Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been dev...Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been developed to some extent but still lack underwater in-situ measurements.Here we present an in-situ detection equipment for radon-in-water(pulsed ionization chamber(PIC)-radon)to measure dissolved radon in ocean and groundwater settings.The equipment has been successfully deployed in the Jiaozhou Bay in July 2022 and has achieved 14 d of unattended underwater in-situ observation.Then it was successfully placed in a groundwater monitoring well in the Laizhou Bay in November 2022 and monitored radon activities for over 30 d.The results showed that this instrument had a good indication of submarine groundwater discharge.The PIC-radon detector takes advantage of smaller size,lower power consumption,and is barely influenced by humidity,making it particularly suitable for long-term in-situ measurement,especially in harsh environments with limited human care or deployment spaces.展开更多
As an important land-ocean interaction process,submarine groundwater discharge(SGD)is composed of multiple dynamical processes at different scales and plays an important role in the study of coastal ocean geochemical ...As an important land-ocean interaction process,submarine groundwater discharge(SGD)is composed of multiple dynamical processes at different scales and plays an important role in the study of coastal ocean geochemical budgets.However,most of the existing studies focus on the quantification of the total groundwater discharge,few studies are about the differentiation and quantification of groundwater discharge processes at different scales(i.e.,short-scale SGD and long-scale SGD).As a world-class river,the Huanghe River is highly turbid and heavily regulated by humans.These natural and anthropogenic factors have a significant impact on groundwater discharge processes in the Huanghe River Estuary(HRE).In this study,the distribution patterns of the natural geochemical tracer radium isotopes(^(224)Ra and^(223)Ra)and other hydrological parameters in the HRE were investigated during four cruises.By solving the mass balance of^(224)Ra and^(223)Ra in the HRE,the long-scale SGD flux was quantified as 0.01−0.19 m/d,and the short-scale SGD flux was 0.03−0.04 m/d.The rate of short-scale SGD remained essentially constant among seasons,while the rate of long-scale SGD varied considerably at different periods and showed a synchronous trend with the variation of river discharge.The results of this study are significant for understanding the SGD dynamics in the HRE and the contribution of SGD to the ocean geochemical budgets.展开更多
基金The National Natural Science Foundation of China under contract Nos U22A20580 and 42130410the Fundamental Research Funds for the Central Universities under contract No.202341002the Pilot Project for the Integration of Science,Education,and Industry under contract No.2022PY069.
文摘Radon is recognized as a powerful tracer of certain geophysical processes in marine and aquatic environments.In the past few decades,the instruments and methods for measuring radon concentration in water have been developed to some extent but still lack underwater in-situ measurements.Here we present an in-situ detection equipment for radon-in-water(pulsed ionization chamber(PIC)-radon)to measure dissolved radon in ocean and groundwater settings.The equipment has been successfully deployed in the Jiaozhou Bay in July 2022 and has achieved 14 d of unattended underwater in-situ observation.Then it was successfully placed in a groundwater monitoring well in the Laizhou Bay in November 2022 and monitored radon activities for over 30 d.The results showed that this instrument had a good indication of submarine groundwater discharge.The PIC-radon detector takes advantage of smaller size,lower power consumption,and is barely influenced by humidity,making it particularly suitable for long-term in-situ measurement,especially in harsh environments with limited human care or deployment spaces.
基金The National Natural Science Foundation of China under contract Nos U22A20580,42130410,U2106203 and 41977173the Fundamental Research Funds for the Central Universities,China under contract No.202341002.
文摘As an important land-ocean interaction process,submarine groundwater discharge(SGD)is composed of multiple dynamical processes at different scales and plays an important role in the study of coastal ocean geochemical budgets.However,most of the existing studies focus on the quantification of the total groundwater discharge,few studies are about the differentiation and quantification of groundwater discharge processes at different scales(i.e.,short-scale SGD and long-scale SGD).As a world-class river,the Huanghe River is highly turbid and heavily regulated by humans.These natural and anthropogenic factors have a significant impact on groundwater discharge processes in the Huanghe River Estuary(HRE).In this study,the distribution patterns of the natural geochemical tracer radium isotopes(^(224)Ra and^(223)Ra)and other hydrological parameters in the HRE were investigated during four cruises.By solving the mass balance of^(224)Ra and^(223)Ra in the HRE,the long-scale SGD flux was quantified as 0.01−0.19 m/d,and the short-scale SGD flux was 0.03−0.04 m/d.The rate of short-scale SGD remained essentially constant among seasons,while the rate of long-scale SGD varied considerably at different periods and showed a synchronous trend with the variation of river discharge.The results of this study are significant for understanding the SGD dynamics in the HRE and the contribution of SGD to the ocean geochemical budgets.
