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不同地区自备井水的阴离子污染水平及其对人群的非致癌健康风险评估

Anion pollution level of self-supplied well water in different region and its non-carcinogenic health risk assessment to the population
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摘要 目的了解我国西藏、青海、广西、云南、黑龙江、北京、内蒙古共7个省、市、自治区的自备井水中4种阴离子F^(-)、Cl^(-)、NO_(3)--N和SO_(4)^(2-)的污染状况。按照美国环境保护局(US EPA)的健康风险评估模型评价健康风险。方法对我国7个省、市、自治区的自备井237份水样,按照《生活饮用水标准检验方法水样的采集和保存》(GB/T 5750.2—2006)进行采样,检测F^(-)、Cl^(-)、NO_(3)^(-)-N和SO_(4)4项水质指标并进行评价。使用US EPA的健康风险评估模型对F-和NO3--N进行非致癌风险评估。结果7个省、市、自治区的自备井水阴离子总不合格率为19.78%。各地区水质污染情况差异大。黑龙江和北京自备井F-和NO3--N超标;西藏和青海SO_(4)^(2-)和Cl^(-)超标;云南和广西NO3--N超标;内蒙古则4种阴离子均超标。7个省、市、自治区的自备井水F-和NO3--N的非致癌健康风险(HI)平均值较小,未超出最高可接受风险(HI<1),F-和NO_(3)^(-)-N均无显著的非致癌风险。结论与南方省份相比,北方自备井水阴离子污染严重,尤其以内蒙古的阴离子污染较为突出,应根据不同阴离子污染水平加强水质监测与净化,保障饮水安全。 Objective To determine the anion pollution level of self-supplied well water in seven provinces or cities of China(Tibet,Qinghai,Guangxi,Yunnan,Heilongjiang,Beijing,Inner Mongolia). The health risk assessment results were evaluated according to the US Environmental Protection Agency(US EPA)health risk assessment model. Methods Water was collected from 237 samples of self-supplied well water in seven provinces or cities of China according to Standard examination methods for drinking water-Collection and preservation of water samples(GB/T 5750.2—2006). The samples were tested for 4 water parameters including F^(-),Cl^(-),NO_(3)^(-)-N and SO_(4)^(2-). F-and NO_(3)^(-)-N were assessed for noncarcinogenic risks using the US EPA health risk assessment model. Results The total unqualified rate of water quality in self-supplied well water was 19.78%. There was significant difference in anion levels between the samples of well water from the 7 regions. F^(-)and NO_(3)^(-)-N were indicators of unqualified water from self-supplied wells in Heilongjiang and Beijing,compared with SO_(4)^(2-)and Cl^(-)in Tibet and Qinghai. NO3--N was the unqualified indicator of samples from Guangxi and Yunnan,and all the 4 types of anions were unqualified indicators of samples from Inner Mongolia. There was no significant non-carcinogenic risk in the average HI(HI<1) of F^(-)and NO_(3)^(-)-N in the self-supplied well water. Conclusion Compared with samples from the southern provinces,the anion pollution of water of self-supplied wells in the Northern provinces is more serious,especially in Inner Mongolia. To ensure the safety of drinking water,monitoring and purification of the self-supplied well water should be strengthened according to different levels of anion pollution.
作者 王天一 白淼 戚红卷 孟洋 张灿 张传福 WANG Tian-yi;BAI Miao;QI Hong-juan;MENG Yang;ZHANG Can;ZHANG Chuan-fu(Center for Disease Control and Prevention of Chinese PLA,Beijing 100071,China;Department of Environmental Science and Engineering,Beijing Technology and Business University,Beijing 100048,China)
出处 《军事医学》 CAS CSCD 2023年第2期135-140,共6页 Military Medical Sciences
基金 国家自然科学基金(52070193) 北京市自然科学基金(8192053) 军队保健专项(20BJZ17)。
关键词 自备井 水质检测 阴离子 健康风险评估 非致癌风险 self-supplied well water quality testing anion health risk assessment non-carcinogenic risk
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