We numerically study the self-compression of the optical pulses centered at 1.8-μm in a hollow-core fiber （HCF） filled with argon. It is found that the pulse can be self-compressed to 2 optical cycles when the inpu...We numerically study the self-compression of the optical pulses centered at 1.8-μm in a hollow-core fiber （HCF） filled with argon. It is found that the pulse can be self-compressed to 2 optical cycles when the input pulse energy is 0.2-mJ and the gas pressure is 500-mbar （1 bar=10^5 Pa）. Inducing a proper positive chirp into the input pulse can lead to a shorter temporal duration after self-compression. These results will benefit the generation of energetic few-cycle mid-infrared pulses.展开更多
The compression of high-energy, linearly polarized pulses in a gas-filled hollow core fiber(HCF) by using a concentric phase mask is studied theoretically. Simulation results indicate that using a properly designed co...The compression of high-energy, linearly polarized pulses in a gas-filled hollow core fiber(HCF) by using a concentric phase mask is studied theoretically. Simulation results indicate that using a properly designed concentric phase mask, a40-fs input pulse centered at 800 nm with energy up to 10.0 mJ can be compressed to a full width at half maximum(FWHM) of less than 5 fs after propagating through a neon-filled HCF with a length of 1 m and diameter of 500 μm with a transmission efficiency of 67%, which is significantly higher than that without a concentric phase mask. Pulses with energy up to 20.0 mJ can also be efficiently compressed to less than 10 fs with the concentric phase mask. The higher efficiency due to the concentric phase mask can be attributed to the redistribution of the transverse intensity profile, which reduces the effect of ionization. The proposed method exhibits great potential for generating few-cycle laser pulse sources with high energy by the HCF compressor.展开更多
We perform a numerical study for temporally compressing radially-polarized（RP） infrared pulses in a gas-filled hollow-core fiber（HCF）. The dynamic transmission and nonlinear compression of RP pulses centered at wa...We perform a numerical study for temporally compressing radially-polarized（RP） infrared pulses in a gas-filled hollow-core fiber（HCF）. The dynamic transmission and nonlinear compression of RP pulses centered at wavelengths of0.8 m, 1.8 m, 3.1 m, and 5.0 m in HCFs are simulated. By comparing the propagation of pulses with the same optical cycles and intensity, we find that under proper conditions these pulses can be compressed down to 2–3 cycles. In the transverse direction, the spatiotemporal beam profile ameliorates from 0.8-m to 1.8-m and 3.1-m pulses before the appearance of high-order dispersion. These results show an alternative method of scaling generation for delivering RP infrared pulses in gas-filled HCFs, which can obtain energetic few-cycle pulses, and will be beneficial for relevant researches in the infrared scope.展开更多
We numerically study the propagation dynamics of intense optical pulses in gas-filled hollow-core fibers（HCFs）. The spatiotemporal dynamics of the pulses show a transition from tightly confined to loosely confined c...We numerically study the propagation dynamics of intense optical pulses in gas-filled hollow-core fibers（HCFs）. The spatiotemporal dynamics of the pulses show a transition from tightly confined to loosely confined characteristics as the fiber core is increased, which manifests as a deterioration in the spatiotemporal uniformity of the beam. It is found that using the gas pressure gradient does not enhance the beam quality in large-core HCFs, while inducing a positive chirp in the pulse to lower the peak power can improve the beam quality. This indicates that the self-focusing effect in the HCFs is the main driving force for the propagation dynamics. It also suggests that pulses at longer wavelengths are more suitable for HCFs with large cores because of the lower critical power of self-focusing, which is justified by the numerical simulations. These results will benefit the generation of energetic few-cycle pulses in large-core HCFs.展开更多
We theoretically study the field-free molecular orientation induced by a three-color laser field. The three-color laser field with a large asymmetric degree can effectively enhance the molecular orientation. In partic...We theoretically study the field-free molecular orientation induced by a three-color laser field. The three-color laser field with a large asymmetric degree can effectively enhance the molecular orientation. In particular, when the intensity ratio of the three-color laser field is tuned to a proper value of I3： I2： I1= 0.09 ： 0.5 ： 1, the molecular orientation can be improved by - 20% compared with that of the two-color laser field at intensity ratio I2： I1= 1 ： 1 for the same total laser intensity of 2×10^13W/cm^2. Moreover, we investigate the effect of the carrier-envelope phase（CEP） on the molecular orientation and use the asymmetric degree of the laser field to explain the result. We also show the influences of the laser intensity, rotational temperature, and pulse duration on the molecular orientation. These results are meaningful for the theoretical and experimental studies on the molecular orientation.展开更多
We numerically study the pulse compression approaches based on atomic or molecular gases in a hollow-core fiber.From the perspective of self-phase modulation（SPM）, we give the extensive study of the SPM influence on...We numerically study the pulse compression approaches based on atomic or molecular gases in a hollow-core fiber.From the perspective of self-phase modulation（SPM）, we give the extensive study of the SPM influence on a probe pulse with molecular phase modulation（MPM） effect. By comparing the two compression methods, we summarize their advantages and drawbacks to obtain the few-cycle pulses with micro- or millijoule energies. It is also shown that the double pump-probe approach can be used as a tunable dual-color source by adjusting the time delay between pump and probe pulses to proper values.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.61475169,61521093,and 11127901)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB16)the International Science and Technology Cooperation Program of China(Grant No.2016YFE0119300)
文摘We numerically study the self-compression of the optical pulses centered at 1.8-μm in a hollow-core fiber （HCF） filled with argon. It is found that the pulse can be self-compressed to 2 optical cycles when the input pulse energy is 0.2-mJ and the gas pressure is 500-mbar （1 bar=10^5 Pa）. Inducing a proper positive chirp into the input pulse can lead to a shorter temporal duration after self-compression. These results will benefit the generation of energetic few-cycle mid-infrared pulses.
基金Project supported by the National Natural Science Foundation of China(Grant No.61521093)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB1603)+1 种基金the International Science and Technology Cooperation Program of China(Grant No.2016YFE0119300)the Program of Shanghai Academic/Technology Research Leader,China(Grant No.18XD1404200)
文摘The compression of high-energy, linearly polarized pulses in a gas-filled hollow core fiber(HCF) by using a concentric phase mask is studied theoretically. Simulation results indicate that using a properly designed concentric phase mask, a40-fs input pulse centered at 800 nm with energy up to 10.0 mJ can be compressed to a full width at half maximum(FWHM) of less than 5 fs after propagating through a neon-filled HCF with a length of 1 m and diameter of 500 μm with a transmission efficiency of 67%, which is significantly higher than that without a concentric phase mask. Pulses with energy up to 20.0 mJ can also be efficiently compressed to less than 10 fs with the concentric phase mask. The higher efficiency due to the concentric phase mask can be attributed to the redistribution of the transverse intensity profile, which reduces the effect of ionization. The proposed method exhibits great potential for generating few-cycle laser pulse sources with high energy by the HCF compressor.
基金Project supported by the National Natural Science Foundation of China(Grant No.61521093)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB16)+1 种基金the International S&T Cooperation Program of China(Grant No.2016YFE0119300)the Program of Shanghai Academic/Technology Research Leader,China(Grant No.18XD1404200)
文摘We perform a numerical study for temporally compressing radially-polarized（RP） infrared pulses in a gas-filled hollow-core fiber（HCF）. The dynamic transmission and nonlinear compression of RP pulses centered at wavelengths of0.8 m, 1.8 m, 3.1 m, and 5.0 m in HCFs are simulated. By comparing the propagation of pulses with the same optical cycles and intensity, we find that under proper conditions these pulses can be compressed down to 2–3 cycles. In the transverse direction, the spatiotemporal beam profile ameliorates from 0.8-m to 1.8-m and 3.1-m pulses before the appearance of high-order dispersion. These results show an alternative method of scaling generation for delivering RP infrared pulses in gas-filled HCFs, which can obtain energetic few-cycle pulses, and will be beneficial for relevant researches in the infrared scope.
文摘We numerically study the propagation dynamics of intense optical pulses in gas-filled hollow-core fibers（HCFs）. The spatiotemporal dynamics of the pulses show a transition from tightly confined to loosely confined characteristics as the fiber core is increased, which manifests as a deterioration in the spatiotemporal uniformity of the beam. It is found that using the gas pressure gradient does not enhance the beam quality in large-core HCFs, while inducing a positive chirp in the pulse to lower the peak power can improve the beam quality. This indicates that the self-focusing effect in the HCFs is the main driving force for the propagation dynamics. It also suggests that pulses at longer wavelengths are more suitable for HCFs with large cores because of the lower critical power of self-focusing, which is justified by the numerical simulations. These results will benefit the generation of energetic few-cycle pulses in large-core HCFs.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61221064,61078037,11134010,61205208,and 61521093)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB16)the International S&T Cooperation Program of China(Grant No.2016YFE0119300)
文摘We theoretically study the field-free molecular orientation induced by a three-color laser field. The three-color laser field with a large asymmetric degree can effectively enhance the molecular orientation. In particular, when the intensity ratio of the three-color laser field is tuned to a proper value of I3： I2： I1= 0.09 ： 0.5 ： 1, the molecular orientation can be improved by - 20% compared with that of the two-color laser field at intensity ratio I2： I1= 1 ： 1 for the same total laser intensity of 2×10^13W/cm^2. Moreover, we investigate the effect of the carrier-envelope phase（CEP） on the molecular orientation and use the asymmetric degree of the laser field to explain the result. We also show the influences of the laser intensity, rotational temperature, and pulse duration on the molecular orientation. These results are meaningful for the theoretical and experimental studies on the molecular orientation.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11204328,61221064,61078037,11127901,11134010,and 61205208)the National Basic Research Program of China(Grant No.2011CB808101)the Natural Science Foundation of Shanghai,China(Grant No.13ZR1414800)
文摘We numerically study the pulse compression approaches based on atomic or molecular gases in a hollow-core fiber.From the perspective of self-phase modulation（SPM）, we give the extensive study of the SPM influence on a probe pulse with molecular phase modulation（MPM） effect. By comparing the two compression methods, we summarize their advantages and drawbacks to obtain the few-cycle pulses with micro- or millijoule energies. It is also shown that the double pump-probe approach can be used as a tunable dual-color source by adjusting the time delay between pump and probe pulses to proper values.
