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Time-resolved evaluation of uranium plasma in different atmospheres by laser-induced breakdown spectroscopy 被引量:1

Time-resolved evaluation of uranium plasma in different atmospheres by laser-induced breakdown spectroscopy
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摘要 This work reports spectroscopic studies of uranium containing plasma generated in air and argon environments. The 532 nm Q-switched Nd:YAG laser generates the optical breakdown plasma, which was recorded by a spectrometer and an intensified charge coupled device having a resolution of 25 pm. Neutral and ionized uranium lines in the wavelength range of 385.8-391.9 nm indicate significant width and shift variations during the first few microseconds. Electron temperature and density of the plasma are determined using the Boltzmann plot and the Saha-Boltzmann equation at various time delay. The study reveals the power law decay pattern of electron temperature and density, which changes to exponential decay pattern if large gate- width is used to acquire the signal, due to an averaging effect. This work reports spectroscopic studies of uranium containing plasma generated in air and argon environments. The 532 nm Q-switched Nd:YAG laser generates the optical breakdown plasma, which was recorded by a spectrometer and an intensified charge coupled device having a resolution of 25 pm. Neutral and ionized uranium lines in the wavelength range of 385.8-391.9 nm indicate significant width and shift variations during the first few microseconds. Electron temperature and density of the plasma are determined using the Boltzmann plot and the Saha-Boltzmann equation at various time delay. The study reveals the power law decay pattern of electron temperature and density, which changes to exponential decay pattern if large gate- width is used to acquire the signal, due to an averaging effect.
出处 《Plasma Science and Technology》 SCIE EI CAS CSCD 2018年第12期65-74,共10页 等离子体科学和技术(英文版)
基金 supported by the fund obtained from DAE-BARC(ⅫPlan)
关键词 URANIUM laser induced plasma plasma parameter temporal evaluation electron temperature electron density LIBS uranium laser induced plasma plasma parameter temporal evaluation electron temperature electron density LIBS
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