We tested and modified the quasi-analytical algorithm （QAA） using 57 groups of field data collected in the spring of 2003 in the Yellow Sea and East China Sea. The QAA performs well in deriving total absorption coef...We tested and modified the quasi-analytical algorithm （QAA） using 57 groups of field data collected in the spring of 2003 in the Yellow Sea and East China Sea. The QAA performs well in deriving total absorption coefficients of typical coastal waters. The average percentage difference （APD） is in a range of 13.9%-38.5% for the total absorption coefficient （13.9% at 440 nm）, and differences in particle backscattering coefficient bbp（2） are less than 50% （in the case of the updated QAA）. To obtain improved results, we modified the QAA by adjusting the empirical relationships. The modified algorithm is then applied to the field data to test its performance. The APDs were 44.7%-46.6% for bbp（λ） and 9.9%-32.8% （9.9% at 555 nm） for the total absorption coefficient. This indicates that the modified QAA derives better results. We also used the modified model to derive phytoplankton pigment absorption （aph） and detritus and CDOM absorption （aug） coefficients. The APDs for aph and a dg at 440 nm are 37.1% and 19.8%. In this paper, we discuss error sources using the measured dataset. More independent field data can improve this algorithm and derive better results.展开更多
Electrochemical water splitting is regarded as the most promising approach to produce hydrogen.However,the sluggish electrochemical reactions occurring at the anode and cathode,namely,the oxygen evolution reaction(OER...Electrochemical water splitting is regarded as the most promising approach to produce hydrogen.However,the sluggish electrochemical reactions occurring at the anode and cathode,namely,the oxygen evolution reaction(OER)and the hydrogen evolution reaction(HER),respectively,consume a tremendous amount of energy,seriously hampering its wide application.Recently,single-atom catalysts(SACs)have been proposed to effectively enhance the kinetics of these two reactions.In this minireview,we focus on the recent progress in SACs for OER and HER applications.Three classes of SACs have been reviewed,i.e.,alloy-based SACs,carbon-based SACs and SACs supported on other compounds.Different factors affecting the activities of SACs are also highlighted,including the inherent element property,the coordination environment,the geometric structure and the loading amount of metal atoms.Finally,we summarize the current problems and directions for future development in SACs.展开更多
The Changjiang （Yangtze） Estuary is located in the East China Sea shelf with shallow water. Affected by the tide mixing and the runoff of the Changjiang River and the Qiantang River the turbidity is very high. Gener...The Changjiang （Yangtze） Estuary is located in the East China Sea shelf with shallow water. Affected by the tide mixing and the runoff of the Changjiang River and the Qiantang River the turbidity is very high. Generally, the water-leaving radiance is high in the turbid water because of the large particle scattering. Based on the in-situ data and ocean color remote sensing data of SeaWiFS, it was found that there was a black water region with the normalized water-leaving radiances less than 0.5 mW/（cm2-μm2-sr）. The optical principle of the occurrence of this black water was analyzed by the inherent optical properties and the ocean color components. The results show that black water is caused by the relative low values of the suspended particle matter concentration and the back scattering ratio. In the black water region, the percentage of the phytoplankton absorption was relatively high, and the large size of the phytoplankton caused the low value of the particle backscattering ratio.展开更多
As a new branch of efficient and low-cost mechanical energy conversion technology,triboelectric nanogenerator(TENG)is a potential solution to provide a long-term power supply for the Internet of Things(IoT)sensors and...As a new branch of efficient and low-cost mechanical energy conversion technology,triboelectric nanogenerator(TENG)is a potential solution to provide a long-term power supply for the Internet of Things(IoT)sensors and portable electronic devices.However,due to inherent working properties of TENG itself such as extremely high internal impedance,pulse,and alternating current(AC)output,TENG can not directly supply power to loads such as batteries efficiently.Based on these,we describe TENG’s performance from a new perspective of powering ability.It consists of two aspects:the ability to transport charge effectively and the ability to output high power quality current steadily.In order to push forward the developments and applications of TENG,it is necessary to improve its power supply capacity from different perspectives.Fortunately,in recent years,a variety of output signal’s management strategies aiming at effectively managing the generated electricity and significantly improving powering ability of TENG have obtained significantly progress.Herein,this paper discusses the working mechanisms and different load characteristics of TENG at first to clarify the electric performance of TENG.Then,on basis of theoretical analysis,the output signal’s management strategies are elaborated from four aspects:improving the cycle output electricity of TENG,increasing the surface charge density of TENG,improving the power quality of TENG-based energy harvesting system,promoting the application of TENG through integrated circuit(IC)technology and TENG network,and the relevant principles and applications are discussed systematically.Finally,the advantages and disadvantages of the above output signal’s management strategies are summarized and discussed,and the future development of the output signal’s management strategies for TENG is prospected.展开更多
基金Supported by the National Natural Science Foundation of China (Nos.40706060,60802089)the National High Technology Research and Development Program of China (863 Program) (No.2007AA092102)the Dragon Project (No.5292)
文摘We tested and modified the quasi-analytical algorithm （QAA） using 57 groups of field data collected in the spring of 2003 in the Yellow Sea and East China Sea. The QAA performs well in deriving total absorption coefficients of typical coastal waters. The average percentage difference （APD） is in a range of 13.9%-38.5% for the total absorption coefficient （13.9% at 440 nm）, and differences in particle backscattering coefficient bbp（2） are less than 50% （in the case of the updated QAA）. To obtain improved results, we modified the QAA by adjusting the empirical relationships. The modified algorithm is then applied to the field data to test its performance. The APDs were 44.7%-46.6% for bbp（λ） and 9.9%-32.8% （9.9% at 555 nm） for the total absorption coefficient. This indicates that the modified QAA derives better results. We also used the modified model to derive phytoplankton pigment absorption （aph） and detritus and CDOM absorption （aug） coefficients. The APDs for aph and a dg at 440 nm are 37.1% and 19.8%. In this paper, we discuss error sources using the measured dataset. More independent field data can improve this algorithm and derive better results.
文摘Electrochemical water splitting is regarded as the most promising approach to produce hydrogen.However,the sluggish electrochemical reactions occurring at the anode and cathode,namely,the oxygen evolution reaction(OER)and the hydrogen evolution reaction(HER),respectively,consume a tremendous amount of energy,seriously hampering its wide application.Recently,single-atom catalysts(SACs)have been proposed to effectively enhance the kinetics of these two reactions.In this minireview,we focus on the recent progress in SACs for OER and HER applications.Three classes of SACs have been reviewed,i.e.,alloy-based SACs,carbon-based SACs and SACs supported on other compounds.Different factors affecting the activities of SACs are also highlighted,including the inherent element property,the coordination environment,the geometric structure and the loading amount of metal atoms.Finally,we summarize the current problems and directions for future development in SACs.
基金The National Basic Research and Development Program ("973" Program) of China under contract No2009CB421202the National Natural Science Foundation of China under contract No 40706061the National High Technol-ogy Development Program ("863" Program) of China under contract Nos 2007AA12Z137 and 2008AA09Z104
文摘The Changjiang （Yangtze） Estuary is located in the East China Sea shelf with shallow water. Affected by the tide mixing and the runoff of the Changjiang River and the Qiantang River the turbidity is very high. Generally, the water-leaving radiance is high in the turbid water because of the large particle scattering. Based on the in-situ data and ocean color remote sensing data of SeaWiFS, it was found that there was a black water region with the normalized water-leaving radiances less than 0.5 mW/（cm2-μm2-sr）. The optical principle of the occurrence of this black water was analyzed by the inherent optical properties and the ocean color components. The results show that black water is caused by the relative low values of the suspended particle matter concentration and the back scattering ratio. In the black water region, the percentage of the phytoplankton absorption was relatively high, and the large size of the phytoplankton caused the low value of the particle backscattering ratio.
基金funded by the National Key R&D Project from Minister of Science and Technology(No.2021YFA1201602)the National Natural Science Foundation of China(Nos.52172203 and U21A20175).
文摘As a new branch of efficient and low-cost mechanical energy conversion technology,triboelectric nanogenerator(TENG)is a potential solution to provide a long-term power supply for the Internet of Things(IoT)sensors and portable electronic devices.However,due to inherent working properties of TENG itself such as extremely high internal impedance,pulse,and alternating current(AC)output,TENG can not directly supply power to loads such as batteries efficiently.Based on these,we describe TENG’s performance from a new perspective of powering ability.It consists of two aspects:the ability to transport charge effectively and the ability to output high power quality current steadily.In order to push forward the developments and applications of TENG,it is necessary to improve its power supply capacity from different perspectives.Fortunately,in recent years,a variety of output signal’s management strategies aiming at effectively managing the generated electricity and significantly improving powering ability of TENG have obtained significantly progress.Herein,this paper discusses the working mechanisms and different load characteristics of TENG at first to clarify the electric performance of TENG.Then,on basis of theoretical analysis,the output signal’s management strategies are elaborated from four aspects:improving the cycle output electricity of TENG,increasing the surface charge density of TENG,improving the power quality of TENG-based energy harvesting system,promoting the application of TENG through integrated circuit(IC)technology and TENG network,and the relevant principles and applications are discussed systematically.Finally,the advantages and disadvantages of the above output signal’s management strategies are summarized and discussed,and the future development of the output signal’s management strategies for TENG is prospected.
