摘要
In recent years,Perovskite Light-Emitting Diodes(PeLEDs)have received considerable attention in academia.However,with the development of PeLEDs,commercial applications of full-color PeLED technology are largely limited by the progress of blue-emitting devices,due to the uncontrollably accurate composition,unstable properties,and low luminance.In this article,we add Cesium chloride(CsCl)to the quasi-two-dimensional(quasi-2D)perovskite precursor solution and achieve the relatively blue shifts of PeLED emission peak by introducing chloride ions for photoluminescence(PL)and electroluminescence(EL).We also found that the introduction of chlorine ions can make quasi-2D perovskite films thinner with smoother surface of 0.408 nm.It is interesting that the EL peaks and intensities of PeLED are adjustable under different driving voltages in high concentration chlorine-added perovskite devices,and different processes of photo-excited,photo-quenched,and photo-excited occur sequentially with the increasing driving voltage.Our work provides a path for demonstrating full-color screens in the future.
基金
supported by the National Key Research and Development Program of China(No.2018YFB2200103)
the National Natural Science Foundation of China(Nos.61875186 and 61975196)
the Project of the Natural Science Foundation of Beijing(No.Z160002)
the Key Research Projects of Beijing Information Science and Technology University(BISTU)(Nos.2019-22,2019-23,2019-27)
the Beijing Key Laboratory for Sensors of BISTU(No.2019CGKF007)。
