y, Bi X H et al., 2005. Emission factors for carbonaceous particles and polycyclic aromatic hydrocarbons from residential coal combustion in China. Environmental Science & Technology, 39(6): 1861-1867. doi: 10.1021/es0493650.

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