Grey system analysis method was used to study the correlation between water pollution in D Lake area and death rate of malignancy with death rate of malignancy as effect sequence and a variety of water pollution index...Grey system analysis method was used to study the correlation between water pollution in D Lake area and death rate of malignancy with death rate of malignancy as effect sequence and a variety of water pollution index as factor sequence. On the basis of grey correlation analysis, grey system predication model was established for death rate of malignancy in population in D Lake area including GM (1, N) model for death rate of malignancy [ MR (t+1) =(9.9987E 1+5.0001E 2 +10.8994E 3+1.1114E 4+165.1029) ·e -0.0070t -9.9987E 1-5.0001E 2-10.8994E 3-1.1114E 4 ] and GM (1, 1) model for related factors [ E 1(t+1) =52.1214-46.9468e -0.0058t , E 2(t+1) =4.6114-4.5664e 0.0015t, E 3(t+1) =1.1389-1.1212e 0.0065t , E 4(t+1) = 554.5867-549.8006e 0.0016t ], and the trend of death rate of malignancy from 2000 to 2010 was predicted.展开更多
[ Objective ] This study aimed to investigate the impacts of different instruments and methods on detection of water samples and evaluate the detection results and pollution share rate. [ Method] Concentrations of six...[ Objective ] This study aimed to investigate the impacts of different instruments and methods on detection of water samples and evaluate the detection results and pollution share rate. [ Method] Concentrations of six heavy metals in three surface water samples and three underground water samples were detected by AAS and ICP-AES to analyze the differences in detection results and calculate the pollution share rate of heavy metals. [Result] As a result, the pollution share rate of six heavy metals varied significantly. Calculation results of comprehensive pollution share rate based on the lower pollution index of the same heavy metal in the same water sample detected by two methods were different from the results using either method. Due to different detection limits of instruments, detection results of heavy metals in the same water sample were different, which affected the accuracy of environmental quality assessment. [ Conclusion ] The detected pollution share rate varies with different detection limits. Therefore, instruments and methods with lower detection limit should be used. To be specific, AAS is suitable for detection of Pb and Cd, while ICP is suitable for detection of Cu, Zn, Fe and Mn.展开更多
In order to enhance the hydraulic loading rate （HLR） of a subsurface wastewater infiltration system （SWIS） used in treating domestic sewage, the intermittent operation mode was employed in the SWIS. The results sh...In order to enhance the hydraulic loading rate （HLR） of a subsurface wastewater infiltration system （SWIS） used in treating domestic sewage, the intermittent operation mode was employed in the SWIS. The results show that the intermittent operation mode contributes to the improvement of the HLR and the pollutant removal rate. When the wetting-drying ratio （RwD） was 1.0, the pollutant removal rate increased by （13.6 ± 0.3）% for NH3-N, （20.7 ± 1.1）% for TN, （18.6± 0.4）% for TP, （12.2 ± 0.5）% for BOD, （10.1 ± 0.3）% for COD, and （36.2 ± 1.2）% for SS, compared with pollutant removal rates under the continuous operation mode. The pollutant removal rate declined with the increase of the HLR. The effluent quality met The Reuse of Urban Recycling Water - Water Quality Standard for Scenic Environment Use （GB/T 18921-2002） even when the HLR was as high as 10 cm/d. Hydraulic conductivity, oxidation reduction potential （ORP）, the quantity of nitrifying bacteria, and the pollutant removal rate of NH3-N increased with the decrease of the RWD. For the pollutant removal rates of TP, BOD, and COD, there were no significant difference （p 〈 0.05） under different RwDS. The suggested RWD was 1.0. Relative contribution of the pretreatment and SWlS to the pollutant removal was examined, and more than 80% removal of NH3-N, TN, TP, COD, and BOD occurred in the SWIS.展开更多
In this study, a risk-based management model is developed and applied to an industrial zone. The models proposed by the United States Environmental Protection Agency and Han Bing have been improved by adding a residua...In this study, a risk-based management model is developed and applied to an industrial zone. The models proposed by the United States Environmental Protection Agency and Han Bing have been improved by adding a residual ratio of volatile organic compounds （VOC） after boiling and deleting the related parameters in half-life. Using this improved model, an integrated process was used to assess human health risk level in the study area. Compared with water quality analysis, the results highlight the importance of applying an integrated approach for decision making on risk levels and water protection. The results of this study demonstrated that： （1） Compared with these permissible level standards in China （GB 3838-2002） and National Primary Drinking Water Regulations of the United States, the residents＇ daily life had not been affected by the groundwater in this area （except for relative bad water quality of HB3-4 and HB3-6）; （2） The typical detected organic contaminants of all groundwater samples were chloroform, carbon tetrachloride, trichloroethylene and tetrachloroethene, and the pollution sources were mainly industrial sources by preliminary investigations; （3） As for groundwater, the non-carcinogenic risk values of all samples do not exceed the permissible level of 1.0 and the carcinogenic risk values are relatively lower than the permissible level of 1.00E-06 to 1.00E-04; （4） Drinking water pathway of trichloroethylene and tetrachloroethylene mainly contribute to increasing the health risk of residents＇ in study areas; （5） In terms of non-carcinogenic risk and carcinogenic risk, the health risk order for drinking water pathway and dermal contact pathway was： drinking water pathway 〉 dermal contact pathway.展开更多
On the basis of investigating rural population, land types, livestock and poultry breeding scale in drinking water conservation area of the Hongfeng Lake in Guiyang City, as well as the urban domestic pol utant discha...On the basis of investigating rural population, land types, livestock and poultry breeding scale in drinking water conservation area of the Hongfeng Lake in Guiyang City, as well as the urban domestic pol utant discharge coefficient, livestock and poultry excretion coefficient, nitrogen fertilizer and phosphate fertilizer loss rate in the first national pollution source survey, this paper tried to explore current situation of agricultural non-point source pollution, and provide scientific support for the pollution control. The results showed that in the drinking water conservation area of the Hongfeng lake in 2013, contribution rate of pollution sources to the water pollution in the Hongfeng Lake followed the sequence "livestock and poultry breeding > rural life > farmland fertilizer". Among all agricultural non-point source pollutants, livestock and poultry breeding pollutants were major pollution sources, with a contribution rate to CODCr, TP and NH3-N in water above 50%; rural domestic pollutants were also important pollution sources, its contribution rate to CODCr and NH3-N was 43.49% and 46.69%, respectively; contribution rate of farmland fertilizer pollutants to TN and TP was 33.76% and 27.71%, respectively, higher than that of rural domestic pollutants(25.87% and 6.75%). Therefore, the control of non-point source pollution within the drinking water conservation area should be enhanced, so as to control the pollution from the source.展开更多
Sulfur dioxide (SO2) is a major air pollutant, especially in developing countries. Many trees are seriously impaired by SO2, while other species can mitigate air pollution by absorbing this gas. Planting appropriate t...Sulfur dioxide (SO2) is a major air pollutant, especially in developing countries. Many trees are seriously impaired by SO2, while other species can mitigate air pollution by absorbing this gas. Planting appropriate tree species near industrial complexes is critical for aesthetic value and pollution mitigation. In this study, six landscape tree species typical of a subtropical area were investigated for their tolerance of SO2: Cinnamomum camphora (L.) J. Presl., Ilex rotunda Thunb., Lysidice rhodostegia Hance, Ceiba insignis (Kunth) P. E. Gibbs & Semir, Cassia surattensis Burm. f., and Michelia chapensis Dandy. We measured net photosynthesis rate, stomatal conductance, leaf sulfur content, relative water content, relative proline content, and other parameters under 1.31 mg·m-3 SO2 fumigation for eight days. The results revealed that the six species differed in their biochemical characteristics under SO2 stress. Based on these data, the most appropriate species for planting in SO2 polluted areas was I. rotunda, because it grew normally under SO2 stress and could absorb SO2.展开更多
In indoor environment, emission factor of the cooking fuel plays a vital role in determining correlation between exposure assessment and health effects. Both indoor and outdoor air pollution exposures are widely influ...In indoor environment, emission factor of the cooking fuel plays a vital role in determining correlation between exposure assessment and health effects. Both indoor and outdoor air pollution exposures are widely influenced by the ventilation status. An optimum control of the air change rate has also significant impact on the exposure pattern. A number of studies revealed that the indoor particulates and gaseous exposures, resulting from the combustion of various cooking fuels, are associated with significant adverse health effects on pregnant mothers and new born babies. The impacts of ventilation status on air pollution exposure in households’ kitchens or living rooms have not been explored enough. Except a few studies with concrete rooms, especially in industries, no other studies have been established on the correlation between the ventilation index and air pollution exposure. The intent of this review is to discuss reported findings focused on the ventilation and exposure to air pollution. This will obviously help better understanding to modulate exposure profile in household condition using simple tool of ventilation measurement.展开更多
Methacrylic acid was used together with a molecular imprinting technique to modify chitosan. In addition, the adsorption kinetics and adsorption isotherms were recorded and the results were analyzed to investigate rep...Methacrylic acid was used together with a molecular imprinting technique to modify chitosan. In addition, the adsorption kinetics and adsorption isotherms were recorded and the results were analyzed to investigate reparative adsorption for Cr（VI） from the polluted Xiangjiang River water. A comparative X-ray analysis shows that the degree of crystallization in the imprinted polymer was significantly weakened, the area of the non-crystalline region was larger. There were more adsorption sites in the imprinted polymer, and the adsorption capacity towards Cr（VI） was increased. The adsorption capacity of the imprinted polymer towards Cr（VI） increased with time and reaches saturation after 8 h. The optimal adsorption time was 4-8 h after the adsorption starting and the optimal pH value for the solution was in the range of 4.5-7.5. When the chitosan reaches saturation, the adsorption capacity achieves a state of equilibrium, and the maximum Cr（VI） extraction rate reaches 33.7%. Moreover, the adsorption capacity of the imprinted polymer towards Cr（VI） increases with increasing chitosan concentration. In this situation, the Cr（VI） extraction rate shows little variation, and the maximum removal rate can reach 98.3%. Furthermore, the Cr（VI） extraction rate increases with an increase in the degree of deacetylation in the chatoyant and chitosan, with the best adsorption effect corresponding to 90% deacetylation. Fitting the adsorption data to the quasi first- and second-order kinetic models yields correlation coefficients of 0.9013 and 0.9875, respectively. The corresponding rate constants for the two models are 0.0091 min-1 and 7.129 g/（mg.min）, respectively. Hence, the adsorption using Cr（VI）-imprinted chitosan is more consistent with the second-order kinetics. Comparing the data to Freundlich and Langrnuir adsorption isotherms shows that the latter has a better linear fit and a maximum adsorption capacity of 15.784 mg/g.展开更多
An innovative approach based on water environmental capacity for non-point source NPS pollution removal rate estimation was discussed by using both univariate and multivariate data analysis.Taking Shenzhen city as the...An innovative approach based on water environmental capacity for non-point source NPS pollution removal rate estimation was discussed by using both univariate and multivariate data analysis.Taking Shenzhen city as the study case a 67% to 74% NPS pollutant load removal rate can lead to meeting the chemical oxygen demand COD pollution control target for most watersheds.In contrast it is hardly to achieve the ammonia nitrogen NH4-N total phosphorus TP and biological oxygen demand BOD5 pollution control target by simply removing NPS pollutants. This highlights that the pollution control strategies should be taken according to different pollutant species and sources in different watersheds rather than one-size-fits-all .展开更多
基金ThisprojectwassupportedbyagrantfromtheNational"TheNinthFive YearPlan"ScienceandTechnologyKeyProjectofChina (No .96 9110 70 2 0 4 )
文摘Grey system analysis method was used to study the correlation between water pollution in D Lake area and death rate of malignancy with death rate of malignancy as effect sequence and a variety of water pollution index as factor sequence. On the basis of grey correlation analysis, grey system predication model was established for death rate of malignancy in population in D Lake area including GM (1, N) model for death rate of malignancy [ MR (t+1) =(9.9987E 1+5.0001E 2 +10.8994E 3+1.1114E 4+165.1029) ·e -0.0070t -9.9987E 1-5.0001E 2-10.8994E 3-1.1114E 4 ] and GM (1, 1) model for related factors [ E 1(t+1) =52.1214-46.9468e -0.0058t , E 2(t+1) =4.6114-4.5664e 0.0015t, E 3(t+1) =1.1389-1.1212e 0.0065t , E 4(t+1) = 554.5867-549.8006e 0.0016t ], and the trend of death rate of malignancy from 2000 to 2010 was predicted.
文摘[ Objective ] This study aimed to investigate the impacts of different instruments and methods on detection of water samples and evaluate the detection results and pollution share rate. [ Method] Concentrations of six heavy metals in three surface water samples and three underground water samples were detected by AAS and ICP-AES to analyze the differences in detection results and calculate the pollution share rate of heavy metals. [Result] As a result, the pollution share rate of six heavy metals varied significantly. Calculation results of comprehensive pollution share rate based on the lower pollution index of the same heavy metal in the same water sample detected by two methods were different from the results using either method. Due to different detection limits of instruments, detection results of heavy metals in the same water sample were different, which affected the accuracy of environmental quality assessment. [ Conclusion ] The detected pollution share rate varies with different detection limits. Therefore, instruments and methods with lower detection limit should be used. To be specific, AAS is suitable for detection of Pb and Cd, while ICP is suitable for detection of Cu, Zn, Fe and Mn.
基金supported by the National Natural Science Foundation of China(Grant No.51108275)the Program for Liaoning Excellent Talents in Universities(LNET)(Grant No.LJQ2012101)+2 种基金the Program for New Century Excellent Talents in Universities(Grant No.NCET-11-1012)the Science and Technology Program of Liaoning Province(Grants No.2011229002 and2013229012)the Basic Science Research Fund in Northeastern University(Grants No.N130501001 and N140105003)
文摘In order to enhance the hydraulic loading rate （HLR） of a subsurface wastewater infiltration system （SWIS） used in treating domestic sewage, the intermittent operation mode was employed in the SWIS. The results show that the intermittent operation mode contributes to the improvement of the HLR and the pollutant removal rate. When the wetting-drying ratio （RwD） was 1.0, the pollutant removal rate increased by （13.6 ± 0.3）% for NH3-N, （20.7 ± 1.1）% for TN, （18.6± 0.4）% for TP, （12.2 ± 0.5）% for BOD, （10.1 ± 0.3）% for COD, and （36.2 ± 1.2）% for SS, compared with pollutant removal rates under the continuous operation mode. The pollutant removal rate declined with the increase of the HLR. The effluent quality met The Reuse of Urban Recycling Water - Water Quality Standard for Scenic Environment Use （GB/T 18921-2002） even when the HLR was as high as 10 cm/d. Hydraulic conductivity, oxidation reduction potential （ORP）, the quantity of nitrifying bacteria, and the pollutant removal rate of NH3-N increased with the decrease of the RWD. For the pollutant removal rates of TP, BOD, and COD, there were no significant difference （p 〈 0.05） under different RwDS. The suggested RWD was 1.0. Relative contribution of the pretreatment and SWlS to the pollutant removal was examined, and more than 80% removal of NH3-N, TN, TP, COD, and BOD occurred in the SWIS.
基金supported by National Science and Technology Major Project(No2009 ZX 05039-003,2009 ZX 05039-004,2011ZX05060-005)the National Natural Science Foundation of China(No 2010CB428801-1)state-owned land resources investigation(1212010430351)
文摘In this study, a risk-based management model is developed and applied to an industrial zone. The models proposed by the United States Environmental Protection Agency and Han Bing have been improved by adding a residual ratio of volatile organic compounds （VOC） after boiling and deleting the related parameters in half-life. Using this improved model, an integrated process was used to assess human health risk level in the study area. Compared with water quality analysis, the results highlight the importance of applying an integrated approach for decision making on risk levels and water protection. The results of this study demonstrated that： （1） Compared with these permissible level standards in China （GB 3838-2002） and National Primary Drinking Water Regulations of the United States, the residents＇ daily life had not been affected by the groundwater in this area （except for relative bad water quality of HB3-4 and HB3-6）; （2） The typical detected organic contaminants of all groundwater samples were chloroform, carbon tetrachloride, trichloroethylene and tetrachloroethene, and the pollution sources were mainly industrial sources by preliminary investigations; （3） As for groundwater, the non-carcinogenic risk values of all samples do not exceed the permissible level of 1.0 and the carcinogenic risk values are relatively lower than the permissible level of 1.00E-06 to 1.00E-04; （4） Drinking water pathway of trichloroethylene and tetrachloroethylene mainly contribute to increasing the health risk of residents＇ in study areas; （5） In terms of non-carcinogenic risk and carcinogenic risk, the health risk order for drinking water pathway and dermal contact pathway was： drinking water pathway 〉 dermal contact pathway.
基金Sponsored by Significant Scientific and Technological Program of Guizhou Province([2015]2001)
文摘On the basis of investigating rural population, land types, livestock and poultry breeding scale in drinking water conservation area of the Hongfeng Lake in Guiyang City, as well as the urban domestic pol utant discharge coefficient, livestock and poultry excretion coefficient, nitrogen fertilizer and phosphate fertilizer loss rate in the first national pollution source survey, this paper tried to explore current situation of agricultural non-point source pollution, and provide scientific support for the pollution control. The results showed that in the drinking water conservation area of the Hongfeng lake in 2013, contribution rate of pollution sources to the water pollution in the Hongfeng Lake followed the sequence "livestock and poultry breeding > rural life > farmland fertilizer". Among all agricultural non-point source pollutants, livestock and poultry breeding pollutants were major pollution sources, with a contribution rate to CODCr, TP and NH3-N in water above 50%; rural domestic pollutants were also important pollution sources, its contribution rate to CODCr and NH3-N was 43.49% and 46.69%, respectively; contribution rate of farmland fertilizer pollutants to TN and TP was 33.76% and 27.71%, respectively, higher than that of rural domestic pollutants(25.87% and 6.75%). Therefore, the control of non-point source pollution within the drinking water conservation area should be enhanced, so as to control the pollution from the source.
文摘Sulfur dioxide (SO2) is a major air pollutant, especially in developing countries. Many trees are seriously impaired by SO2, while other species can mitigate air pollution by absorbing this gas. Planting appropriate tree species near industrial complexes is critical for aesthetic value and pollution mitigation. In this study, six landscape tree species typical of a subtropical area were investigated for their tolerance of SO2: Cinnamomum camphora (L.) J. Presl., Ilex rotunda Thunb., Lysidice rhodostegia Hance, Ceiba insignis (Kunth) P. E. Gibbs & Semir, Cassia surattensis Burm. f., and Michelia chapensis Dandy. We measured net photosynthesis rate, stomatal conductance, leaf sulfur content, relative water content, relative proline content, and other parameters under 1.31 mg·m-3 SO2 fumigation for eight days. The results revealed that the six species differed in their biochemical characteristics under SO2 stress. Based on these data, the most appropriate species for planting in SO2 polluted areas was I. rotunda, because it grew normally under SO2 stress and could absorb SO2.
文摘In indoor environment, emission factor of the cooking fuel plays a vital role in determining correlation between exposure assessment and health effects. Both indoor and outdoor air pollution exposures are widely influenced by the ventilation status. An optimum control of the air change rate has also significant impact on the exposure pattern. A number of studies revealed that the indoor particulates and gaseous exposures, resulting from the combustion of various cooking fuels, are associated with significant adverse health effects on pregnant mothers and new born babies. The impacts of ventilation status on air pollution exposure in households’ kitchens or living rooms have not been explored enough. Except a few studies with concrete rooms, especially in industries, no other studies have been established on the correlation between the ventilation index and air pollution exposure. The intent of this review is to discuss reported findings focused on the ventilation and exposure to air pollution. This will obviously help better understanding to modulate exposure profile in household condition using simple tool of ventilation measurement.
基金Project(41271332)supported by the National Natural Science Foundation of ChinaProject(2010YBB186)supported by the Social Science Foundation of Hunan Province,Chian
文摘Methacrylic acid was used together with a molecular imprinting technique to modify chitosan. In addition, the adsorption kinetics and adsorption isotherms were recorded and the results were analyzed to investigate reparative adsorption for Cr（VI） from the polluted Xiangjiang River water. A comparative X-ray analysis shows that the degree of crystallization in the imprinted polymer was significantly weakened, the area of the non-crystalline region was larger. There were more adsorption sites in the imprinted polymer, and the adsorption capacity towards Cr（VI） was increased. The adsorption capacity of the imprinted polymer towards Cr（VI） increased with time and reaches saturation after 8 h. The optimal adsorption time was 4-8 h after the adsorption starting and the optimal pH value for the solution was in the range of 4.5-7.5. When the chitosan reaches saturation, the adsorption capacity achieves a state of equilibrium, and the maximum Cr（VI） extraction rate reaches 33.7%. Moreover, the adsorption capacity of the imprinted polymer towards Cr（VI） increases with increasing chitosan concentration. In this situation, the Cr（VI） extraction rate shows little variation, and the maximum removal rate can reach 98.3%. Furthermore, the Cr（VI） extraction rate increases with an increase in the degree of deacetylation in the chatoyant and chitosan, with the best adsorption effect corresponding to 90% deacetylation. Fitting the adsorption data to the quasi first- and second-order kinetic models yields correlation coefficients of 0.9013 and 0.9875, respectively. The corresponding rate constants for the two models are 0.0091 min-1 and 7.129 g/（mg.min）, respectively. Hence, the adsorption using Cr（VI）-imprinted chitosan is more consistent with the second-order kinetics. Comparing the data to Freundlich and Langrnuir adsorption isotherms shows that the latter has a better linear fit and a maximum adsorption capacity of 15.784 mg/g.
基金The National Science and Technology Major Project of China(No.2012ZX07301-001)the Shenzhen Environmental Research Project,China Postdoctoral Science Foundation(No.2013M530642)
文摘An innovative approach based on water environmental capacity for non-point source NPS pollution removal rate estimation was discussed by using both univariate and multivariate data analysis.Taking Shenzhen city as the study case a 67% to 74% NPS pollutant load removal rate can lead to meeting the chemical oxygen demand COD pollution control target for most watersheds.In contrast it is hardly to achieve the ammonia nitrogen NH4-N total phosphorus TP and biological oxygen demand BOD5 pollution control target by simply removing NPS pollutants. This highlights that the pollution control strategies should be taken according to different pollutant species and sources in different watersheds rather than one-size-fits-all .
