We investigate nonlinear interaction of nitrogen molecules with a two-color laser field composed by an intense 800 nm laser pulse and a weak 400 nm laser pulse.It is demonstrated that the spectrum of 400 nm pulses is ...We investigate nonlinear interaction of nitrogen molecules with a two-color laser field composed by an intense 800 nm laser pulse and a weak 400 nm laser pulse.It is demonstrated that the spectrum of 400 nm pulses is dramatically broadened when the two beams temporally overlap.In comparison,the spectral broadening in argon is less pronounced,although argon atoms and nitrogen molecules have comparable ionization potentials.We reveal that the dramatic spectral broadening originates from the greatly enhanced nonlinear optical effects in the near-resonant condition of interaction between the 400 nm pulses and the nitrogen molecular ions.展开更多
基金Supported by the National Key Research and Development Program of China under Grant No 2018YFB0504400the National Natural Science Foundation of China under Grant Nos 11822410,11734009 and 61575211+4 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences under Grant No XDB16030300the Key Research Program of Frontier Sciences of the Chinese Academy of Sciences under Grant No QYZDJ-SSW-SLH010the Key Project of the Shanghai Science and Technology Committee under Grant No 18DZ1112700the Shanghai Rising-Star Program under Grant No 17QA1404600the Youth Innovation Promotion Association of the Chinese Academy of Sciences under Grant No 2018284
文摘We investigate nonlinear interaction of nitrogen molecules with a two-color laser field composed by an intense 800 nm laser pulse and a weak 400 nm laser pulse.It is demonstrated that the spectrum of 400 nm pulses is dramatically broadened when the two beams temporally overlap.In comparison,the spectral broadening in argon is less pronounced,although argon atoms and nitrogen molecules have comparable ionization potentials.We reveal that the dramatic spectral broadening originates from the greatly enhanced nonlinear optical effects in the near-resonant condition of interaction between the 400 nm pulses and the nitrogen molecular ions.
基金the National Natural Science Foundation of China(11822410,12034013,11734009,and 11974245)the National Key R&D Program of China(2017YFA0303701 and 2019YFA0705000)+10 种基金the Shanghai Municipal Science and Technology Major Project(2019SHZDZX01)the Program of Shanghai Academic Research Leader(20XD1424200)the Natural Science Foundation of Shanghai(19ZR1475700)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB16030300)the Key Research Program of Frontier Sciences of Chinese Academy of Sciences(QYZDJ-SSW-SLH010)the Youth Innovation Promotion Association of Chinese Academy of Sciences(2018284)NSF(ECCS-1509268,and CMMI-1826078)AFOSR(FA9550-20-1-0366)partially supported by the Fundamental Research Funds for the Central Universitiesthe support from the Program for Professor of Special Appointment(Eastern Scholar)at Shanghai Institutions of Higher Learningthe support from Shandong Quancheng Scholarship(00242019024)。
