The strong-field coherent control of the nonresonant ionization of nitrous oxide using shaped pulses is investigated.We study the dependence of periodic coherent oscillation of the total ionization yield on the variat...The strong-field coherent control of the nonresonant ionization of nitrous oxide using shaped pulses is investigated.We study the dependence of periodic coherent oscillation of the total ionization yield on the variation of laser phase parameters. The physical mechanism of the strong-field coherent control is investigated experimentally and theoretically by the nonresonant spectral phase interferences in the frequency domain. We show that the intense shaped pulses with broadband and off-resonance can be used as a robust strong-field coherent control method.展开更多
In this work, we mainly investigate the NH3 molecular multiphoton ionization process by using the photoelectron velocity map imaging technique. Under the condition of femtosecond laser(wavelength at 800 nm), the photo...In this work, we mainly investigate the NH3 molecular multiphoton ionization process by using the photoelectron velocity map imaging technique. Under the condition of femtosecond laser(wavelength at 800 nm), the photoelectron images are detected. The channel switching and above-threshold ionization(ATI) effect are also confirmed. The kinetic energy spectrum(KES) and the photoelectron angular distributions(PADs) are obtained through the anti-Abel transformation from the original images, and then three ionization channels are confirmed successfully according to the Freeman resonance effect in a relatively low laser intensity region. In the excitation process, the intermediate resonance Rydberg states are C^1 A 1(6 + 2 photons process), B^1 E(6 + 2 photons process) and C^1 A 1(7 + 2 photons process), respectively. At the same time, we also find that the photoelectron angular distributions are independent of laser intensity. In addition, the electrons produced by different processes interfere with each other and they can produce a spider-like structure. We also find ac-Stark movement according to the Stark-shift-induced resonance effect when the laser intensity is relatively high.展开更多
Coherent control of fragmentation of CH_3I using shaped femtosecond pulse train is investigated.The dissociation processes can be modulated by changing the separation of the shaped pulse train, and the yield of I^+und...Coherent control of fragmentation of CH_3I using shaped femtosecond pulse train is investigated.The dissociation processes can be modulated by changing the separation of the shaped pulse train, and the yield of I^+under the irradiation of the optimal pulse is significantly increased compared with that using the transform-limited pulse.We discuss the control mechanism of dissociation processes with coherent interference in time domain.A three-pulse control model is proposed to explain the counterintuitive experimental results.展开更多
基金supported by the National Natural Science Foundation of China(Grant No.11374124)
文摘The strong-field coherent control of the nonresonant ionization of nitrous oxide using shaped pulses is investigated.We study the dependence of periodic coherent oscillation of the total ionization yield on the variation of laser phase parameters. The physical mechanism of the strong-field coherent control is investigated experimentally and theoretically by the nonresonant spectral phase interferences in the frequency domain. We show that the intense shaped pulses with broadband and off-resonance can be used as a robust strong-field coherent control method.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11574116,11534004,10704028,and 11474123)
文摘In this work, we mainly investigate the NH3 molecular multiphoton ionization process by using the photoelectron velocity map imaging technique. Under the condition of femtosecond laser(wavelength at 800 nm), the photoelectron images are detected. The channel switching and above-threshold ionization(ATI) effect are also confirmed. The kinetic energy spectrum(KES) and the photoelectron angular distributions(PADs) are obtained through the anti-Abel transformation from the original images, and then three ionization channels are confirmed successfully according to the Freeman resonance effect in a relatively low laser intensity region. In the excitation process, the intermediate resonance Rydberg states are C^1 A 1(6 + 2 photons process), B^1 E(6 + 2 photons process) and C^1 A 1(7 + 2 photons process), respectively. At the same time, we also find that the photoelectron angular distributions are independent of laser intensity. In addition, the electrons produced by different processes interfere with each other and they can produce a spider-like structure. We also find ac-Stark movement according to the Stark-shift-induced resonance effect when the laser intensity is relatively high.
基金Project supported by the National Natural Science Foundation of China(Grant No.11374124)
文摘Coherent control of fragmentation of CH_3I using shaped femtosecond pulse train is investigated.The dissociation processes can be modulated by changing the separation of the shaped pulse train, and the yield of I^+under the irradiation of the optimal pulse is significantly increased compared with that using the transform-limited pulse.We discuss the control mechanism of dissociation processes with coherent interference in time domain.A three-pulse control model is proposed to explain the counterintuitive experimental results.
