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Sawtooth and dune auroras simultaneously driven by waves around the plasmapause 被引量:1
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作者 Fei He ZhongHua Yao +10 位作者 BinBin Ni Xing Cao ShengYi Ye RuiLong Guo JinXing Li ZhiPeng Ren XinAn Yue YongLiang zhang Yong Wei xiaoxin zhang ZuYin Pu 《Earth and Planetary Physics》 EI CSCD 2023年第2期237-246,共10页
The dune aurora,at a scale of~30 kilometers,was reported recently using ground camera.The small-scale dune aurora occurs on the duskside and exhibits a monochromatic oscillation in the auroral emission,implying fundam... The dune aurora,at a scale of~30 kilometers,was reported recently using ground camera.The small-scale dune aurora occurs on the duskside and exhibits a monochromatic oscillation in the auroral emission,implying fundamental energy conversions.However,whether the dune auroras correspond to atmospheric waves or are associated with magnetospheric dynamics should be determined.This paper reports a dune aurora that occurred during a storm;further,we demonstrate that it was the substructure of the sawtooth aurora that was generated by plasmapause surface waves.Conjugate observations in the magnetospheric source region suggest that the exohiss waves,which are periodically modulated by the plasmapause surface wave-excited ultralow frequency wave,might be responsible for the generation of the dune aurora.Most reported dune aurora events have occurred simultaneously with sawtooth auroras,suggesting that both are plasmapause-driven cross-scale auroral structures. 展开更多
关键词 sawtooth aurora dune aurora plasmapause surface wave exohiss
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Cross-satellite calibration of high-energy electron fluxes measured by FengYun-4A based on Arase observations
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作者 XiaoYu Wang Xing Cao +5 位作者 Xin Ma xiaoxin zhang AnQin Chen JunHu Dong BinBin Ni XianKang Dou 《Earth and Planetary Physics》 CAS CSCD 2023年第5期565-575,共11页
We use the High-energy Electron Experiments(HEP)instrument onboard Arase(ERG)to conduct an energy-dependent cross-satellite calibration of electron fluxes measured by the High Energy Particle Detector(HEPD)onboard Fen... We use the High-energy Electron Experiments(HEP)instrument onboard Arase(ERG)to conduct an energy-dependent cross-satellite calibration of electron fluxes measured by the High Energy Particle Detector(HEPD)onboard FengYun-4A(FY-4A)spanning from April 1,2017,to September 30,2019.By tracing the two-dimensional magnetic positions(L,magnetic local time[MLT])of FY-4A at each time,we compare the datasets of the conjugate electron fluxes over the range of 245–894 keV in 6 energy channels for the satellite pair within different sets of L×MLT.The variations in the electron fluxes observed by FY-4A generally agree with the Arase measurements,and the percentages of the ratios of electron flux conjunctions within a factor of 2 are larger than 50%.Compared with Arase,FY-4A systematically overestimates electron fluxes at all 6 energy channels,with the corresponding calibration factors ranging from 0.67 to 0.81.After the cross-satellite calibration,the electron flux conjunctions between FY-4A and Arase show better agreement,with much smaller normalized root mean square errors.Our results provide a valuable reference for the application of FY-4A high-energy electron datasets to in-depth investigations of the Earth’s radiation belt electron dynamics. 展开更多
关键词 cross-satellite calibration high-energy electron flux FengYun-4A Arase
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Green Production Technology of the Monomer of Nylon-6: Caprolactam 被引量:12
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作者 Baoning Zong Bin Sun +5 位作者 Shibiao Cheng Xuhong Mu Keyong Yang Junqi Zhao xiaoxin zhang Wei Wu 《Engineering》 SCIE EI 2017年第3期379-384,共6页
After two decades' endeavor, the Research Institute of Petroleum Processing (RIPP) has successfully de- veloped a green caprolactam (CPL) production technology. This technology is based on the integration of tita... After two decades' endeavor, the Research Institute of Petroleum Processing (RIPP) has successfully de- veloped a green caprolactam (CPL) production technology. This technology is based on the integration of titanium silicate (TS)-I zeolite with the slurry-bed reactor for the ammoximation of cyclohexanone, the integration of silicalite-1 zeolite with the moving-bed reactor for the gas-phase rearrangement of cyclohex- anone oxime, and the integration of an amorphous nickel (Ni) catalyst with the magnetically stabilized bed reactor for the purification of caprolactam. The world's first industrial plant based on this green CPL produc- tion technology has been built and possesses a capacity of 200 kt·a-1. Compared with existing technologies, the plant investment is pronouncedly reduced, and the nitrogen (N) atom utilization is drastically improved. The waste emission is reduced significantly; for example, no ammonium sulfate byproduct is produced. As a result, the price difference between CPL and benzene drops. In 2015, the capacity of the green CPL produc- tion technology reached 3 ×10-6 t·a-1, making China the world's largest CPL producer, with a global market share exceeding 50%. 展开更多
关键词 Green chemistry Green engineering CAPROLACTAM Production technology
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Advancement in separation materials for blood purification therapy 被引量:5
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作者 Jia Ju Feixue Liang +6 位作者 xiaoxin zhang Ran Sun Xiaoguang Pan Xiaoyun Guan Guanning Cui Xuan He Mengyan Li 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2019年第6期1383-1390,共8页
Blood purification refers to the extra corporeal therapies of removing potentially toxic substances, in which blood is circulated through an adsorption system loading separation materials. High-efficient inexpensive s... Blood purification refers to the extra corporeal therapies of removing potentially toxic substances, in which blood is circulated through an adsorption system loading separation materials. High-efficient inexpensive separation materials are critical to success. In this review, separation materials such as polymers and nanomaterials are summarized and compared. Combining the advantages of the adsorptive membranes and nanomaterials, organic–inorganic hybrid/blend membranes have been developed explosively. These hybrid/blend membranes have both the characteristics of high permeability, easy fabrication, good biocompatibility of adsorptive membranes, and characteristics of fast adsorption rate and high adsorption capacity of nanomaterials. The preparation and modification methodology of the separation materials is reviewed. For affinity separation materials, the relationship of ligand chemistry, ligand density and pores of the matrix is discussed. This paper also summarizes some interesting applications in separation materials for removal of bilirubin, endotoxin, toxic metal ions, cytokine, etc. 展开更多
关键词 Blood purification Organic INORGANIC hybrid/blend membrane Albumin-bound TOXINS Preparation and modification LIGAND density
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Characterization of Aquabacterium parvum sp. Strain B6 during Nitrate-Dependent Fe(Ⅱ) Oxidation Batch Cultivation with Various Impact Factors 被引量:2
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作者 xiaoxin zhang Ulrich Szewzyk Fang Ma 《Transactions of Tianjin University》 EI CAS 2017年第4期315-324,共10页
In order to assess the capacity of Aquabacterium parvum sp. strain B6 for nitrate-dependent Fe(II) oxidation, batch cultivation was conducted, and its ability to oxidize Fe(II) coupled to nitrate reduction in the pres... In order to assess the capacity of Aquabacterium parvum sp. strain B6 for nitrate-dependent Fe(II) oxidation, batch cultivation was conducted, and its ability to oxidize Fe(II) coupled to nitrate reduction in the presence of diverse organic substrates was studied. Meanwhile, the nitrate-removal rate of B6 with various impact factors was further optimized by the response surface methodology (RSM). The results show that strain B6 is capable of utilizing different organic compounds as substrates for nitrate reduction. Compared with yeast extract, B6 showed a greater potential of chemical oxygen demand (COD) degradation and cell proliferation with acetate and glucose mediums, respectively, while citrate was not beneficial for this process due to its low consumption rate. RSM analysis demonstrated that the maximum nitrate-reduction rate of 30.64% could be achieved with an initial pH of 7.4, incubation temperature of 25.0 °C, and carbon source concentration of 266.10 mg/L. © 2017, Tianjin University and Springer-Verlag Berlin Heidelberg. 展开更多
关键词 Carbon Cell proliferation Iron compounds NITRATES Optimization OXIDATION
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Channel Stability Analysis by One-Way Fluid Structure Interaction: A Case Study in China 被引量:2
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作者 Xiaobin Zhu Xiaoling Wang +2 位作者 Minghui Liu Zhen Wang xiaoxin zhang 《Transactions of Tianjin University》 EI CAS 2017年第5期451-460,共10页
Channel engineering stability with underground goafs is a complex three-dimensional problem, especially when considering channel leakage, and is influenced by a number of processes, such as seepage, fluid structure in... Channel engineering stability with underground goafs is a complex three-dimensional problem, especially when considering channel leakage, and is influenced by a number of processes, such as seepage, fluid structure interaction (FSI), modeling, and selection of geological mechanical parameters. In this study, stability finite element analysis by one-way FSI was performed by establishing an integrated 3D engineering geological model. The extended Fourier amplitude sensitivity test was used to quantitatively assess the first-order and total sensitivities of the engineering model to critical geological mechanical parameters. Results illustrate that the channel engineering deformation is under a reasonable range and the elastic modulus is the highest total sensitivity parameter for the channel tilt and curvature at 0.7395 and 0.7525, respectively. Moreover, the most observable coupling effects for the curvature and horizontal strain are cohesion (0.1933) and density (0.7410), respectively. © 2017, Tianjin University and Springer-Verlag GmbH Germany. 展开更多
关键词 Elastic moduli Fluid structure interaction GEOLOGY STABILITY
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An empirical model of the global distribution of plasmaspheric hiss based on Van Allen Probes EMFISIS measurements 被引量:4
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作者 JingZhi Wang Qi Zhu +7 位作者 XuDong Gu Song Fu JianGuang Guo xiaoxin zhang Juan Yi YingJie Guo BinBin Ni Zheng Xiang 《Earth and Planetary Physics》 CSCD 2020年第3期246-265,共20页
Using wave measurements from the EMFISIS instrument onboard Van Allen Probes,we investigate statistically the spatial distributions of the intensity of plasmaspheric hiss waves.To reproduce these empirical results,we ... Using wave measurements from the EMFISIS instrument onboard Van Allen Probes,we investigate statistically the spatial distributions of the intensity of plasmaspheric hiss waves.To reproduce these empirical results,we establish a fitting model that is a thirdorder polynomial function of L-shell,magnetic local time(MLT),magnetic latitude(MLAT),and AE*.Quantitative comparisons indicate that the model’s fitting functions can reflect favorably the major empirical features of the global distribution of hiss wave intensity,including substorm dependence and the MLT asymmetry.Our results therefore provide a useful analytic model that can be readily employed in future simulations of global radiation belt electron dynamics under the impact of plasmaspheric hiss waves in geospace. 展开更多
关键词 hiss Van Allen Probes global model
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Production of High Purity Metals: A Review on Zone Refining Process 被引量:8
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作者 xiaoxin zhang Semiramis Friedrich Bernd Friedrich 《Journal of Crystallization Process and Technology》 2018年第1期33-55,共23页
Purification is a primary application of zone melting, in which the improvement of efficiency, production yield and minimum achievable impurity level are always the research focus due to the increasing demand for high... Purification is a primary application of zone melting, in which the improvement of efficiency, production yield and minimum achievable impurity level are always the research focus due to the increasing demand for high purity metals. This paper has systematically outlined the whole development of related research on zone refining of metals including basic theories, variants of zone refining, parametric optimization, numerical models, and high purity analytical methods. The collection of this information could be of good value to improve the refining efficiency and the production of high purity metals by zone refining. 展开更多
关键词 ZONE REFINING ZONE MELTING High PURITY Distribution Coefficient Aluminium GERMANIUM ULTRA-PURE Metal
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Proton belt variations traced back to Fengyun-1C satellite observations 被引量:2
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作者 ChunQin Wang Zheng Chang +8 位作者 xiaoxin zhang GuoHong Shen ShenYi zhang YueQiang Sun JiaWei Li Tao Jing HuanXin zhang Ying Sun BinQuan zhang 《Earth and Planetary Physics》 CSCD 2020年第6期611-618,共8页
We used historical data to trace trapped protons observed by the Fengyun-1C(FY-1C)satellite at low Earth orbits(~800 km)and chose data at 5–10 MeV,10–40 MeV,40–100 MeV,and^100–300 MeV from 25 March to 18 April 200... We used historical data to trace trapped protons observed by the Fengyun-1C(FY-1C)satellite at low Earth orbits(~800 km)and chose data at 5–10 MeV,10–40 MeV,40–100 MeV,and^100–300 MeV from 25 March to 18 April 2000 to analyze the proton variations.Only one isolated strong storm was associated with a solar proton event during this period,and there was no influence from previous proton variations.Complex dynamic phenomena of proton trapping and loss were affected by this disturbance differently depending on the energy and L location.The flux of 5–10 MeV protons increased and created new trapping with a maximum at L^2.0,and the peak flux was significantly higher than that at the center of the South Atlantic Anomaly.However,at higher L,the flux showed obvious loss,with retreat of the outer boundary from L^2.7 to L^2.5.The increase in the 10–40 MeV proton flux was similar to that of the 5–10 MeV flux;however,the peak flux intensity was lower than that at the center of the South Atlantic Anomaly.The loss of the 10–40 MeV proton flux was closer to the Earth side,and the outer boundary was reduced from L^2.3 to L^2.25.For the higher energy protons of 40–100 MeV and 100–300 MeV,no new trapping was found.Loss of the 40–100 MeV protons was observed,and the outer boundary shifted from L^2.0 to L^1.9.Loss was not obvious for the 100–400 MeV protons,which were distributed within L<1.8.New proton trapping was more likely to be created at lower energy in the region of solar proton injection by the strong magnetic storm,whereas loss occurred in a wide energy range and reduced the outer boundary on the Earth side.Similar dynamic changes were observed by the NOAA-15 satellite in the same period,but the FY-1C satellite observed more complex changes in lower energy protons.These results revealed that the dynamic behavior of protons with different L-shells was due to differences in the pitch angle.Possible mechanisms related to new trapping and loss are also discussed.These mechanisms are very important for understanding the behavior of the proton belt in the coming solar cycle. 展开更多
关键词 high-energy proton TRAPPING loss DISTURBANCE inner radiation belt
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Correlations between plasmapause evolutions and auroral signatures during substorms observed by Chang'e-3 EUV Camera 被引量:2
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作者 xiaoxin zhang Fei He +2 位作者 Bo Chen Chao Shen HuaNing Wang 《Earth and Planetary Physics》 2017年第1期35-43,共9页
The plasmapause locations determined from the Chang'e-3(CE-3) Extreme Ultraviolet Camera(EUVC) images and the auroral boundaries determined from the Defense Meteorological Satellite Program(DMSP) Special Sensor Ul... The plasmapause locations determined from the Chang'e-3(CE-3) Extreme Ultraviolet Camera(EUVC) images and the auroral boundaries determined from the Defense Meteorological Satellite Program(DMSP) Special Sensor Ultraviolet Spectrographic Imager(SSUSI) images are used to investigate the plasmaspheric evolutions during substorms. The most important finding is a nightside pointing plasmaspheric plume observed at 23:05 UT on 21 April 2014 under quiet solar wind and geomagnetic conditions, which drifted from the dusk sector. High correlations between the plasmapause evolutions and the auroral signatures exist during substorms. After substorm onset, the plasmapause erosion and the equatorward expansion of the auroral oval occur almost simultaneously in both MLT and UT, and then both the erosion and the expansion propagate westward and eastward. It is suggested that the plasmaspheric erosion and its MLT propagations are induced by the enhanced earthward plasma convection during substorm period, and the substorm dipolarization causes pitch-angle scattering of plasma sheet electrons and the resulting precipitation excites aurora emissions at the same time. 展开更多
关键词 PLASMASPHERE Chang’e-3 EUVC minimum L Algorithm SUBSTORM
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Wide-field aurora imager onboard Fengyun satellite:Data products and validation 被引量:1
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作者 GuangXing Ding JiaWei Li +12 位作者 xiaoxin zhang Fei He LingPing He KeFei Song Liang Sun Shuang Dai ShiJie Liu Bo Chen Chao Yu XiuQing Hu SongYan Gu ZhongDong Yang Peng zhang 《Earth and Planetary Physics》 CSCD 2021年第1期73-78,共6页
New observations of auroras based on the wide-field aurora imager(WAI)onboard Fengyun-3D(FY-3D)satellite are exhibited in this paper.Validity of the WAI data is analyzed by comparing auroral boundaries derived from WA... New observations of auroras based on the wide-field aurora imager(WAI)onboard Fengyun-3D(FY-3D)satellite are exhibited in this paper.Validity of the WAI data is analyzed by comparing auroral boundaries derived from WAI observations with results obtained from data collected by the Special Sensor Ultraviolet Spectrographic Imager(SSUSI)aboard the Defense Meteorological Satellite Program(DMSP F18).Dynamic variations of the aurora with the solar wind,interplanetary magnetic field(IMF)parameters,and the SYM-H index are also investigated.The comparison of auroral boundaries indicates that the WAI data are morphologically valid and suitable to the study of auroral dynamics.Effective responses to solar wind parameters indicate that the WAI data can be useful to monitor and predict the Earth’s space weather.Since the configuration of aurora is a good indicator of the solar wind–magnetosphere–ionosphere(SW-M-I)coupling system,and can reflect the disturbance of the space environment,the WAI will provide important data to help us to study the physical processes in space. 展开更多
关键词 WAI FY-3D auroral dynamics SSUSI SW-M-I
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A New Post-hoc Flat Field Measurement Method for the Solar X-Ray and Extreme Ultraviolet Imager Onboard the FengYun-3E Satellite
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作者 Qiao Song Xianyong Bai +13 位作者 Bo Chen Xiuqing Hu Yajie Chen Zhenyong Hou Xiaofan zhang Lingping He Kefei Song Peng zhang Jing-Song Wang xiaoxin zhang Weiguo Zong Jinping Dun Hui Tian Yuanyong Deng 《Research in Astronomy and Astrophysics》 SCIE CAS CSCD 2022年第10期1-10,共10页
Extreme ultraviolet(EUV)observations are widely used in solar activity research and space weather forecasting since they can observe both the solar eruptions and the source regions of the solar wind.Flat field process... Extreme ultraviolet(EUV)observations are widely used in solar activity research and space weather forecasting since they can observe both the solar eruptions and the source regions of the solar wind.Flat field processing is indispensable to remove the instrumental non-uniformity of a solar EUV imager in producing high-quality scientific data from original observed data.FengYun-3E(FY-3E)is a meteorological satellite operated in a Sunsynchronous orbit,and the routine EUV imaging data from the Solar X-ray and Extreme Ultraviolet Imager(X-EUVI)onboard FY-3E has the characteristic of concentric rotation.Taking advantage of the concentric rotation,we propose a post-hoc flat field measurement method for its EUV 195A channel in this paper.This method removes the small-scale and time-varying component of coronal activities by taking the median value for each pixel along the time axis of a concentric rotation data cube,and then derives the large-scale and invariable component of the quiet coronal radiation,and finally generates a flat field image.The flat field can be generated with cadences from hundreds of minutes(one orbit)to several days.Higher flat field accuracy can be achieved by employing more data.Further analysis shows that our method is able to measure the instrumental spot-like nonuniformity possibly caused by contamination on the detector,which mostly disappears after the in-orbit selfcleaning process.It can also measure the quasi-periodic grid-like non-uniformity,possibly from the obscuration of the support mesh on the rear filter.After flat field correction,these instrumental non-uniformities from the original data are effectively removed.Moreover,the X-EUVI 195A data after dark and flat field corrections are consistent with the 193A imaging data from the Atmospheric Imaging Assembly onboard the Solar Dynamics Observatory,verifying the suitability of the method.The post-hoc method does not occupy observation time,which is advantageous for space weather operations.Our method is not only suitable for FY-3E/X-EUVI but also a candidate method for the flat field measurement of future solar EUV telescopes. 展开更多
关键词 SUN corona-techniques image processing-methods data analysis-methods OBSERVATIONAL
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The authors acknowledge the financial support from the National Natural Science Foundation of China(project No.31971247).
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作者 Yan Wei Guixin Zhu +8 位作者 Zifan Zhao Chengcheng Yin Qin Zhao Hudi Xu Jinyang Wang Jinglun zhang xiaoxin zhang Yufeng zhang Haibin Xia 《International Journal of Oral Science》 SCIE CAS CSCD 2021年第2期148-155,共8页
Mineralized tissue regeneration is an important and challenging part of the field of tissue engineering and regeneration.At present,autograft harvest procedures may cause secondary trauma to patients,while bone scaffo... Mineralized tissue regeneration is an important and challenging part of the field of tissue engineering and regeneration.At present,autograft harvest procedures may cause secondary trauma to patients,while bone scaffold materials lack osteogenic activity,resulting in a limited application.Loaded with osteogenic induction growth factor can improve the osteoinductive performance of bone graft,but the explosive release of growth factor may also cause side effects.In this study,we innovatively used platelet-rich fibrin(PRF)-modified bone scaffolds(Bio-Oss®)to replace autograft,and used cytokine(BMP-2)to enhance osteogenesis.Encouragingly,this mixture,which we named“Autograft Mimic(AGM)”,has multiple functions and advantages.(1)The fiber network provided by PRF binds the entire bone scaffold together,thereby shaping the bone grafts and maintaining the space of the defect area.(2)The sustained release of BMP-2 from bone graft promoted bone regeneration continuously.(3)AGM recruited bone marrow mesenchymal stem cells(BMSCs)and promote their proliferation,migration,and osteogenic differentiation.Thus,AGM developed in this study can improve osteogenesis,and provide new guidance for the development of clinical bone grafts. 展开更多
关键词 SUSTAINED GRAFT replace
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Advancing the Multilateral Regional Cooperation in Economy and Trade with the Scheme Reform of Zero Tariffs
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作者 Hongqiang Yang Shuli Zhou xiaoxin zhang 《Chinese Business Review》 2004年第11期67-73,共7页
China's tariff arrangement in the transition period after "entry to WTO" influences the process of the multilateral trade system in the world. Establishing the free trade area and customs union according to WTO/GAT... China's tariff arrangement in the transition period after "entry to WTO" influences the process of the multilateral trade system in the world. Establishing the free trade area and customs union according to WTO/GATS 1994 article 24, or according to authorizing the clause (Enabling Clause ) to sign the regional trade agreement between developing countries or signed the protocol of economic integration taking promoting and serving the liberalization of trade as purpose according to WTO/GATS article 5, include the regional trade agreement in the multilateral trade system frame to standardize, supervise and coordinate to China, reduce trade protectionism and improve the multilateral trade system's influence in the world greatly. Drawing lessons from CEPA and China the system of the manoeuvre ahead of time of overall "entry to WTO" of ASEAN Free Trade Area and arrange, accelerate multilateral regional cooperation in economy and trade, zero tariff scheme reform favors route choice. 展开更多
关键词 Scheme of zero tariff Regional trade agreement CEPA China-ASEAN Free Trade Area
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太阳立体探测任务设想 被引量:7
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作者 杨孟飞 汪景琇 +27 位作者 王赤 宗秋刚 张效信 代树武 邓元勇 冯学尚 王颖 朱成林 张也弛 张庆祥 沈锋钢 田百义 周文艳 李林凌 颜毅华 周桂萍 杨尚斌 熊明 张爱兵 何建森 田晖 李嘉巍 甘为群 夏利东 彭吉龙 黄长宁 姜杰 全林 《科学通报》 EI CAS CSCD 北大核心 2023年第8期859-871,共13页
太阳空间探测在太阳物理前沿科学问题研究和空间天气预报应用研究方面具有重要的意义.人类在60余年的太阳空间探测活动中,取得了一系列重要成果,但仍存在诸多根本性重大问题有待解决.太阳立体探测可以克服单视角观测的局限,获取全方位... 太阳空间探测在太阳物理前沿科学问题研究和空间天气预报应用研究方面具有重要的意义.人类在60余年的太阳空间探测活动中,取得了一系列重要成果,但仍存在诸多根本性重大问题有待解决.太阳立体探测可以克服单视角观测的局限,获取全方位、多要素的物理数据,促进解决太阳物理中的重大科学问题.本文介绍了太阳内部结构和磁场起源、太阳活动机理研究、太阳活动的全日球空间天气效应和空间天气预报模式研究4个科学目标,太阳立体探测任务空间布局、系统组成和探测器总体设计,以及太阳立体探测任务的有效载荷配置和主要技术指标. 展开更多
关键词 太阳物理 太阳立体探测 太阳活动 空间天气
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Advances in component and operation optimization of solid oxide electrolysis cell 被引量:2
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作者 xiaoxin zhang Bo Liu +5 位作者 Yanling Yang Jianhui Li Jian Li Yingru Zhao Lichao Jia Yifei Sun 《Chinese Chemical Letters》 SCIE CAS CSCD 2023年第5期155-164,共10页
Considering the earth powered by intermittent renewable energy in the coming future,solid oxide electrolysis cell(SOEC)will play an indispensable role in efficient energy conversion and storage on demand.The thermolyt... Considering the earth powered by intermittent renewable energy in the coming future,solid oxide electrolysis cell(SOEC)will play an indispensable role in efficient energy conversion and storage on demand.The thermolytic and kinetic merits grant SOEC a bright potential to be directly integrated with electrical grid and downstream chemical synthesis process.Meanwhile,the scientific community are still endeavoring to pursue the SOEC assembled with better materials and operated at a more energy-efficient way.In this review article,at cell level,we focus on the recent development of electrolyte,cathode,anode and buffer layer materials for both steam and CO_(2)electrolysis.On the other hand,we also discuss the next generation SOEC operated with the assistant of other fuels to further reduce the energy consumption and enhance the productivity of the electrolyzer.And stack level,the sealant,interconnect and stack operation strategies are collectively covered.Finally,the challenges and future research direction in SOECs are included. 展开更多
关键词 Solid oxide electrolysis cell Fuel assistant STACK Operation condition ANODE CATHODE
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Rational construction of multiple hollow silicalite-1 zeolite with enhanced quasi acidity for robust vapor-phase Beckmann rearrangement 被引量:2
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作者 Peng zhang Xianfeng Yi +9 位作者 Changjiu Xia Xinxin Peng Shuai zhang Chengxiang Li Anmin Zheng xiaoxin zhang Yibin Luo Lifeng Cui Fuhong Yu Xingtian Shu 《Nano Research》 SCIE EI CSCD 2023年第5期7958-7966,共9页
Developing efficient and stable zeolites for vapor-phase Beckmann rearrangement of cyclohexanone oxime is still a great challenge to realizeε-caprolactam(CPL)green production.In this work,the hierarchical porous sili... Developing efficient and stable zeolites for vapor-phase Beckmann rearrangement of cyclohexanone oxime is still a great challenge to realizeε-caprolactam(CPL)green production.In this work,the hierarchical porous silicalite-1 zeolites with multiple hollow structure(S-1-M)are explored by in-situ desilication−recrystallization post-treatment of spongy highway-like zeolites(S-1-S),which are synthesized through silanization synthesis of conventional bulky silicalite-1(S-1).Compared to S-1,S-1-M achieves superior catalytic performance,with improving the CPL selectivity from 85.7%to 94.1%and prolonging the catalyst lifetime from 74 to 126 h at a weight hourly space velocity(WHSV)of 6 h^(−1).Comprehensive physiochemical studies demonstrate that the highly dispersed intracrystalline cavities within S-1-M endow greater mass diffusion and better quasi acidity inducing by the enhanced H-bonds among abundant H-bonded silanols,which is cooperatively responsible for its superior catalytic performance. 展开更多
关键词 hollow silicalite-1 H-bonded silanols quasi acidity vapor-phase Beckmann rearrangement
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Interaction between neutrophil extracellular traps and cardiomyocytes contributes to atrial fibrillation progression 被引量:1
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作者 Li He Ruiqi Liu +7 位作者 Honghua Yue xiaoxin zhang Xiaohui Pan Yutao Sun Jun Shi Guonian Zhu Chaoyi Qin Yingqiang Guo 《Signal Transduction and Targeted Therapy》 SCIE CSCD 2023年第8期3849-3861,共13页
Atrial fibrillation(AF)is a frequent arrhythmia associated with cardiovascular morbidity and mortality.Neutrophil extracellular traps(NETs)are DNA fragments with cytoplasm proteins released from neutrophils,which are ... Atrial fibrillation(AF)is a frequent arrhythmia associated with cardiovascular morbidity and mortality.Neutrophil extracellular traps(NETs)are DNA fragments with cytoplasm proteins released from neutrophils,which are involved in various cardiovascular diseases.To elucidate the role of NETs in AF,we investigated the effect of NETs on AF progression and the secretion of NETs in AF.Results showed that:NETs induced the autophagic apoptosis of cardiomyocytes,and NETs also led to mitochondrial injury by promoting mitochondrial depolarization and ROS production.Ongoing tachy-pacing led to the structural loss of cardiomyocytes and provided potent stimuli to induce NETs secretion from neutrophils.In the meanwhile,increased Ang II in AF facilitated NETs formation through the upregulation of AKT phosphorylation,while it could not directly initiate NETosis as the autophagy was not induced.In vivo,DNase I was administrated to abrogate NETs formation,and AF-related fibrosis was ameliorated as expected.Correspondingly,the duration of the induced AF was reduced.Our study addresses the formation mechanism of NETs in AF and demonstrates the lethal effects of NETs on cardiomyocytes through the induction of mitochondrial injury and autophagic cell death,which comprehensively describes the positive feedback comprised of NETs and stimuli secreted by cardiomyocytes that sustains the progression of AF and AF related fibrosis. 展开更多
关键词 CARDIOMYOCYTES FIBRILLATION CARDIOVASCULAR
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In-situ construction of novel sulfur-vacancy-rich Bi/Bi_(2)S_(3)/SnS_(2)Z-scheme heterostructure photocatalysts for efficient Cr(Ⅵ)reduction and nitrogen fixation
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作者 Meng Lan Xiaoli Dong +3 位作者 Nan Zheng xiaoxin zhang Yu Wang Xinxin zhang 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2023年第36期237-247,共11页
Highly competent and economical photocatalysts are one of the most charming targets in environmental restoration and clean production.Herein,a novel sulfur-vacancy-rich Bi/Bi_(2)S_(3)/SnS_(2)Z-scheme heterostruc-ture ... Highly competent and economical photocatalysts are one of the most charming targets in environmental restoration and clean production.Herein,a novel sulfur-vacancy-rich Bi/Bi_(2)S_(3)/SnS_(2)Z-scheme heterostruc-ture was constructed in situ and applied for the photoreduction Cr(VI)and nitrogen fixation.The fab-ricated Bi/Bi_(2)S_(3)/SnS_(2)-2 exhibits the optimum photoreduction Cr(VI)performance with the efficiency of 94.5%within 15 min visible light irradiation.The remarkably enhanced catalytic efficiency derived from the synergistic effect of the construction of intimate contacted interface,abundant sulfur vacancy and surface plasmon resonance(SPR)effect of metal Bi.Meanwhile,the excellent photocatalytic nitrogen fix-ation property(96.4μmol g^(-1)h^(-1))was achieved by Bi/Bi_(2)S_(3)/SnS_(2)-2 under full solar illumination because sulfur vacancy could provide sufficient catalytic sites to accelerate the adsorption and nitrogen activation.The Z-scheme heterostructure was proposed to expound the photocatalytic mechanism.This work offers a new perspective on hierarchical heterostructure with plentiful vacancies for environmental remediation and energy development. 展开更多
关键词 Sulfur-vacancy-rich Bi/Bi_(2)s_(3)/SnS_(2) Z-scheme heterostructure SPR effect Cr(VI)reduction Nitrogen fixation
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壳层厚度对骨架Fe@HZSM-5核壳催化剂费托合成催化性能的影响 被引量:8
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作者 孙冬 孙博 +5 位作者 裴燕 闫世润 范康年 乔明华 张晓昕 宗保宁 《化学学报》 SCIE CAS CSCD 北大核心 2021年第6期771-777,共7页
在不同的水热合成时间下,以铁铝合金为铁源和铝源,四丙基氢氧化铵为分子筛的模板剂和抽提合金中的铝的碱,一步制得了以骨架铁为核、不同厚度的HZSM-5分子筛为壳的Raney Fe@HZSM-5催化剂.采用元素分析、氮物理吸附、X射线粉末衍射、氨脱... 在不同的水热合成时间下,以铁铝合金为铁源和铝源,四丙基氢氧化铵为分子筛的模板剂和抽提合金中的铝的碱,一步制得了以骨架铁为核、不同厚度的HZSM-5分子筛为壳的Raney Fe@HZSM-5催化剂.采用元素分析、氮物理吸附、X射线粉末衍射、氨脱附、扫描电子显微镜等手段,考察了水热时间对催化剂基本物化性质的影响.随着水热时间的延长,HZSM-5分子筛壳层不断增厚,结晶度不断增大,但分子筛组成基本不变,酸量与分子筛壳层厚度正相关.在费托合成反应中,Raney Fe@HZSM-5核壳催化剂上的CO转化率和汽油段产物选择性随分子筛壳层厚度呈火山型变化趋势,说明反应需要适宜的酸量,酸量过低或过高均不利于得到高的催化活性及汽油段产物选择性.在水热合成时间为4 d制得的Raney Fe@HZSM-5核壳催化剂上,当CO转化率为92%时,C5~C11汽油段产物选择性可达71%,异正比为1.9.当合成气中的n(H2)/n(CO)比从2降为1时,汽油段产物选择性和异正比进一步提高至73%和2.1,显示了将该催化剂用于煤基或生物质基合成气转化为高辛烷值汽油的良好潜力. 展开更多
关键词 骨架Fe HZSM-5 核壳结构 费托合成 汽油
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