摘要
CO_(2)的过量排放导致温室效应对环境的影响越来越严重,通过电催化、光催化、热催化、光热催化或光电催化将CO_(2)还原成高附加值的化学品是解决CO_(2)排放的有效途径.其中, CO_(2)的光热催化转化是当前的主要研究领域之一.我们对光热催化进行了总结分类:热助光、光助热、光驱热和光热协同催化,并详细介绍相应的催化机理,总结了金属催化剂用于光热催化CO_(2)还原的最新研究进展,最后提出了光热催化面临的挑战与展望.
Excessive emissions of CO_(2) lead to an increasingly serious environmental impact of the greenhouse effect.The reduction of CO_(2) into high value-added chemicals through electrocatalysis,photocatalysis,thermocatalysis,photothermal catalysis or photocatalysis is an effective way to address CO_(2) emissions.Among them,the photothermal catalytic conversion of CO_(2) is one of the main research areas at present.This paper summarises the classification of photothermal catalysis:thermal-assisted photocatalysis,photo-assisted thermocatalysis,photo-driven thermocatalysis and photo-thermal co-catalysis,and details the corresponding catalytic mechanisms,summarises the latest research progress on metal catalysts for photothermal catalytic CO_(2) reduction,and finally presents the challenges and prospects for photothermal catalysis.
作者
赫山林
王庆庆
李银辉
HE Shan-lin;WANG Qing-qing;LI Yin-hui(College of Chemical Engineering,Hebei University of Technology,Tianjin 300130,China)
出处
《分子催化》
CAS
CSCD
北大核心
2023年第5期512-521,I0004,共11页
Journal of Molecular Catalysis(China)
基金
国家留学基金(202106705005)。
