摘要
CO_(2)光热催化转化是一种新型的CO_(2)利用技术,该过程绿色、经济且无须额外能量输入,是当下的热门研究领域之一。本文主要总结了CO_(2)光热催化转化领域的最新研究进展,介绍了基于光热转化的光热催化剂设计方法,同时从光热催化机理出发解析了CO_(2)还原反应的光热催化剂构建策略,并揭示了CO_(2)还原反应中的光热协同耦合机制,为光热催化剂的设计以及CO_(2)的高效转化和利用提供参考。
Photothermal catalytic conversion of CO_(2) is a new type of CO_(2) utilization technology.The process is green,economical,and requires no additional energy input.It is one of the current hot research fields.This paper introduced recent advances in photothermal catalytic conversion of CO_(2) and summarized design methods for photothermal catalysts based on photo-to-thermal conversion.In addition,fabrication strategies were also investigated in the perspective of photothermal catalytic mechanism and the synergy between photo-and thermo effects was also discussed.This work aims to promote the understanding of photothermal synergy for CO_(2) reduction reaction and provides reference for the design of photothermal catalysts and CO_(2) valorization.
作者
闫帅
杨海平
陈应泉
王贤华
曾阔
陈汉平
YAN Shuai;YANG Haiping;CHEN Yingquan;WANG Xianhua;ZENG Kuo;CHEN Hanping(State Key Laboratory of Coal Combustion,Huazhong University of Science and Technology,Wuhan 430074,Hubei,China)
出处
《化工学报》
EI
CSCD
北大核心
2022年第10期4298-4310,共13页
CIESC Journal
基金
国家杰出青年科学基金项目(52125601)。
关键词
CO_(2)利用
光热催化
光热转化
催化剂设计
CO_(2)utilization
photothermal catalysis
photothermal conversion
catalysts design