Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency t...Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency transfer,measurement of fundamental physical constants,and high-precision ranging,achieving a series of milestone results in ground-based environments.With the continuous maturation and evolution of femtosecond lasers and related technologies,optical frequency combs are moving from ground-based applications to astronomical and space-based applications,playing an increasingly important role in atomic clocks,exoplanet observations,gravitational wave measurements,and other areas.This paper,focusing on astronomical and space-based applications,reviews research progress on astronomical frequency combs,optical clock time-frequency networks,gravitational waves,dark matter measurement,dual-comb large-scale absolute ranging,and high-resolution atmospheric spectroscopy.With enhanced performance and their gradual application in the field of space-based research,optical frequency combs will undoubtedly provide more powerful support for astronomical science and cosmic exploration in the future.展开更多
Femtosecond optical frequency combs correlate the microwave and optical frequencies accurately and coherently.Therefore,any optical frequency in visible to near-infrared region can be directly traced to a microwave fr...Femtosecond optical frequency combs correlate the microwave and optical frequencies accurately and coherently.Therefore,any optical frequency in visible to near-infrared region can be directly traced to a microwave frequency.As a result,the length unit“meter”is directly related to the time unit“second”.This paper validates the capability of the national wavelength standards based on a home-made Er-doped fiber femtosecond optical frequency comb to measure the laser frequencies ranging from visible to near-infrared region.Optical frequency conversion in the femtosecond optical frequency comb is achieved by combining spectral broadening in a highly nonlinear fiber with a single-point frequencydoubling scheme.The signal-to-noise ratio of the beat notes between the femtosecond optical frequency comb and the lasers at 633,698,729,780,1064,and 1542 nm is better than 30 d B.The frequency instability of the above lasers is evaluated by using a hydrogen clock signal with a instability of better than 1×10^(-13)at 1-s averaging time.The measurement is further validated by measuring the absolute optical frequency of an iodine-stabilized 532-nm laser and an acetylenestabilized 1542-nm laser.The results are within the uncertainty range of the international recommended values.Our results demonstrate the accurate optical frequency measurement of lasers at different frequencies using the femtosecond optical frequency comb,which is not only important for the precise and accurate traceability and calibration of the laser frequencies,but also provides technical support for establishing the national wavelength standards based on the femtosecond optical frequency comb.展开更多
We numerically simulate the generation of an optical frequency comb(OFC) in a microring based on the traditional Si_3N_4 strip waveguide and a temperature compensated slot waveguide.The results show that OFCs are susc...We numerically simulate the generation of an optical frequency comb(OFC) in a microring based on the traditional Si_3N_4 strip waveguide and a temperature compensated slot waveguide.The results show that OFCs are susceptible to temperature with strip waveguide while they can keep stable when temperature changes 10 Kin either low-Q(10~5) or highQ(10~6) microcavity with the well-designed slot waveguide,which has great superiority in practical applications where the temperature drift of the cavity due to the intense pump or surrounding change is unavoidable.展开更多
Direct-comb spectroscopy techniques uses optical frequency combs(OFCs)as spectroscopic light source.They deliver high sensitivity,high frequency resolution and precision in a broad spectral range.Due to these features...Direct-comb spectroscopy techniques uses optical frequency combs(OFCs)as spectroscopic light source.They deliver high sensitivity,high frequency resolution and precision in a broad spectral range.Due to these features,the field has burgeoned in recent years.In this work we constructed an OFC-based cavity-enhanced Fourier-transform spectrometer in the nearinfrared region and used it for a line-shape study of rovibrational transitions of CO perturbed by Ar.The highly sensitive measurements spanned the wavenumber range from 6270 cm^-1 to 6410 cm^-1,which covered both P and R branch of the second overtone band of CO.The spectrometer delivers high-resolution surpassing the Fourier-transform resolution limit determined by interferogram length,successfully removing ringing and broadening effects caused by instrumental line shape function.The instrumental-line-shape-free method and high signal-to-noise ratio in the measurement allowed us to observe collisional effects beyond those described by the Voigt profile.We retrieved collisional line-shape parameters by fitting the speed-dependent Voigt profile and found good agreement with the values given by precise cavity ring-down spectroscopy measurements that used a continuous-wave laser referenced to a stabilized OFC.The results demonstrate that OFC-based cavity-enhanced Fouriertransform spectroscopy is a strong tool for accurate line-shape studies that will be crucial for future spectral databases.展开更多
We demonstrate an optical frequency comb(OFC)based on a turnkey mode-locked laser with a figure-9-shape structure and polarization-maintaining fibers,for the comparison of frequency among optical clocks with wavelengt...We demonstrate an optical frequency comb(OFC)based on a turnkey mode-locked laser with a figure-9-shape structure and polarization-maintaining fibers,for the comparison of frequency among optical clocks with wavelengths of 698 nm,729 nm,1068 nm,and 1156 nm.We adopt a multi-branch approach in order to produce high power OFC signals at these specific wavelengths,enabling the signal-to-noise ratio of the beatnotes between the OFC and the clock lasers to exceed30 d B at a resolution bandwidth of 300 k Hz.This approach makes the supercontinuum spectra much easier to be generated than a single branch OFC.However,more out-of-loop fibers degrade the long-term frequency instability due to thermal drift.To minimize the thermal drift effect,we set the fiber lengths of different branches to be similar,and we stabilize the temperature as well.The out-of-loop frequency instability of the OFC due to the incoherence of the multi-branch is about5.5×10^(19) for 4000 s,while the in-loop frequency instability of fceo and that of fbeat are 7.5×10^(18) for 1 s and 8.5×10^(18) for 1 s,respectively.The turnkey OFC meets the requirement for the comparison of frequency between the best optical clocks.展开更多
We numerically investigate the mid-infrared(MIR)supercontinuum(SC)and SC-based optical frequency comb(OFC)generations when the three optical modes(LP_(01),LP_(02),and LP_(12))are considered in a multimode tellurite ph...We numerically investigate the mid-infrared(MIR)supercontinuum(SC)and SC-based optical frequency comb(OFC)generations when the three optical modes(LP_(01),LP_(02),and LP_(12))are considered in a multimode tellurite photonic crystal fiber(MM-TPCF).The geometrical parameters of the MM-TPCF are optimized to support the multimode propagation and obtain the desired dispersion characteristics of the considered three optical modes.When the pump pulse with center wavelengthλ=2.5μm,width T=80 fs,and peak power P=18 kW is coupled into the anomalous dispersion region of the LP_(01),LP_(02),and LP_(12)modes of the MM-TPCF,the-40-dB bandwidth of the generated MIR SCs can be up to 2.56,1.39,and 1.12 octaves,respectively,along with good coherence.Moreover,the nonlinear dynamics of the generated SCs are analyzed.Finally,the MIR SCs-based OFCs are demonstrated when a train of 50 pulses at 1-GHz repetition rate is used as the pump source and launched into the MM-TPCF.展开更多
The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective f...The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective four wave-mixing in the active semiconductor gain medium. The low-noise Gaussian-like pulse can be obtained by locking the relaxation oscillation and compensating the gain asymmetry. The simulations suggest that pulse trains of width below 30 ps and repetition rate in GHz frequency can be generated simply by the optical injection locking of semiconductor lasers. Since the optical injection locking can broaden the spectrum and amplify the optical power simultaneously, it can be a good initial stage for generating optical frequency combs from dual-frequency lasers by multi-stage of spectral broadening in nonlinear waveguides.展开更多
We demonstrate an optical frequency comb based on an erbium-doped-fiber femtosecond laser with the nonlinear polarization evolution scheme.The repetition rate of the laser is about 209 MHz.By controlling an intra-cavi...We demonstrate an optical frequency comb based on an erbium-doped-fiber femtosecond laser with the nonlinear polarization evolution scheme.The repetition rate of the laser is about 209 MHz.By controlling an intra-cavity electrooptic modulator and a piezo-transducer,the repetition rate can be stabilized with a high-bandwidth servo in a frequency range of 3 k Hz,enabling long-term repetition rate phase-locking.The in-loop frequency stability of repetition rate is about1.6×10-13 in an integration time of 1 s,limited by the measurement system;and it is inversely proportional to integration time in the short term.Furthermore,using a common path f –2 f interferometer,the carrier envelope offset frequency of the comb is obtained with a signal-to-noise ratio of 40 d B in a 3-MHz resolution bandwidth.Stabilized carrier envelope offset frequency exhibits a deviation of 0.6 m Hz in an integration time of 1 s.展开更多
Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study...Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study of signals during the generation of the Kerr optical frequency combs(OFCs). We find that the signals in different states, including the Turing pattern, the chaos, the single soliton state, and the multi-solitons state, can be distinguished according to different distributions of the eigenvalue spectrum. Specially, the eigenvalue spectrum of the single soliton pulse is composed of a pair of conjugate symmetric discrete eigenvalues and the quasi-continuous eigenvalue spectrum with eye-like structure.Moreover, we have successfully demonstrated that the number of discrete eigenvalue pairs in the eigenvalue spectrum corresponds to the number of solitons formed in a round-trip time inside the Kerr microresonator. This work shows that some characteristics of the time-domain signal can be well reflected in the nonlinear domain.展开更多
This paper reports that two identical external-cavity-diode-laser (ECDL) based spectrometers are constructed at 634 nm referencing on the hyperfine B-X transition R(80)8-4 of 127I2. The lasers are stabilized on the Do...This paper reports that two identical external-cavity-diode-laser (ECDL) based spectrometers are constructed at 634 nm referencing on the hyperfine B-X transition R(80)8-4 of 127I2. The lasers are stabilized on the Doppler-free absorption signals using the third-harmonic detection technique. The instability of the stabilized laser is measured to be 2.8 × 10-12 (after 1000 s) by counting the beat note between the two lasers. The absolute optical frequency of the transition is, for the first time, determined to be 472851936189.5 kHz by using an optical frequency comb referenced on the microwave caesium atomic clock. The uncertainty of the measurement is less than 4.9 kHz.展开更多
The generation of high-repetition rate(frep≥10 GHz)ultra-broadband optical frequency combs(OFCs)at 1550 nm and 1310 nm is investigated by seeding two types of highly nonlinear fibers(HNLFs)with 10 GHz picosecond puls...The generation of high-repetition rate(frep≥10 GHz)ultra-broadband optical frequency combs(OFCs)at 1550 nm and 1310 nm is investigated by seeding two types of highly nonlinear fibers(HNLFs)with 10 GHz picosecond pulses at the pump wavelength of 1550 nm.When pumped near the zero dispersion wavelength(ZDW)in the normal dispersion region of a HNLF,10 GHz flat-topped OFC with 43 nm bandwidth within 5 dB power variation is generated by self-phase modulation(SPM)-based OFC spectral broadening at 26.5 dBm pump power,and 291 fs pulse trains with 10 GHz repetition rate are obtained at 18 dBm pump power without complicated pulse shaping methods.Furthermore,when pumped in the abnormal dispersion region of a HNLF,OFCs with dispersive waves around 1310 nm are studied using a common HNLF and fluorotellurite fibers,which maintain the good coherence of the pump light at 1550 nm.At the same time,sufficient tunability of the generated dispersive waves is achieved when tuning the pump power or ZDW.展开更多
The high precision two-photon excitation measurements for 5S1/2(F87g = 2) to 5D5/2(Fe = 4 to 1) ofRb are performed by using an optical frequency comb.The two counter-propagating femtosecond pulses(5S1/2→5P3/2at 780 n...The high precision two-photon excitation measurements for 5S1/2(F87g = 2) to 5D5/2(Fe = 4 to 1) ofRb are performed by using an optical frequency comb.The two counter-propagating femtosecond pulses(5S1/2→5P3/2at 780 nm,and 5P3/2→5D5/2at 776 nm) act on87 Rb vapor,and the Doppler broadened background signal is effectively eliminated.The temperature and power dependences of the two-photon spectrum are studied in this paper.展开更多
The results of an optoelectronic system—frequency-shifted feedback(FSF)laser experimental examination are presented.The considered FSF laser is seeded only with optical amplifer spontaneous emission(ASE)and operates ...The results of an optoelectronic system—frequency-shifted feedback(FSF)laser experimental examination are presented.The considered FSF laser is seeded only with optical amplifer spontaneous emission(ASE)and operates in the mode-locked regime,whereby the output radiation is sequence of short pulses with a repetition rate determined by the delay time in its optical feedback circuit.In the frequency domain,the spectrum of such a pulse sequence is an optical frequency comb(OFC).These OFCs we call initial.We consider the possibility of tunable acousto-optic(AO)dual and quad-comb frequency spacing downconversion in the FSF laser seeded with ASE and operating in the mode-locked regime.The examined system applies a single frequency shifting loop with single AO tunable flter as the frequency shifter that is fed with several radio frequency signals simultaneously.The initial OFCs with frequency spacing of about 6.5 MHz may be obtained in the wide spectral range and their width,envelope shape and position in the optical spectrum may be tuned.The dual-combs are obtained with a pair of initial OFCs aroused by two various ultrasound waves in the acousto-optic tunable flter(AOTF).The dual-combs frequency spacing is determined by the frequency diference of the signals applied to the AOTF piezoelectric transducer and can be tuned simply.The quad-combs are obtained with three initial OFCs,forming a pair of dual-combs,appearing when three ultrasound frequencies feed the AOTF transducer.The quad-combs frequency spacing is defned by the diference between the frequency spacing of dual-combs.Quad-combs with more than 5000 spectral lines and tunable frequency spacing are observed.The successive frequency downconversion gives the possibility to reduce the OFC frequency spacing form several MHz for initial OFC to tens of kHz for quad-combs.展开更多
Future inter-satellite clock comparison on high orbit will require optical time and frequency transmission technology between moving objects.Here,we demonstrate robust optical frequency transmission under the conditio...Future inter-satellite clock comparison on high orbit will require optical time and frequency transmission technology between moving objects.Here,we demonstrate robust optical frequency transmission under the condition of variable link distance.This variable link is accomplished by the relative motion of a single telescope fixed on the experimental platform to a corner-cube reflector(CCR)installed on a sliding guide.Two acousto–optic modulators with different frequencies are used to separate forward signal from backward signal.With active phase noise suppression,when the CCR moves back and forth at a constant velocity of 20 cm/s and an acceleration of 20 cm/s^(2),we achieve the best frequency stability of 1.9×10^(-16) at 1 s and 7.9×10^(-19) at 1000 s indoors.This work paves the way for future studying optical frequency transfer between ultra-high-orbit satellites.展开更多
Raman lasers are essential in atomic physics,and the development of portable devices has posed requirements for time-division multiplexing of Raman lasers.We demonstrate an innovative gigahertz frequency hopping appro...Raman lasers are essential in atomic physics,and the development of portable devices has posed requirements for time-division multiplexing of Raman lasers.We demonstrate an innovative gigahertz frequency hopping approach of a slave Raman laser within an optical phase-locked loop(OPLL),which finds practical application in an atomic gravimeter,where the OPLL frequently switches between near-resonance lasers and significantly detuned Raman lasers.The method merges the advantages of rapid and extensive frequency hopping with the OPLL’s inherent low phase noise,and exhibits a versatile range of applications in compact laser systems,promising advancements in portable instruments.展开更多
We demonstrate coherent optical frequency dissemination over a distance of 972 km by cascading two spans where the phase noise is passively compensated for.Instead of employing a phase discriminator and a phase lockin...We demonstrate coherent optical frequency dissemination over a distance of 972 km by cascading two spans where the phase noise is passively compensated for.Instead of employing a phase discriminator and a phase locking loop in the conventional active phase control scheme,the passive phase noise cancellation is realized by feeding double-trip beat-note frequency to the driver of the acoustic optical modulator at the local site.This passive scheme exhibits fine robustness and reliability,making it suitable for long-distance and noisy fiber links.An optical regeneration station is used in the link for signal amplification and cascaded transmission.The phase noise cancellation and transfer instability of the 972-km link is investigated,and transfer instability of 1.1×10^(-19)at 10^(4)s is achieved.This work provides a promising method for realizing optical frequency distribution over thousands of kilometers by using fiber links.展开更多
Optical spectral measurements are crucial for optical sensors and many other applications,but the prevailing methods,such as optical spectrum analysis and tunable laser spectroscopy,often have to make compromises amon...Optical spectral measurements are crucial for optical sensors and many other applications,but the prevailing methods,such as optical spectrum analysis and tunable laser spectroscopy,often have to make compromises among resolution,speed,and accuracy.Optical frequency combs are widely used for metrology of discrete atomic and molecular spectral lines.However,they are usually generated by optical methods and have large comb spacing,which limits the resolution for direct sampling of continuous spectra.To overcome these problems,this paper presents an original method to digitally generate an ultrafine optical frequency comb(UFOFC)as the frequency ruler for spectral measurements.Each comb line provides one sampling point,and the full spectrum can be captured at the same time using coherent detection.For an experimental demonstration,we adopted the inverse fast Fourier transform to generate a UFOFC with a comb spacing of 1.46 MHz over a 10-GHz range and demonstrated its functions using a Mach–Zehnder refractive index sensor.The UFOFC obtains a spectral resolution of 0.01 pm and response time of 0.7 μs;both represent 100-fold improvements over the state of the art and could be further enhanced by several orders of magnitude.The UFOFC presented here could facilitate new label-free sensor applications that require both high resolution and fast speed,such as measuring binding kinetics and single-molecule dynamics.展开更多
Dual-pumped microring-resonator-based optical frequency combs(OFCs) and their temporal characteristics are numerically investigated and experimentally explored. The calculation results obtained by solving the driven a...Dual-pumped microring-resonator-based optical frequency combs(OFCs) and their temporal characteristics are numerically investigated and experimentally explored. The calculation results obtained by solving the driven and damped nonlinear Schr?dinger equation indicate that an ultralow coupled pump power is required to excite the primary comb modes through a non-degenerate four-wave-mixing(FWM) process and, when the pump power is boosted, both the comb mode intensities and spectral bandwidths increase. At low pump powers, the field intensity profile exhibits a cosine variation manner with frequency equal to the separation of the two pumps, while a roll Turing pattern is formed resulting from the increased comb mode intensities and spectral bandwidths at high pump powers. Meanwhile, we found that the power difference between the two pump fields can be transferred to the newly generated comb modes, which are located on both sides of the pump modes, through a cascaded FWM process. Experimentally, the dual-pumped OFCs were realized by coupling two self-oscillating pump fields into a microring resonator. The numerically calculated comb spectrum is verified by generating an OFC with 2.0 THz mode spacing over 160 nm bandwidth. In addition, the formation of a roll Turing pattern at high pump powers is inferred from the measured autocorrelation trace of a 10 free spectral range(FSR) OFC. The experimental observations accord well with the numerical predictions. Due to their large and tunable mode spacing, robustness,and flexibility, the proposed dual-pumped OFCs could find potential applications in a wide range of fields,including arbitrary optical waveform generation, high-capacity optical communications, and signal-processing systems.展开更多
We demonstrated stable midinfrared(MIR) optical frequency comb at the 3.0 μm region with difference frequency generation pumped by a high power, Er-doped, ultrashort pulse fiber laser system. A soliton mode-locked161...We demonstrated stable midinfrared(MIR) optical frequency comb at the 3.0 μm region with difference frequency generation pumped by a high power, Er-doped, ultrashort pulse fiber laser system. A soliton mode-locked161 MHz high repetition rate fiber laser using a single wall carbon nanotube was fabricated. The output pulse was amplified in an Er-doped single mode fiber amplifier, and a 1.1–2.2 μm wideband supercontinuum(SC) with an average power of 205 m W was generated in highly nonlinear fiber. The spectrogram of the generated SC was examined both experimentally and numerically. The generated SC was focused into a nonlinear crystal, and stable generation of MIR comb around the 3 μm wavelength region was realized.展开更多
We report a long-term frequency-stabilized optical frequency comb at 530–1100 nm based on a turnkey Ti:sapphire modelocked laser.With the help of a digital controller,turnkey operation is realized for the Ti:sapphire...We report a long-term frequency-stabilized optical frequency comb at 530–1100 nm based on a turnkey Ti:sapphire modelocked laser.With the help of a digital controller,turnkey operation is realized for the Ti:sapphire mode-locked laser.Under optimized design of the laser cavity,the laser can be mode-locked over a month,limited by the observation time.The combination of a fast piezo and a slow one inside the Ti:sapphire mode-locked laser allows us to adjust the cavity length with moderate bandwidth and tuning range,enabling robust locking of the repetition rate(f_(r)) to a hydrogen maser.By combining a fast analog feedback to pump current and a slow digital feedback to an intracavity wedge and the pump power of the Ti:sapphire mode-locked laser,the carrier envelope offset frequency(f_(ceo)) of the comb is stabilized.We extend the continuous frequency-stabilized time of the Ti:sapphire optical frequency comb to five days.The residual jitters of f;and f;are 0.08 m Hz and 2.5 m Hz at 1 s averaging time,respectively,satisfying many applications demanding accuracy and short operation time for optical frequency combs.展开更多
基金support of the National Natural Sci-ence Foundation of China(NSFC)(62305373)the Strategic Priority Research Program of the Chinese Academy of Sciences(XDA1502040404,XDB2101040004).
文摘Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency transfer,measurement of fundamental physical constants,and high-precision ranging,achieving a series of milestone results in ground-based environments.With the continuous maturation and evolution of femtosecond lasers and related technologies,optical frequency combs are moving from ground-based applications to astronomical and space-based applications,playing an increasingly important role in atomic clocks,exoplanet observations,gravitational wave measurements,and other areas.This paper,focusing on astronomical and space-based applications,reviews research progress on astronomical frequency combs,optical clock time-frequency networks,gravitational waves,dark matter measurement,dual-comb large-scale absolute ranging,and high-resolution atmospheric spectroscopy.With enhanced performance and their gradual application in the field of space-based research,optical frequency combs will undoubtedly provide more powerful support for astronomical science and cosmic exploration in the future.
基金the National Key Research and Development Program of China(Grant No.2016YFF0200204)。
文摘Femtosecond optical frequency combs correlate the microwave and optical frequencies accurately and coherently.Therefore,any optical frequency in visible to near-infrared region can be directly traced to a microwave frequency.As a result,the length unit“meter”is directly related to the time unit“second”.This paper validates the capability of the national wavelength standards based on a home-made Er-doped fiber femtosecond optical frequency comb to measure the laser frequencies ranging from visible to near-infrared region.Optical frequency conversion in the femtosecond optical frequency comb is achieved by combining spectral broadening in a highly nonlinear fiber with a single-point frequencydoubling scheme.The signal-to-noise ratio of the beat notes between the femtosecond optical frequency comb and the lasers at 633,698,729,780,1064,and 1542 nm is better than 30 d B.The frequency instability of the above lasers is evaluated by using a hydrogen clock signal with a instability of better than 1×10^(-13)at 1-s averaging time.The measurement is further validated by measuring the absolute optical frequency of an iodine-stabilized 532-nm laser and an acetylenestabilized 1542-nm laser.The results are within the uncertainty range of the international recommended values.Our results demonstrate the accurate optical frequency measurement of lasers at different frequencies using the femtosecond optical frequency comb,which is not only important for the precise and accurate traceability and calibration of the laser frequencies,but also provides technical support for establishing the national wavelength standards based on the femtosecond optical frequency comb.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61435002,61527823,and 61321063)
文摘We numerically simulate the generation of an optical frequency comb(OFC) in a microring based on the traditional Si_3N_4 strip waveguide and a temperature compensated slot waveguide.The results show that OFCs are susceptible to temperature with strip waveguide while they can keep stable when temperature changes 10 Kin either low-Q(10~5) or highQ(10~6) microcavity with the well-designed slot waveguide,which has great superiority in practical applications where the temperature drift of the cavity due to the intense pump or surrounding change is unavoidable.
文摘Direct-comb spectroscopy techniques uses optical frequency combs(OFCs)as spectroscopic light source.They deliver high sensitivity,high frequency resolution and precision in a broad spectral range.Due to these features,the field has burgeoned in recent years.In this work we constructed an OFC-based cavity-enhanced Fourier-transform spectrometer in the nearinfrared region and used it for a line-shape study of rovibrational transitions of CO perturbed by Ar.The highly sensitive measurements spanned the wavenumber range from 6270 cm^-1 to 6410 cm^-1,which covered both P and R branch of the second overtone band of CO.The spectrometer delivers high-resolution surpassing the Fourier-transform resolution limit determined by interferogram length,successfully removing ringing and broadening effects caused by instrumental line shape function.The instrumental-line-shape-free method and high signal-to-noise ratio in the measurement allowed us to observe collisional effects beyond those described by the Voigt profile.We retrieved collisional line-shape parameters by fitting the speed-dependent Voigt profile and found good agreement with the values given by precise cavity ring-down spectroscopy measurements that used a continuous-wave laser referenced to a stabilized OFC.The results demonstrate that OFC-based cavity-enhanced Fouriertransform spectroscopy is a strong tool for accurate line-shape studies that will be crucial for future spectral databases.
基金Project supported by the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB35030101)the National Natural Science Foundation of China(Grant No.61825505)+1 种基金the Quantum Control and Quantum Information of the National Key Research and Development Program of China(Grant No.2020YFA0309800)the Natural Science Basic Research Program of Shaanxi Province,China(Grant No.2020JQ434)。
文摘We demonstrate an optical frequency comb(OFC)based on a turnkey mode-locked laser with a figure-9-shape structure and polarization-maintaining fibers,for the comparison of frequency among optical clocks with wavelengths of 698 nm,729 nm,1068 nm,and 1156 nm.We adopt a multi-branch approach in order to produce high power OFC signals at these specific wavelengths,enabling the signal-to-noise ratio of the beatnotes between the OFC and the clock lasers to exceed30 d B at a resolution bandwidth of 300 k Hz.This approach makes the supercontinuum spectra much easier to be generated than a single branch OFC.However,more out-of-loop fibers degrade the long-term frequency instability due to thermal drift.To minimize the thermal drift effect,we set the fiber lengths of different branches to be similar,and we stabilize the temperature as well.The out-of-loop frequency instability of the OFC due to the incoherence of the multi-branch is about5.5×10^(19) for 4000 s,while the in-loop frequency instability of fceo and that of fbeat are 7.5×10^(18) for 1 s and 8.5×10^(18) for 1 s,respectively.The turnkey OFC meets the requirement for the comparison of frequency between the best optical clocks.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12074331,61875238,and 61971373)the Natural Science Foundation of Hebei Province,China(Grant Nos.F2021203002,F2019203549,and F2020203050)the Science and Technology Support Projects of Research and Development Plans of Qinhuangdao City(Grant No.202004A001).
文摘We numerically investigate the mid-infrared(MIR)supercontinuum(SC)and SC-based optical frequency comb(OFC)generations when the three optical modes(LP_(01),LP_(02),and LP_(12))are considered in a multimode tellurite photonic crystal fiber(MM-TPCF).The geometrical parameters of the MM-TPCF are optimized to support the multimode propagation and obtain the desired dispersion characteristics of the considered three optical modes.When the pump pulse with center wavelengthλ=2.5μm,width T=80 fs,and peak power P=18 kW is coupled into the anomalous dispersion region of the LP_(01),LP_(02),and LP_(12)modes of the MM-TPCF,the-40-dB bandwidth of the generated MIR SCs can be up to 2.56,1.39,and 1.12 octaves,respectively,along with good coherence.Moreover,the nonlinear dynamics of the generated SCs are analyzed.Finally,the MIR SCs-based OFCs are demonstrated when a train of 50 pulses at 1-GHz repetition rate is used as the pump source and launched into the MM-TPCF.
基金Project supported by the National Natural Science Foundation of China(Grant No.62005215)。
文摘The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective four wave-mixing in the active semiconductor gain medium. The low-noise Gaussian-like pulse can be obtained by locking the relaxation oscillation and compensating the gain asymmetry. The simulations suggest that pulse trains of width below 30 ps and repetition rate in GHz frequency can be generated simply by the optical injection locking of semiconductor lasers. Since the optical injection locking can broaden the spectrum and amplify the optical power simultaneously, it can be a good initial stage for generating optical frequency combs from dual-frequency lasers by multi-stage of spectral broadening in nonlinear waveguides.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.91336101 and 61127901)West Light Foundation of the Chinese Academy of Sciences(Grant No.2013ZD02)
文摘We demonstrate an optical frequency comb based on an erbium-doped-fiber femtosecond laser with the nonlinear polarization evolution scheme.The repetition rate of the laser is about 209 MHz.By controlling an intra-cavity electrooptic modulator and a piezo-transducer,the repetition rate can be stabilized with a high-bandwidth servo in a frequency range of 3 k Hz,enabling long-term repetition rate phase-locking.The in-loop frequency stability of repetition rate is about1.6×10-13 in an integration time of 1 s,limited by the measurement system;and it is inversely proportional to integration time in the short term.Furthermore,using a common path f –2 f interferometer,the carrier envelope offset frequency of the comb is obtained with a signal-to-noise ratio of 40 d B in a 3-MHz resolution bandwidth.Stabilized carrier envelope offset frequency exhibits a deviation of 0.6 m Hz in an integration time of 1 s.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61475099 and 61922040)Program of State Key Laboratory of Quantum Optics and Quantum Optics Devices,China(Grant No.KF201701)the Key R&D Program of Guangdong Province,China(Grant No.2018B030325002)。
文摘Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study of signals during the generation of the Kerr optical frequency combs(OFCs). We find that the signals in different states, including the Turing pattern, the chaos, the single soliton state, and the multi-solitons state, can be distinguished according to different distributions of the eigenvalue spectrum. Specially, the eigenvalue spectrum of the single soliton pulse is composed of a pair of conjugate symmetric discrete eigenvalues and the quasi-continuous eigenvalue spectrum with eye-like structure.Moreover, we have successfully demonstrated that the number of discrete eigenvalue pairs in the eigenvalue spectrum corresponds to the number of solitons formed in a round-trip time inside the Kerr microresonator. This work shows that some characteristics of the time-domain signal can be well reflected in the nonlinear domain.
基金Project supported by the National Fundamental Research Program of China (Grant Nos 2005CB3724500 and 2006CB921400)the Major Program of National Natural Science Foundation of China (Grant No 60490280)National Natural Science Foundation of China (Grant No 10574005)
文摘This paper reports that two identical external-cavity-diode-laser (ECDL) based spectrometers are constructed at 634 nm referencing on the hyperfine B-X transition R(80)8-4 of 127I2. The lasers are stabilized on the Doppler-free absorption signals using the third-harmonic detection technique. The instability of the stabilized laser is measured to be 2.8 × 10-12 (after 1000 s) by counting the beat note between the two lasers. The absolute optical frequency of the transition is, for the first time, determined to be 472851936189.5 kHz by using an optical frequency comb referenced on the microwave caesium atomic clock. The uncertainty of the measurement is less than 4.9 kHz.
基金We are grateful for financial supports from the National Natural Science Foundation of China(Grant No.61527823)the National Key R&D Program of China(Grant No.2017YFB0405301).
文摘The generation of high-repetition rate(frep≥10 GHz)ultra-broadband optical frequency combs(OFCs)at 1550 nm and 1310 nm is investigated by seeding two types of highly nonlinear fibers(HNLFs)with 10 GHz picosecond pulses at the pump wavelength of 1550 nm.When pumped near the zero dispersion wavelength(ZDW)in the normal dispersion region of a HNLF,10 GHz flat-topped OFC with 43 nm bandwidth within 5 dB power variation is generated by self-phase modulation(SPM)-based OFC spectral broadening at 26.5 dBm pump power,and 291 fs pulse trains with 10 GHz repetition rate are obtained at 18 dBm pump power without complicated pulse shaping methods.Furthermore,when pumped in the abnormal dispersion region of a HNLF,OFCs with dispersive waves around 1310 nm are studied using a common HNLF and fluorotellurite fibers,which maintain the good coherence of the pump light at 1550 nm.At the same time,sufficient tunability of the generated dispersive waves is achieved when tuning the pump power or ZDW.
基金Project supported by the National Basic Research Program of China(Grant No.2012CB921603)the Program for Changjiang Scholars and Innovative Research Team in University(Grant No.IRT13076)+2 种基金the National Natural Science Foundation of China(Grant Nos.61378049 and 10934004)the International Science and Technology Cooperation Program of China(Grant No.2011DFA12490)the Natural Science Foundation of Shanxi Province,China(Grant No.2011011004)
文摘The high precision two-photon excitation measurements for 5S1/2(F87g = 2) to 5D5/2(Fe = 4 to 1) ofRb are performed by using an optical frequency comb.The two counter-propagating femtosecond pulses(5S1/2→5P3/2at 780 nm,and 5P3/2→5D5/2at 776 nm) act on87 Rb vapor,and the Doppler broadened background signal is effectively eliminated.The temperature and power dependences of the two-photon spectrum are studied in this paper.
基金Russian Science Foundation.Sections 1,2,and 3.3 were supported by Grant 23-12-00057,Sects.3.1 and 3.2 were supported by Grant 20-12-00344.
文摘The results of an optoelectronic system—frequency-shifted feedback(FSF)laser experimental examination are presented.The considered FSF laser is seeded only with optical amplifer spontaneous emission(ASE)and operates in the mode-locked regime,whereby the output radiation is sequence of short pulses with a repetition rate determined by the delay time in its optical feedback circuit.In the frequency domain,the spectrum of such a pulse sequence is an optical frequency comb(OFC).These OFCs we call initial.We consider the possibility of tunable acousto-optic(AO)dual and quad-comb frequency spacing downconversion in the FSF laser seeded with ASE and operating in the mode-locked regime.The examined system applies a single frequency shifting loop with single AO tunable flter as the frequency shifter that is fed with several radio frequency signals simultaneously.The initial OFCs with frequency spacing of about 6.5 MHz may be obtained in the wide spectral range and their width,envelope shape and position in the optical spectrum may be tuned.The dual-combs are obtained with a pair of initial OFCs aroused by two various ultrasound waves in the acousto-optic tunable flter(AOTF).The dual-combs frequency spacing is determined by the frequency diference of the signals applied to the AOTF piezoelectric transducer and can be tuned simply.The quad-combs are obtained with three initial OFCs,forming a pair of dual-combs,appearing when three ultrasound frequencies feed the AOTF transducer.The quad-combs frequency spacing is defned by the diference between the frequency spacing of dual-combs.Quad-combs with more than 5000 spectral lines and tunable frequency spacing are observed.The successive frequency downconversion gives the possibility to reduce the OFC frequency spacing form several MHz for initial OFC to tens of kHz for quad-combs.
基金Project supported by the National Key Research and Development Program of China(Grant No.2020YFB0408300)the National Natural Science Foundation of China(Grant No.62175246)+2 种基金the Natural Science Foundation of Shanghai,China(Grant No.22ZR1471100)the Youth Innovation Promotion Association of Chinese Academy of Sciences(Grant No.YIPA2021244)the Innovation Program for Quantum Science and Technology(Grant No.2021ZD0300701).
文摘Future inter-satellite clock comparison on high orbit will require optical time and frequency transmission technology between moving objects.Here,we demonstrate robust optical frequency transmission under the condition of variable link distance.This variable link is accomplished by the relative motion of a single telescope fixed on the experimental platform to a corner-cube reflector(CCR)installed on a sliding guide.Two acousto–optic modulators with different frequencies are used to separate forward signal from backward signal.With active phase noise suppression,when the CCR moves back and forth at a constant velocity of 20 cm/s and an acceleration of 20 cm/s^(2),we achieve the best frequency stability of 1.9×10^(-16) at 1 s and 7.9×10^(-19) at 1000 s indoors.This work paves the way for future studying optical frequency transfer between ultra-high-orbit satellites.
基金Project supported by the National Key Research and Development Program of China(Grant Nos.2021YFA0718300 and 2021YFA1400900)the National Natural Science Foundation of China(Grant Nos.11920101004,11934002,and 92365208)+1 种基金Science and Technology Major Project of Shanxi(Grant No.202101030201022)Space Application System of China Manned Space Program.
文摘Raman lasers are essential in atomic physics,and the development of portable devices has posed requirements for time-division multiplexing of Raman lasers.We demonstrate an innovative gigahertz frequency hopping approach of a slave Raman laser within an optical phase-locked loop(OPLL),which finds practical application in an atomic gravimeter,where the OPLL frequently switches between near-resonance lasers and significantly detuned Raman lasers.The method merges the advantages of rapid and extensive frequency hopping with the OPLL’s inherent low phase noise,and exhibits a versatile range of applications in compact laser systems,promising advancements in portable instruments.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12103059,12033007,12303077,and 12303076)the Fund from the Xi’an Science and Technology Bureau,China(Grant No.E019XK1S04)the Fund from the Youth Innovation Promotion Association of the Chinese Academy of Sciences(Grant No.1188000XGJ).
文摘We demonstrate coherent optical frequency dissemination over a distance of 972 km by cascading two spans where the phase noise is passively compensated for.Instead of employing a phase discriminator and a phase locking loop in the conventional active phase control scheme,the passive phase noise cancellation is realized by feeding double-trip beat-note frequency to the driver of the acoustic optical modulator at the local site.This passive scheme exhibits fine robustness and reliability,making it suitable for long-distance and noisy fiber links.An optical regeneration station is used in the link for signal amplification and cascaded transmission.The phase noise cancellation and transfer instability of the 972-km link is investigated,and transfer instability of 1.1×10^(-19)at 10^(4)s is achieved.This work provides a promising method for realizing optical frequency distribution over thousands of kilometers by using fiber links.
基金Zhaohui Li acknowledges the support of the National Basic Research Programme of China(973)(Project No.2012CB315603)National High Technology 863 Research and Development Program of China(Nos.2013AA013300 and 2013AA013403)+5 种基金the Research Fund for the Doctoral Program of Higher Education of China(20124401110003)National Natural Science Foundation of China(NSFC)(Grant No.61435006)the Program for New Century Excellent Talents in University(NCET-12-0679)in ChinaXuming Zhang acknowledges the NSFC(Grant No.61377068)the Hong Kong Research Grant Council(Grant Nos.PolyU 5327/11E and N_PolyU505/13)the Hong Kong Polytechnic University(Grant Nos.G-YN07,4-BCAL and G-YBBE).
文摘Optical spectral measurements are crucial for optical sensors and many other applications,but the prevailing methods,such as optical spectrum analysis and tunable laser spectroscopy,often have to make compromises among resolution,speed,and accuracy.Optical frequency combs are widely used for metrology of discrete atomic and molecular spectral lines.However,they are usually generated by optical methods and have large comb spacing,which limits the resolution for direct sampling of continuous spectra.To overcome these problems,this paper presents an original method to digitally generate an ultrafine optical frequency comb(UFOFC)as the frequency ruler for spectral measurements.Each comb line provides one sampling point,and the full spectrum can be captured at the same time using coherent detection.For an experimental demonstration,we adopted the inverse fast Fourier transform to generate a UFOFC with a comb spacing of 1.46 MHz over a 10-GHz range and demonstrated its functions using a Mach–Zehnder refractive index sensor.The UFOFC obtains a spectral resolution of 0.01 pm and response time of 0.7 μs;both represent 100-fold improvements over the state of the art and could be further enhanced by several orders of magnitude.The UFOFC presented here could facilitate new label-free sensor applications that require both high resolution and fast speed,such as measuring binding kinetics and single-molecule dynamics.
基金Strategic Priority Research Program of the Chinese Academy of Sciences(CAS)(XDB 24030600)National Key Research and Development Program of China(2016YFF0200702)+1 种基金National Natural Science Foundation of China(NSFC)(61690222,61308037,61635013)CASSAFEA International Partnership Program for Creative Research Teams
文摘Dual-pumped microring-resonator-based optical frequency combs(OFCs) and their temporal characteristics are numerically investigated and experimentally explored. The calculation results obtained by solving the driven and damped nonlinear Schr?dinger equation indicate that an ultralow coupled pump power is required to excite the primary comb modes through a non-degenerate four-wave-mixing(FWM) process and, when the pump power is boosted, both the comb mode intensities and spectral bandwidths increase. At low pump powers, the field intensity profile exhibits a cosine variation manner with frequency equal to the separation of the two pumps, while a roll Turing pattern is formed resulting from the increased comb mode intensities and spectral bandwidths at high pump powers. Meanwhile, we found that the power difference between the two pump fields can be transferred to the newly generated comb modes, which are located on both sides of the pump modes, through a cascaded FWM process. Experimentally, the dual-pumped OFCs were realized by coupling two self-oscillating pump fields into a microring resonator. The numerically calculated comb spectrum is verified by generating an OFC with 2.0 THz mode spacing over 160 nm bandwidth. In addition, the formation of a roll Turing pattern at high pump powers is inferred from the measured autocorrelation trace of a 10 free spectral range(FSR) OFC. The experimental observations accord well with the numerical predictions. Due to their large and tunable mode spacing, robustness,and flexibility, the proposed dual-pumped OFCs could find potential applications in a wide range of fields,including arbitrary optical waveform generation, high-capacity optical communications, and signal-processing systems.
基金Japan Science and Technology Agency(JST)Japan Agency for Medical Research and Development(AMED)
文摘We demonstrated stable midinfrared(MIR) optical frequency comb at the 3.0 μm region with difference frequency generation pumped by a high power, Er-doped, ultrashort pulse fiber laser system. A soliton mode-locked161 MHz high repetition rate fiber laser using a single wall carbon nanotube was fabricated. The output pulse was amplified in an Er-doped single mode fiber amplifier, and a 1.1–2.2 μm wideband supercontinuum(SC) with an average power of 205 m W was generated in highly nonlinear fiber. The spectrogram of the generated SC was examined both experimentally and numerically. The generated SC was focused into a nonlinear crystal, and stable generation of MIR comb around the 3 μm wavelength region was realized.
基金supported by the National Key R&D Program of China(No.2017YFA0304403)the National Natural Science Foundation of China(Nos.11927810,11822402,and11804094)。
文摘We report a long-term frequency-stabilized optical frequency comb at 530–1100 nm based on a turnkey Ti:sapphire modelocked laser.With the help of a digital controller,turnkey operation is realized for the Ti:sapphire mode-locked laser.Under optimized design of the laser cavity,the laser can be mode-locked over a month,limited by the observation time.The combination of a fast piezo and a slow one inside the Ti:sapphire mode-locked laser allows us to adjust the cavity length with moderate bandwidth and tuning range,enabling robust locking of the repetition rate(f_(r)) to a hydrogen maser.By combining a fast analog feedback to pump current and a slow digital feedback to an intracavity wedge and the pump power of the Ti:sapphire mode-locked laser,the carrier envelope offset frequency(f_(ceo)) of the comb is stabilized.We extend the continuous frequency-stabilized time of the Ti:sapphire optical frequency comb to five days.The residual jitters of f;and f;are 0.08 m Hz and 2.5 m Hz at 1 s averaging time,respectively,satisfying many applications demanding accuracy and short operation time for optical frequency combs.
