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Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method 被引量:5

Recovery of Hydrogen from Ammonia Plant Tail Gas by Absorption-Hydration Hybrid Method
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摘要 In this work, the absorption-hydration hybrid method was used to recover (hydrogen + nitrogen) from (hydrogen + nitrogen + methane + argon) tail gas mixtures of synthetic ammonia plant through hydrate formation/dissociation. A high-pressure reactor with magnetic stirrer was used to study the separation efficiency. The in-fluences of the concentration of anti-agglomerant, temperature, pressure, initial gas-liquid volume ratio, and oil-water volume ratio on the separation efficiency were systematically investigated in the presence of tetrahydro-furan (THF). Anti-agglomerant was used to disperse hydrate particles into the condensate phase for water-in-oil emulsion system. Since nitrogen is the material for ammonia production, the objective production in our separation process is (hydrogen + nitrogen). Our experimental results show that by adopting appropriate operating conditions, high concentration of (hydrogen + nitrogen) can be obtained using the proposed technology based on forming hydrate. 在这个工作,吸收水和混血儿方法被用来恢复(氢 + 氮) 从(氢 + 氮 + 甲烷 + 氩) 合成的氨的尾巴气体混合物通过水合物形成 / 分离种。有磁性的 stirrer 的一个高压的反应堆被用来学习分离效率。anti-agglomerant,温度,压力,起始的煤气液体的体积比率,和分离效率上的油水体积比率的集中的影响系统地面对 tetrahydrofuran (THF ) 被调查。Anti-agglomerant 被用来为 water-in-oil 乳剂系统驱散水合物粒子进冷凝物阶段。因为氮是为氨生产的材料,在我们的分离过程的客观生产是(氢 + 氮) 。我们的试验性的结果由采用适当操作条件显示出那,高集中(氢 + 氮) 能基于形成水合物用建议技术被获得。
出处 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2011年第5期784-791,共8页 中国化学工程学报(英文版)
基金 Supported by the National/qatural Science Foundation of China (20925623, 21006126), the Special Funds for Major State Basic Research Program of China (No. 2009CB219504), the Research Funds of China University of Petroleum, Beijing (BJBJRC-2010-01), and Beijing Nova Program (2010B069).
关键词 SEPARATION HYDRATE HYDROGEN synthetic ammonia plant tail gas 混合方法 尾气吸收 合成氨厂 氢回收 水化 水合物形成 合成氨生产 分离效率
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