Based on the Danckwerts surface renewal model, a simple explicit expression of the enhancement factor in ozone absorption with a first order ozone self-decomposition and parallel second order ozonation reactions has b...Based on the Danckwerts surface renewal model, a simple explicit expression of the enhancement factor in ozone absorption with a first order ozone self-decomposition and parallel second order ozonation reactions has been derived. The results are compared with our previous work based on the film theory. The 2,4-dichlorophenol destruction rate by ozonation is predicted using the enhancement factor model in this paper.展开更多
Beryllium-7 (7Be) and lead-210 (210Pb) radioac- tivity in aerosols collected, from October 2002 to January 2004 at Mt. Waliguan, by the Global Atmospheric Watch (GAW) Station, Qinghai Province is presented. The data w...Beryllium-7 (7Be) and lead-210 (210Pb) radioac- tivity in aerosols collected, from October 2002 to January 2004 at Mt. Waliguan, by the Global Atmospheric Watch (GAW) Station, Qinghai Province is presented. The data were analyzed together with simultaneously measured surface ozone concentrations. We found that short time variations of 7Be and 210Pb were linked to alternations of synoptic weather around the Mt. Waliguan region. 210Pb showed the lowest concentration in summer while Be showed no obvious sea- 7 sonal changes. Relatively high Be and 7 210 Pb radioactivity was observed at Mt. Waliguan when compared with the ob- servations at other mountain sites in other parts of the world. Surface ozone and 7Be showed a consistent seasonalvariation. Surface ozone correlated fairly well with 7Be/210Pb ratio. This suggested that vertical transport from higher altitudes of the atmosphere has predominant effects on the budget of surface ozone at Mt. Waliguan.展开更多
基金Supported by the China Scholarship Council and Guangdong Provincial Natural Science Foundation of China(No.950215).
文摘Based on the Danckwerts surface renewal model, a simple explicit expression of the enhancement factor in ozone absorption with a first order ozone self-decomposition and parallel second order ozonation reactions has been derived. The results are compared with our previous work based on the film theory. The 2,4-dichlorophenol destruction rate by ozonation is predicted using the enhancement factor model in this paper.
基金This work was financially supported by the National Natural Science Foundation of China(Grant No.20175032).
文摘Beryllium-7 (7Be) and lead-210 (210Pb) radioac- tivity in aerosols collected, from October 2002 to January 2004 at Mt. Waliguan, by the Global Atmospheric Watch (GAW) Station, Qinghai Province is presented. The data were analyzed together with simultaneously measured surface ozone concentrations. We found that short time variations of 7Be and 210Pb were linked to alternations of synoptic weather around the Mt. Waliguan region. 210Pb showed the lowest concentration in summer while Be showed no obvious sea- 7 sonal changes. Relatively high Be and 7 210 Pb radioactivity was observed at Mt. Waliguan when compared with the ob- servations at other mountain sites in other parts of the world. Surface ozone and 7Be showed a consistent seasonalvariation. Surface ozone correlated fairly well with 7Be/210Pb ratio. This suggested that vertical transport from higher altitudes of the atmosphere has predominant effects on the budget of surface ozone at Mt. Waliguan.
