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汲取液对正渗透微生物燃料电池处理垃圾渗滤液的影响 被引量:1

Effect of draw solution on the performance of osmosis microbial fuel cell for landfill leachate treatment
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摘要 以垃圾渗滤液为阳极液,系统研究了汲取液种类和浓度对正渗透微生物燃料电池(OsMFC)工艺处理垃圾渗滤液性能的影响.结果表明,在汲取液为氯化钠的情况下,OsMFC工艺的最大功率密度可达0.44 W·m^(-2),表观内阻为236.75Ω,水通量为0.98 L·m^(-2)·h^(-1),TOC、NH_4^+-N、TN和TP的去除率分别达到89.51%、93.27%、94.01%和96.95%,均好于碳酸氢钠和碳酸氢铵作为汲取液时的处理效果.此外,氯化钠汲取液浓度越大,产电性能越好,表观内阻越小,水通量越大.产电性能随汲取液浓度的增大变化不大,在汲取液浓度为1 mol·L^(-1)的情况下,水通量和盐返混量的比值最大,处理效果最好. Effect of types and concentrations of draw solutions on the treatment of landfill leachate by osmosis microbial fuel cell( Os MFC) was systematically studied using the leachate as theanodic solution. Experimental results indicate that the Os MFC could achieve maximum power density of 0.44W·m^-2,apparent internal resistance of 236.75 Ω,water flux of 0.98 L·m^-2·h^-1,89.51% of TOC removal,93.27% of NH4+-N removal,94. 01% of TN removal,and 96. 95% of TP removalwhen employing sodium chloride as draw solution,which performed much better compared with that of sodium bicarbonate and ammonium bicarbonate. Furthermore,the power generation and water flux increased,while the apparent internal resistance decreased,with the increasingdraw solution concentration. The power generation performance change little with different draw solution concentration,and 1 mol·L^-1 was identified as optimal draw solution concentration due to the maximum ratio of water flux with reverse salt flux.
作者 黄丽 黄满红 陈亮 黄建乐 蔡腾 HUANG Li HUANG Manhong CHEN Liang HUANG Jianle CAI Teng(College of Environmental Science and Engineering, Donghua University, Shanghai 201620 National Environmental Protection Engineering Center for Pollution Prevention and Control (Textile Industry), Shanghai 201620)
出处 《环境科学学报》 CAS CSCD 北大核心 2017年第10期3830-3836,共7页 Acta Scientiae Circumstantiae
基金 国家自然科学基金(No.21477018 21507142) 交通运输部科技项目(No.2010353343290) 中央高校基本科研业务费专项资金重点项目(No.15D111323)~~
关键词 正渗透 微生物燃料电池 垃圾渗滤液 汲取液 产电性能 forward osmosis microbial fuel cell landfill leachate draw solution power generation
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