Metal-halide perovskites have garnered considerable research attention as highly efficient light emitters in recent years due to their outstanding optoelectronic properties with remarkable tunability and excellent sol...Metal-halide perovskites have garnered considerable research attention as highly efficient light emitters in recent years due to their outstanding optoelectronic properties with remarkable tunability and excellent solution processabilities.Substantial advancements have been achieved in the development of novel halide perovskites,and the exploitations of these materials in lightemitting devices.This review comprehensively outlines recent breakthroughs in metal-halide perovskites,encompassing the rational design of perovskite materials with tunable light emission properties,the controllable growth of single crystal for a deeper understanding of their structure-property relationships,as well as the fundamental insights into the photophysics and carrier dynamics in perovskite systems.Additionally,it provides an overview of recent applications of perovskite materials in high-performance light-emitting diodes(LEDs)and lasers.展开更多
Laser displays,benefiting from the characteristic merits of lasers,have led to the revolution of next-generation display technologies owing to their superior color expression.However,the acquisition of pixelated laser...Laser displays,benefiting from the characteristic merits of lasers,have led to the revolution of next-generation display technologies owing to their superior color expression.However,the acquisition of pixelated laser arrays as self-emissive panels for flat-panel laser displays remains challenging.Liquid crystal(LC)materials with excellent processability and optoelectronic properties offer considerable potential for the construction of highly ordered multicolor laser arrays.Here,we demonstrate flat-panel laser displays on LC microlaser pixel arrays through a microtemplate-assisted inkjet printing method.Individual organic red-green-blue(RGB)microlaser pixel arrays were obtained by doping dyes into LCs with photonic band edges to obtain single-mode RGB lasing,leading to a much broader color gamut,compared with the standard RGB color space.Then we acquired periodically patterned RGB pixel matrices by positioning LC microlasers precisely into highly ordered arrays,according to the well-organized geometry of the microtemplates.Subsequently,we demonstrated full-color flat-panel laser displays using the LC microlaser pixel matrices as self-emissive panels.These results provide valuable enlightenment for the construction of next-generation flat-panel laser display devices.展开更多
Organic composite materials have been attracting extensive research interest for light-emitting applications.A wide variety of luminescent organic composite materials have been synthesized,which are of great significa...Organic composite materials have been attracting extensive research interest for light-emitting applications.A wide variety of luminescent organic composite materials have been synthesized,which are of great significance for both the investigation of basic photophysics and the realization of high-performance photonic devices.Function-oriented syntheses of luminescent organic composite materials rely on the understanding and manipulating of molecular excited states.In this review,we focus on the discussion about the structure design and dynamics modulation of the electronic excited states in the organic composite materials.The excited-state structures and dynamics involve singlet/triplet levels,vibronic transition,charge transfer,and energy transfer,and so on,while the light-emitting behaviors include fluorescence,phosphorescence,persistent luminescence,electroluminescence,and lasing.We aim to give insight into the relationship between light-emitting properties and excited states of organic composite materials,which is beneficial for reaching higher tiers of design and applications of luminescent organic composite materials.展开更多
The discovery and continued development of the lasers have led to a revolution in both fundamental researches and optoelectronic industry.Recently,micro/nanolasers that can generate intense coherent light signals at(s...The discovery and continued development of the lasers have led to a revolution in both fundamental researches and optoelectronic industry.Recently,micro/nanolasers that can generate intense coherent light signals at(sub)wavelength scale have become a research focus due to their potential applications in a variety of fields ranging from chemical and biological sensing to integrated optoelectronic circuitry[1,2].Organic materials are a kind of excel-展开更多
Over the past sixty years,lasers have undergone substantial developments and have revolutionized sciences,technologies,and industries.In particular,the invention of compact semiconductor lasers has made this technolog...Over the past sixty years,lasers have undergone substantial developments and have revolutionized sciences,technologies,and industries.In particular,the invention of compact semiconductor lasers has made this technology an integral part of everyday life.Metal halide perovskites have recently emerged as an outstanding class of semiconductors holding great potentials in further advancing the laser technology[1].展开更多
基金financially supported by the National Natural Science Foundation of China(2131608-ECCS)the Ministry of Science and Technology of China(2022YFA1204403)National Natural Science Foundation of China(22090023)。
文摘Metal-halide perovskites have garnered considerable research attention as highly efficient light emitters in recent years due to their outstanding optoelectronic properties with remarkable tunability and excellent solution processabilities.Substantial advancements have been achieved in the development of novel halide perovskites,and the exploitations of these materials in lightemitting devices.This review comprehensively outlines recent breakthroughs in metal-halide perovskites,encompassing the rational design of perovskite materials with tunable light emission properties,the controllable growth of single crystal for a deeper understanding of their structure-property relationships,as well as the fundamental insights into the photophysics and carrier dynamics in perovskite systems.Additionally,it provides an overview of recent applications of perovskite materials in high-performance light-emitting diodes(LEDs)and lasers.
基金supported financially by the Ministry of Science and Technology of China(no.2017YFA0204502)the National Natural Science Foundation of China(grant nos.21533013 and 21790364).
文摘Laser displays,benefiting from the characteristic merits of lasers,have led to the revolution of next-generation display technologies owing to their superior color expression.However,the acquisition of pixelated laser arrays as self-emissive panels for flat-panel laser displays remains challenging.Liquid crystal(LC)materials with excellent processability and optoelectronic properties offer considerable potential for the construction of highly ordered multicolor laser arrays.Here,we demonstrate flat-panel laser displays on LC microlaser pixel arrays through a microtemplate-assisted inkjet printing method.Individual organic red-green-blue(RGB)microlaser pixel arrays were obtained by doping dyes into LCs with photonic band edges to obtain single-mode RGB lasing,leading to a much broader color gamut,compared with the standard RGB color space.Then we acquired periodically patterned RGB pixel matrices by positioning LC microlasers precisely into highly ordered arrays,according to the well-organized geometry of the microtemplates.Subsequently,we demonstrated full-color flat-panel laser displays using the LC microlaser pixel matrices as self-emissive panels.These results provide valuable enlightenment for the construction of next-generation flat-panel laser display devices.
基金Ministry of Science andTechnology of China,Grant/Award Number:2017YFA0204502National Natural Science Foundation of China,Grant/Award Numbers:22090023,21790364,51903238+1 种基金Postdoctoral InnovationTalent Support Project,Grant/Award Number:BX20180314China Postdoctoral Science Foundation,Grant/Award Number:2019M650854。
文摘Organic composite materials have been attracting extensive research interest for light-emitting applications.A wide variety of luminescent organic composite materials have been synthesized,which are of great significance for both the investigation of basic photophysics and the realization of high-performance photonic devices.Function-oriented syntheses of luminescent organic composite materials rely on the understanding and manipulating of molecular excited states.In this review,we focus on the discussion about the structure design and dynamics modulation of the electronic excited states in the organic composite materials.The excited-state structures and dynamics involve singlet/triplet levels,vibronic transition,charge transfer,and energy transfer,and so on,while the light-emitting behaviors include fluorescence,phosphorescence,persistent luminescence,electroluminescence,and lasing.We aim to give insight into the relationship between light-emitting properties and excited states of organic composite materials,which is beneficial for reaching higher tiers of design and applications of luminescent organic composite materials.
基金supported by Beijing Municipal Natural Science Foundation (2142017)the National Natural Science Foundation of China (21533013)the Chinese Academy of Sciences (XDB12030300)
文摘The discovery and continued development of the lasers have led to a revolution in both fundamental researches and optoelectronic industry.Recently,micro/nanolasers that can generate intense coherent light signals at(sub)wavelength scale have become a research focus due to their potential applications in a variety of fields ranging from chemical and biological sensing to integrated optoelectronic circuitry[1,2].Organic materials are a kind of excel-
文摘Over the past sixty years,lasers have undergone substantial developments and have revolutionized sciences,technologies,and industries.In particular,the invention of compact semiconductor lasers has made this technology an integral part of everyday life.Metal halide perovskites have recently emerged as an outstanding class of semiconductors holding great potentials in further advancing the laser technology[1].
