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堆制处理过程中的多环芳烃降解 被引量:11

DEGRADATION OF POLYCYCLIC AROMATIC HYDROCARBONS IN COMPOSTING OF SOIL
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摘要 用实验室模拟方法,研究了堆制处理过程对污染土壤中4 ~6 环的多环芳烃(PAHs) 的降解. 结果表明,堆制对6 种难降解的PAHs 都有不同程度的降解作用,PAHs 的降解随着苯环数的增加而降低,其去除率的大小顺序为荧蒽> 苯并[a] 蒽、苯并[a] 芘> 苯并[b] 荧蒽、苯并[k] 荧蒽> 苯并[ghi] 北. 其中,荧蒽的去除率为46.0 % ~92.9% ;苯并[a] 蒽的去除率为7.7% ~37 .2 % . 当PAHs 的初始浓度提高约50 倍时,除荧蒽外其它PAHs 的降解随着污染浓度的提高而降低. 不同C/N均有类似的规律,但C/N25:1 比C/N40:1 为好. 堆中各种PAHs 浓度在高温期以前都有所提高,但在降温期以后又有不同程度的降低. 细菌总数测定表明,数量变化呈双峰型. Laboratory scale test was conducted to evaluate the degradation of polycyclic aromatic hydrocarbons(PAHs) in composting of soil. Six PAHs were involved, including fluoranthene (FA), benzo[a]anthracene (B[a]A), benzo[b]fluoranthene (B[b]F), benzo[k]fluoranthene (B[k]F), benzo[a]pyrene (B[a]P) and benzo[g,h,i]perylene(B[ghi]Pe). The results indicated that all PAHs were degraded to some extent in the composting. The order of the percentage of PAHs loss was FA, B[a]A, B[a]P, B[b]F, B[k]F and B[ghi]Pe. Among those, FA removal rate was 46.0%~92.9% and B[a]A 7.7%~37.2%. The removal rates of the most PAHs decreased with rise of initial PAHs concentration, except FA. Similar rule was found in different C/N ratios (25:1~40:1), but 25:1 was better. The concentrations of PAHs increased during the temperature increasing stage and thermophic stage of the composting, but decreased during the temperature decreasing stage and curing stage. Total count of bacteria in the composting had two peak values.
出处 《应用与环境生物学报》 CAS CSCD 1999年第6期605-609,共5页 Chinese Journal of Applied and Environmental Biology
基金 国家自然科学基金!(No:29577269)
关键词 堆制处理 土壤 多环芳烃 生物降解 生物修复 composting soil polycyclic aromatic hydrocarbons bioremediation biodegradation
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参考文献4

  • 1钱易.重点有机污染物生物降解性能评介[J]环境科学,1986(02).
  • 2中国科学院南京土壤研究所微生物室.土壤微生物研究法[M]科学出版社,1985.
  • 3南京农学院.土壤农化分析[M]农业出版社,1980.
  • 4Richard T. Williams,P. Scott Ziegenfuss,Wayne E. Sisk. Composting of explosives and propellant contaminated soils under thermophilic and mesophilic conditions[J] 1992,Journal of Industrial Microbiology(2):137~144

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