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原子转移自由基聚合法制备氮卤胺型抗菌棉织物及性能 被引量:1
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作者 彭盼盼 杨建军 +4 位作者 程传政 吴庆云 吴明元 张建安 刘久逸 《高分子材料科学与工程》 EI CAS CSCD 北大核心 2023年第8期17-25,共9页
合成了氮卤胺前驱体2-(3-(6-甲基-4-氧-1,4-二氢嘧啶-2-基)脲基)甲基丙烯酸乙酯(SCMHBMA),通过原子转移自由基聚合(ATRP)法接枝在棉织物表面,制备出棉织物接枝SCMHBMA聚合物(Cotton-g-PSMA),通过氯化处理得到抗菌棉织物。探究了棉织物... 合成了氮卤胺前驱体2-(3-(6-甲基-4-氧-1,4-二氢嘧啶-2-基)脲基)甲基丙烯酸乙酯(SCMHBMA),通过原子转移自由基聚合(ATRP)法接枝在棉织物表面,制备出棉织物接枝SCMHBMA聚合物(Cotton-g-PSMA),通过氯化处理得到抗菌棉织物。探究了棉织物接枝前后的元素变化、热力学性能等,并对氯化后的棉织物进行储存稳定性、洗涤耐久性和抗菌性能测试。结果表明,氯化棉织物(Cotton-g-PSMA-Cl)经过5次洗涤和60 d常规储存后,活性氯浓度(Cl^(+)%)仅分别降低22%和18%,并且降低的活性有效氯可以通过简单的再氯化作用得到有效的提高。在抗菌测试中,抗菌棉织物Cotton-g-PSMA-Cl与金黄色葡萄球菌和大肠杆菌接触1 min后,基本杀灭100%菌株。合成出的氮卤胺型抗菌棉织物表现优异的抗菌性能,在长期抗菌领域具有广阔的应用前景。 展开更多
关键词 氮卤胺 抗菌 棉织物
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Rational construction and decoration of Li_(5)Cr_(7)Ti_(6)O_(25)@Cnanofibers as stable lithium storage materials 被引量:5
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作者 Ting-Ting Wei panpan peng +3 位作者 Yu-Rui Ji Yan-Rong Zhu Ting-Feng Yi Ying Xie 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2022年第8期400-410,I0011,共12页
Li_(5)Cr_(7)Ti_(6)O_(25) is regarded as a promising anode material for Li-ion batteries(LIBs)because of its low cost and high theoretical capacity.However,the inherently poor conductivity significantly limits the enha... Li_(5)Cr_(7)Ti_(6)O_(25) is regarded as a promising anode material for Li-ion batteries(LIBs)because of its low cost and high theoretical capacity.However,the inherently poor conductivity significantly limits the enhancement of its rate capability and cycling stability,especially at high current densities.In this work,we construct one-dimensional Li_(5)Cr_(7)Ti_(6)O_(25)/C nanofibers by electrospinning method to enhance the kinetic,which realizes high cycling stability.Carbon coating enhances the structure stability,insertion/extraction reversibility of Li-ions and electrochemical reaction activity,and facilitates the transfer of Li-ions.Benefited from the unique architecture and component,the Li_(5)Cr_(7)Ti_(6)O_(25)/C(6.6 wt%)nanofiber shows an excellent rate capability with a reversible de-lithiation capacity of 370.8,290.6,269.2,254.3 and 244.9 m Ah g^(-1) at 200,300,500,800 and 1000 m A g^(-1),respectively.Even at a higher current density of 1 A g^(-1),Li_(5)Cr_(7)Ti_(6)O_(25)/C(6.6 wt%)nanofiber shows high cycling stability with an initial de-lithiation capacity of 237.8 m Ah g^(-1) and a capacity retention rate of about 84%after 500 cycles.The density functional theory calculation result confirms that the introduction of carbon on the surface of Li_(5)Cr_(7)Ti_(6)O_(25) changes the total density of states of Li_(5)Cr_(7)Ti_(6)O_(25),and thus improves electronic conductivity of the composite,resulting in a good electrochemical performance of Li_(5)Cr_(7)Ti_(6)O_(25)/C nanofibers.Li_(5)Cr_(7)Ti_(6)O_(25)/C nanofibers indicate a great potential as an anode material for the next generation of high-performance LIBs. 展开更多
关键词 Lithium-ion battery Anode Li_(5)Cr_(7)Ti_(6)O_(25) Electrospinning NANOFIBERS
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Advancement of technology towards high-performance non-aqueous aluminum-ion batteries 被引量:2
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作者 Ting-Ting Wei panpan peng +2 位作者 Si-Yu Qi Yan-Rong Zhu Ting-Feng Yi 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2021年第6期169-188,I0005,共21页
Al-ion batteries(AIBs) have been identified as one of the most hopeful energy storage systems after Li-ion batteries on account for the ultrahigh volumetric capacity,high safety and low cost from the rich abundance of... Al-ion batteries(AIBs) have been identified as one of the most hopeful energy storage systems after Li-ion batteries on account for the ultrahigh volumetric capacity,high safety and low cost from the rich abundance of Al.Nonetheless,some inevitable shortcomings,such as the formation of passive oxide film,hydrogen side reactions and anode corrosion,finally limit the large-scale application of aqueous AIBs.The nonaqueous AIBs have been considered as one of most hopeful alternatives for high-powered electrochemical energy storage devices.Nonetheless,various technical and scientific obstacles should be resolved because nonaqueous AIBs are still nascent.Some significant efforts have aimed to resolve these issues towards large-scale applications,and some important advancement has been made.In the present review,we mainly intended to offer an overview of non-aqueous AIBs systems,and we comprehensively reviewed the recent research advancement of the cathode materials,anode materials electrolyte and collectors as well as the fundamental understanding of the functional mechanisms.In addition,we have also analyzed several technical challenges and summarized the strategies used for overcoming the challenges in improving the electrochemical properties,including morphology control,surface engineering,doping and construction of composite electrodes as well as the charge storage mechanisms of the materials with different crystal structures.At last,future research orientation and development prospect of the AIBs are proposed. 展开更多
关键词 Al-ion batteries ELECTRODE ELECTROLYTE COLLECTOR Electrochemical performance
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