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Response of warm season secondary pollutants to emissions and meteorology in the North China Plain region during 2018-2022
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作者 Yueqi Gao Siyu Wang +7 位作者 Zhaolei Zhang Wenxuan Yu Shuai Wang shengqiang zhu Peng Wang Yan Li Yele Sun Hongliang Zhang 《Atmospheric and Oceanic Science Letters》 CSCD 2024年第4期58-64,共7页
自2013年起中国空气质量虽改善,但华北平原(NCP)重污染仍存在且二次污染加剧,而人们对其成因和变化了解有限.本研究利用2018-2022年数据,借助CMAQ模型探讨此污染响应.结果显示,在2018-2022年间,PM_(2.5)浓度显著下降31%-37%,O_(3)和NO_... 自2013年起中国空气质量虽改善,但华北平原(NCP)重污染仍存在且二次污染加剧,而人们对其成因和变化了解有限.本研究利用2018-2022年数据,借助CMAQ模型探讨此污染响应.结果显示,在2018-2022年间,PM_(2.5)浓度显著下降31%-37%,O_(3)和NO_(2)的年下降速率分别为1%和0.5%SIA和SOA也显著减少,每年分别减少9%和6%PM_(2.5)主要因排放减少而下降,而O_(3)则受气象影响而波动.硫酸盐和铵下降的主因是减排,而硝酸盐对气象变化敏感排放和气象变化对SOA的总体减少同样重要,但人为SOA对排放控制敏感生物SOA易受气象变化影响.研究强调了控制人为排放对缓解NCP地区夏季二次污染的重要性. 展开更多
关键词 PM_(2.5) 二次污染物 人为排放 气象 华北平原
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Linking Perceived Risk of Public Health Emergency to Psychological Distress among Chinese College Students: The Chain Mediation Role of Balanced Time Perspective and Negative Coping Styles
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作者 Biru Chang shengqiang zhu +1 位作者 Qian Xie Yanghui Dai 《International Journal of Mental Health Promotion》 2024年第8期599-610,共12页
Background:With public health emergencies(PHE)worldwide increasing,the perceived risk of PHE has been one of the critical factors influencing college students’psychological distress.However,the mechanisms by which th... Background:With public health emergencies(PHE)worldwide increasing,the perceived risk of PHE has been one of the critical factors influencing college students’psychological distress.However,the mechanisms by which the perceived risk of PHE affects college students’psychological distress are not clear.The study’s purpose was to investigate the mediation roles of deviation from a balanced time perspective(DBTP)and negative coping styles between the perceived risk of PHE and psychological distress.Methods:A convenience sampling method was used to survey 1054 Chinese college students with self-reporting.Data was collected using the Public Risk Perception Scale(PRPS),the Zimbardo Time Perspective Inventory(ZTPI),the Simplified Coping Style Questionnaire(SCSQ),the PHE Anxiety Scale,and the Chinese version of the Patient Health Questionnaire(PHQ).The associations between the perceived risk of PHE,DBTP,negative coping styles,and psychological distress were clarified using the correlation analysis.Additionally,the mediating roles of DBTP and negative coping styles between the perceived risk of PHE and psychological distress were investigated using a structural equation model.Results:The findings revealed low to moderate correlations between the variables studied.Students’perceived risk of PHE was a positive predictor of their psychological distress(b=0.219,p<0.01).DBTP and negative coping styles played chain mediation roles between them with the effect being 0.009 and a 95%Boot CI of[0.003,0.023].This chain mediation model had an excellent fit index(χ^(2)/df=4.732,CFI=0.973,TLI=0.930,RMSEA=0.048,SRMR=0.047).Conclusion:These findings showed how the perceived risk of PHE affected college students’psychological distress.Specifically,these results suggested that improving students’mental ability to switch effectively among different time perspectives depending on task features and situational considerations and reducing their negative coping styles might be effective ways to promote their mental health. 展开更多
关键词 Perceived risk of public health emergency balanced time perspective negative coping styles psychological distress college students China
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Consumption Based Source Apportionment Indicates Different Regional Contributions to O3 Concentrations and Health Effects
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作者 shengqiang zhu Peng Wang +4 位作者 Siyu Wang Guannan Geng Hongyan Zhao Yuan Wang Hongliang Zhang 《Engineering》 SCIE EI CAS CSCD 2023年第9期130-138,共9页
China is confronting aggravated ozone(O_(3))pollution,leading to adverse health impacts.This study quantifies the regional contributions to O_(3)in China using two approaches;estimating(1)where goods are produced(the ... China is confronting aggravated ozone(O_(3))pollution,leading to adverse health impacts.This study quantifies the regional contributions to O_(3)in China using two approaches;estimating(1)where goods are produced(the production method),and(2)where goods are consumed(the consumption method).The production method predicts higher local source contribution than the consumption method;this difference can be attributed to exports.Occurrence of high-O_(3)episodes suggests a major contribution to O_(3)concentration as a result of trade activities.Based on the consumption method,9219 out of 18532 daily premature mortalities were caused by local sources in north China,while it increased to 14471 of the production method when neglecting contributions due to export and consumption in other regions.This study suggests that O_(3)control should consider both where goods are consumed and emissions are emitted,especially taking account of international trade activities. 展开更多
关键词 O_(3)pollution TRADE Source-oriented CMAQ Health risks
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大气氧化性及其对二次污染物形成的贡献 被引量:11
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作者 王芃 朱盛强 +3 位作者 张梦媛 邵田 Qi Ying 张宏亮 《科学通报》 EI CAS CSCD 北大核心 2022年第18期2069-2078,共10页
大气氧化性(atmospheric oxidation capacity,AOC)是指大气化学过程对一次污染物的氧化能力,一般用氧化剂的浓度或者总反应速率来表征.AOC对二次污染的形成起重要的作用,是研究二次污染物的重要指标.本研究利用三维空气质量模式(Communi... 大气氧化性(atmospheric oxidation capacity,AOC)是指大气化学过程对一次污染物的氧化能力,一般用氧化剂的浓度或者总反应速率来表征.AOC对二次污染的形成起重要的作用,是研究二次污染物的重要指标.本研究利用三维空气质量模式(Community Multi-scale Air Quality model,CMAQ)模拟了2013和2020年我国主要大气氧化剂(HO_(2)、OH和NO_(3)自由基)与二次污染物(臭氧和二次颗粒物)及其前体物,并结合观测数据,综合讨论了AOC对二次污染物生成的作用.结果表明,从2013~2020年,颗粒物浓度显著下降,而AOC水平并未明显降低,甚至在华北平原(NCP)和珠江三角洲(PRD)地区还略有上升.主要氧化剂浓度呈现一定的区域特征,HO_(x)(OH+HO_(2))在四川盆地浓度水平较高,而NO_(3)自由基在华北平原的浓度水平较高.O_(3)光解过程是生成AOC最主要的来源,而OH自由基和二氧化氮生成硝酸的过程是AOC最主要的汇.AOC与二次污染物浓度关系密切,在O_(3)重污染情况下,AOC的浓度水平与年均值相比增幅明显(最高可达475%);同时,在高AOC水平下,二次有机气溶胶(secondary organic aerosol,SOA)的浓度也有显著升高.因为二次无机气溶胶(secondary inorganic aerosol,SIA)的生成过程包含气相和其他相位过程,并且受排放的季节性变化影响较大,因此总浓度与AOC关系不直接.此外,通过情景模拟分析了AOC和二次污染物浓度对不同污染物减排的响应.在夏季,减少氮氧化物(NO_(x))排放可以降低AOC,而在冬季AOC对排放调整的响应较为复杂,呈现较强的区域差异性特征.研究表明,在减少一次排放的同时要控制AOC的升高,才能高效地实现空气质量的提升和细颗粒物(PM_(2.5))与O_(3)协同控制的目标. 展开更多
关键词 大气氧化性 二次污染物 三维空气质量模式 臭氧 减排政策
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Is atmospheric oxidation capacity better in indicating tropospheric O_(3) formation? 被引量:2
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作者 Peng Wang shengqiang zhu +3 位作者 Mihalis Vrekoussis Guy PBrasseur Shuxiao Wang Hongliang Zhang 《Frontiers of Environmental Science & Engineering》 SCIE EI CSCD 2022年第5期127-133,共7页
Tropospheric ozone(O_(3))concentration is increasing in China along with dramatic changes in precursor emissions and meteorological conditions,adversely affecting human health and ecosystems.O_(3) is formed from the c... Tropospheric ozone(O_(3))concentration is increasing in China along with dramatic changes in precursor emissions and meteorological conditions,adversely affecting human health and ecosystems.O_(3) is formed from the complex nonlinear photochemical reactions from nitrogen oxides(NOx=NO+NO_(2))and volatile organic compounds(VOCs).Although the mechanism of O_(3) formation is rather clear,describing and analyzing its changes and formation potential at fine spatial and temporal resolution is still a challenge today.In this study,we briefly summarized and evaluated different approaches that indicate O_(3) formation regimes.We identify that atmospheric oxidation capacity(AOC)is a better indicator of photochemical reactions leading to the formation of O_(3) and other secondary pollutants.Results show that AOC has a prominent positive relationship to O_(3) in the major city clusters in China,with a goodness of fit(R^(2))up to 0.6.This outcome provides a novel perspective in characterizing O_(3) formation and has significant implications for formulating control strategies of secondary pollutants. 展开更多
关键词 O_(3) AOC O_(3) formation regime
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