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青藏高原气溶胶单颗粒类型及粒度分布 被引量:2

Types and size distribution of individual particles in the Tibetan Plateau
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摘要 应用场发射扫描电镜(FESEM)对青藏高原纳木错综合观测站和香格里拉本底站2011年7~8月份不同天气情况下收集的气溶胶样品进行研究。结果表明,区域内气溶胶单颗粒类型主要包括烟尘集合体、球形颗粒(焦油球、燃煤飞灰)、似球形颗粒、矿物颗粒、生物颗粒等,香格里拉的球形颗粒中出现了飞灰颗粒,而纳木错样品中没有。纳木错气溶胶颗粒的数量-粒度峰值和体积-粒度峰值分别出现在0.2~0.3μm和1~2.5μm,矿物颗粒数量和体积最多,分别占44.4%和61.7%。香格里拉气溶胶颗粒的数量-粒度峰值和体积-粒度峰值都呈现双峰分布,主峰均分布在>2.5μm范围,矿物颗粒数量和体积最多,分别占51.7%和58.7%。细粒子和粗粒子分别为纳木错和香格里拉气溶胶的主要类型。纳木错气溶胶中矿物颗粒最多,数量百分比为44.4%,其次为烟尘集合体(29.5%)和球形颗粒(26.1%),香格里拉气溶胶中矿物颗粒数量百分比为51.7%,其次为球形颗粒(29%)和烟尘集合体(19.3%);纳木错气溶胶总颗粒物主要分布在0.2~0.3μm粒径范围中,数量百分比为32.59%,其中矿物颗粒最多(15%),其次为球形颗粒(11.5%)和烟尘集合体(6.1%)。香格里拉气溶胶颗粒物主要分布在>2.5μm粒径范围中,数量百分比为37.5%,其中矿物颗粒最多(17.9%),其次为球形颗粒(10%)和烟尘集合体(9.6%)。 Field emission scanning electron microscopy (FESEM) was used to study the aerosol samples collected in Nam Co and air of Shangri-La under different weather conditions during July~August,2011.The results showed that particles could be subdivided into 5 major morphological categories,namely soot aggregates,spherical particles (tar ball and fly ash),spherical particles,mineral particles and bio-particles.There existed fly ash in Shangri-La aerosol samples,which however did not exist in Nam Co.Number-size and volume-size distribution of particles in Nam Co aerosol samples displayed peaks in the size range of 0.2~0.3μm and 1 ~2.5μm.The proportion of quantity(44.4 %)and that of volume(61.7 %)of mineral particles were the highest; size distribution of particles in Shangri-La aerosol samples displayed two major peaks in the size range of over 2.5μm.The proportion of quantity (51.7%) and that of volume (58.7%) of mineral particles were the highest.Fine particles and coarse particles were the major types of aerosol samples of Nam Co and Shangri-La respectively.The amount (44.4%) of mineral particles was the highest in Nam Co,followed by soot aggregates (29.5%) and spherical particles (26.1%).The quantity proportion (32.59%) of Nam Co aerosol samples was mainly in the size range of 0.2~0.3 μm.Mineral particles were the highest (15%),followed by spherical partides (11.5%) and soot aggregates (6.1%).The quantity proportion (37.5%) of Shangri-La aerosol samples was mainly in the size range of over 2.5 μm.Mineral particles were the highest (17.9%),followed by spherical particles (10 %) and soot aggregates (9.6 %).
出处 《岩石矿物学杂志》 CAS CSCD 北大核心 2013年第6期863-872,共10页 Acta Petrologica et Mineralogica
基金 公益性行业(气象)专项资助项目(GYHY20110623)
关键词 气溶胶 场发射扫描电镜 青藏高原 aerosol field emission scanning electron microscopy (FESEM) Tibetan Plateau
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