期刊文献+

脉冲电晕放电等离子体-活性炭协同去除废水中重金属离子和有机物 被引量:20

Simultaneous Removal of Heavy Metal Ions and Organic Compounds in Wastewater by Pulsed Corona Discharge Plasma Combined with Activated Carbon
原文传递
导出
摘要 为了同时去除废水中的重金属离子和有机污染物,以镉离子(Cd2+)和酸性橙7(AO7)为目标污染物,研究比较了活性炭(AC)、脉冲电晕放电等离子体(PCDP)以及PCDP结合AC(PCDP-AC)3种体系对废水中Cd2+和AO7的去除效果。考察了脉冲放电电压、载气种类、溶液初始pH值和电导率对Cd2+和AO7去除的影响。结果表明:PCDP-AC体系可以同时有效地去除废水中的Cd2+和AO7,且去除效果明显好于AC和PCDP单独处理;增加脉冲放电电压,可以提高Cd2+和AO7去除率;氧气作为载气的去除效果高于空气或氮气作为载气的去除效果;酸性条件下AO7的去除率好于碱性条件,而Cd2+的去除率在碱性条件下好于酸性条件;增加溶液初始电导率,会导致Cd2+和AO7去除率下降。 In order to remove heavy metal ions and organic pollutants in wastewater simultaneously, choosing cadmium ions (Cd2+) and acid orange 7 (AO7) as the target pollutants, we compared the removal effects of Cd2+ and AO7 in three systems, i.e. an activated carbon (AC) adsorption system alone, an pulsed corona discharge plasma combined (PCDP) treatment system alone, and a system that combined PCDP with AC (PCDP-AC) treatment system. We also investigated the effects of pulse discharge voltage, gas kinds, initial solution pH and electrical conductivity on the removal of Cd2+ and AO7 in the systems. The results show that Cd2+ and AO7 in wastewater are removed simultaneously by the PCDP-AC treatment system, with removal efficiency significantly higher than that in the AC adsorption system alone or the PCDP treatment system alone. An increasing pulsed voltage enhances the removal of Cd2+ and AO7. Compared with nitrogen or air, oxygen as the feeding gas will lead to a higher removal efficiency of Cd2+ and AO7. Lower pH benefits the removal of AO7, while higher pH helps to remove Cd2+. With the same input power and solution pH, increasing the solution's initial electrical conductivity reduces the efficiency of removing Cd2+ and AO7.
出处 《高电压技术》 EI CAS CSCD 北大核心 2014年第1期201-205,共5页 High Voltage Engineering
基金 国家自然科学基金(21107085) 中央高校基本科研业务费专项资金(QN2013073)~~
关键词 脉冲放电 等离子体 活性炭 重金属离子 有机污染物 废水处理 pulsed discharge plasma activated carbon heavy metal ions organic pollutants waste water treatment
  • 相关文献

参考文献13

  • 1Chen A W, Zeng G M, Chen G Q, et al. Simultaneous cadmium re- moval and 2,4-dichlorophenol degradation from aqueous solutions by P nology, 2011, 91(3): 811-821 J]. Applied Microbiology and Biotech-.
  • 2Chen A W, Zeng G M, Chen G Q, et al. Novel thiourea-modified magnetic ion-imprinted chitosan/TiO2 composite for simultaneous re- moval of cadmium and 2,4-dichlorophenol[J]. Chemical Engineering Journal, 2012, 191: 85-94.
  • 3Jin X L, Li Y F, Yu C, et al. Synthesis of novel inorganic-organic hybrid materials for simultaneous adsorption of metal ions and organic molecules in aqueous solution[J]. Journal of Hazardous Materials, 2011, 198: 247-256.
  • 4Tovar-G6mez R, Rivera-Ramirez D A, Hemhndez-Montoya V, et al. Synergic adsorption in the simultaneous removal of acid blue 25 and heavy metals from water using a Ca(POa)2-modified carbon[J]. Journal of Hazardous Materials, 2012, 199/200: 290-300.
  • 5王晓云,车向然.炼油废水水质特性及其治理技术[J].水科学与工程技术,2008(6):53-55. 被引量:23
  • 6刘成,周红蕾,张顺喜.重金属有机废水治理工艺进展[J].天津化工,2003,17(3):31-33. 被引量:3
  • 7WANG Huijuan. A synergistic process of pulsed discharge plas- ma-streamer photocatalysis for organic pollutants degradation in aqueous phase[D]. Dalian, China: Dalian University of Technology, 2007, 11-19.
  • 8蒋展鹏,杨津湘.苯酚与重金属在活性炭上的竞争吸附[J].水处理技术,1989,15(6):313-319. 被引量:6
  • 9孙冰,高志鹰,内爱,朱小梅,严志宇,宋艳静.多针-板脉冲放电气液混合反应器气液中活性物质的生成和转移特性[J].高电压技术,2013,39(1):109-116. 被引量:14
  • 10Sugiarto AT, Ohshima T, Sato M. Advanced oxidation processes using pulsedstreamer corona discharge in water[J]. Thin Solid Films, 2002, 407(1/2): 174-178.

二级参考文献88

  • 1张瑶,张克荣,罗永义,李崇福,蒋丽.活性炭对铅镉镍钴离子的吸附机理探讨[J].华西医科大学学报,1995,26(3):322-325. 被引量:16
  • 2张建策,毛立新.表面改性对活性炭吸附重金属性能的影响[J].化工时刊,2005,19(12):28-29. 被引量:21
  • 3文湘华,杜青,汤鸿霄.乐安江沉积物对重金属的吸附模式研究──表面络合模式在天然沉积物研究中的应用[J].环境科学学报,1996,16(1):12-22. 被引量:16
  • 4Mellor R B.Reduction of nitrate in water by immobilized enzymes[J].Nature,1992,355:717-719.
  • 5Teresa J. Bandosz, Jacek Jagiello, James A. Schwarz, Langmuir [ J ], 1996,12 (26) :6480 - 64 86.
  • 6Daniela M. Nevskaia, Eva Castillejos - Lopez, Antonio Guerrero - Ruiz, Carbon [ J ], 2004,42 (3) : 653 - 665.
  • 7Haghseresht, F., Nouri, S., Finnerty, J.J., Lu, G. Q. ,2002. Effects of surface chemistry on aromatic compound adsorption from dilute aqueous solutions by activated carbon [M]. J. Phys. Chem. B 106:10935 - 10943.
  • 8Dastgheib Seyed A, Rockstraw David A. A model for the adsorption of single metal ion solute - s in aqueous solution onto activated carbon produced from pecan shells [ J ]. Carbon, 2002(40) : 1843 - 1851.
  • 9Chu K H. Removal of copper from aqueous solution by chitosan in prawn shell: adsorption equilibrium and kinetics [ J]. Journal of Hazardous Materials B,2002(90) :77 - 95.
  • 10Maria Pesavento, Antonella Profumo, Giancarla Alberti, etal. Adsorption of lead( II) and cop - per(II) on activated carbon by complexation with surface fimctional groups [ J ]. Analytical Chi - mical Acta,2003 (480) : 171 - 180.

共引文献76

同被引文献487

引证文献20

二级引证文献182

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部