Tunable Airy beams with controllable propagation trajectories have sparked interest in various fields,such as optical manipulation and laser fabrication.Existing research approaches encounter challenges related to ins...Tunable Airy beams with controllable propagation trajectories have sparked interest in various fields,such as optical manipulation and laser fabrication.Existing research approaches encounter challenges related to insufficient compactness and integration feasibility,or they require enhanced tunability to enable real-time dynamic manipulation of the propagation trajectory.In this work,we present a novel method that utilizes a dual metasurface system to surpass these limitations,significantly enhancing the practical potential of the Airy beam.Our approach involves encoding a cubic phase profile and two off-axis Fresnel lens phase profiles across the two metasurfaces.The validity of the proposed strategy has been confirmed through simulation and experimental results.The proposed meta-device addresses the existing limitations and lays the foundation for broadening the applicability of Airy beams across diverse domains,encompassing light-sheet microscopy,laser fabrication,optical tweezers,etc.展开更多
The seawater desalination based on solardriven interfacial evaporation has emerged as a promising technique to alleviate the global crisis on freshwater shortage.However,achieving high desalination performance on actu...The seawater desalination based on solardriven interfacial evaporation has emerged as a promising technique to alleviate the global crisis on freshwater shortage.However,achieving high desalination performance on actual,oil-contaminated seawater remains a critical challenge,because the transport channels and evaporation interfaces of the current solar evaporators are easily blocked by the oil slicks,resulting in undermined evaporation rate and conversion efficiency.Herein,we propose a facile strategy for fabricating a modularized solar evaporator based on flexible MXene aerogels with arbitrarily tunable,highly ordered cellular/lamellar pore structures for high-efficiency oil interception and desalination.The core design is the creation of 1D fibrous MXenes with sufficiently large aspect ratios,whose superior flexibility and plentiful link forms lay the basis for controllable 3D assembly into more complicated pore structures.The cellular pore structure is responsible for effective contaminants rejection due to the multi-sieving effect achieved by the omnipresent,isotropic wall apertures together with underwater superhydrophobicity,while the lamellar pore structure is favorable for rapid evaporation due to the presence of continuous,large-area evaporation channels.The modularized solar evaporator delivers the best evaporation rate(1.48 kg m-2h-1)and conversion efficiency(92.08%)among all MXene-based desalination materials on oil-contaminated seawater.展开更多
Solar-driven interfacial evaporation is an emerging technology for water desalination.Generally,double-layered structure with separate surface wettability properties is usually employed for evaporator construction.How...Solar-driven interfacial evaporation is an emerging technology for water desalination.Generally,double-layered structure with separate surface wettability properties is usually employed for evaporator construction.However,creating materials with tunable properties is a great challenge because the wettability of existing materials is usually monotonous.Herein,we report vinyltrimethoxysilane as a single molecular unit to hybrid with bacterial cellulose(BC)fibrous network,which can be built into robust aerogel with entirely distinct wettability through controlling assembly pathways.Siloxane groups or carbon atoms are exposed on the surface of BC nanofibers,resulting in either superhydrophilic or superhydrophobic aerogels.With this special property,single component-modified aerogels could be integrated into a double-layered evaporator for water desalination.Under 1 sun,our evaporator achieves high water evaporation rates of 1.91 and 4.20 kg m^(-2)h^(-1)under laboratory and outdoor solar conditions,respectively.Moreover,this aerogel evaporator shows unprecedented lightweight,structural robustness,long-term stability under extreme conditions,and excellent salt-resistance,highlighting the advantages in synthesis of aerogel materials from the single molecular unit.展开更多
Localized surface plasmon resonance(LSPR) has caused extensive concern and achieved widespread applications in optoelectronics. However, the weak coupling of plasmons and excitons in a nanometal/semiconductor system r...Localized surface plasmon resonance(LSPR) has caused extensive concern and achieved widespread applications in optoelectronics. However, the weak coupling of plasmons and excitons in a nanometal/semiconductor system remains to be investigated via energy transfer. Herein, bandgap tunable perovskite films were synthesized to adjust the emission peaks,for further coupling with stable localized surface plasmons from gold nanoparticles. The degree of mismatch, using steadystate and transient photoluminescence(PL), was investigated systematically in two different cases of gold nanoparticles that were in direct contacting and insulated. The results demonstrated the process of tuning emission coupled to LSPR via wavelength-dependent photoluminescence intensity in the samples with an insulating spacer. In the direct contact case,the decreased radiative decay rate involves rapid plasmon resonance energy transfer to the perovskite semiconductor and non-radiative energy transfer to metal nanoparticles in the near-field range.展开更多
Metamaterials have attracted increasing attention in recent years due to their powerful abilities in manipulating electromagnetic (EM) waves. However, most previously reported metamaterials are unable to actively cont...Metamaterials have attracted increasing attention in recent years due to their powerful abilities in manipulating electromagnetic (EM) waves. However, most previously reported metamaterials are unable to actively control full-band EM waves. In this paper, we propose a thermo-tunable broadband metamaterial (T-TBM) using paraffin-based composites (PD-Cs) with different phase transition temperatures. Active control of the T-TBM reflection loss peaks from low to high frequency is realized by manipulating the solid–liquid state of the PD-Cs at different phase transition temperatures. The absorption peak bandwidth (where the reflection loss value is less than −30 dB) can be changed, while the broad bandwidth absorption (where the reflection loss value is less than −10 dB) is satisfied by adjusting the temperature of the T-TBM. It is shown that the stagnation of the phase transition temperature of the PD-Cs in the T-TBM provides a time window for actively controlling the EM wave absorption response under different thermal conditions. The device has a broad application prospect in the fields of EM absorption, intelligent metamaterials, multifunctional structural devices, and more.展开更多
Transparent microwave absorbers that exhibit high optical transmittance and microwave absorption capability are ideal,although having a fixed absorption performance limits their applicability.Here,a simple,transparent...Transparent microwave absorbers that exhibit high optical transmittance and microwave absorption capability are ideal,although having a fixed absorption performance limits their applicability.Here,a simple,transparent,and thermally tunable microwave absorber is proposed,based on a patterned vanadium dioxide(VO_(2))film.Numerical calculations and experiments demonstrate that the proposed VO_(2)absorber has a high optical transmittance of 84.9%at 620 nm;its reflection loss at 15.06 GHz can be thermally tuned from–4.257 to–60.179 dB,and near-unity absorption is achieved at 523.750 K.Adjusting only the patterned VO_(2)film duty cycle can change the temperature of near-unity absorption.Our VO_(2)absorber has a simple composition,a high optical transmittance,a thermally tunable microwave absorption performance,a large modulation depth,and an adjustable temperature tuning range,making it promising for application in tunable sensors,thermal emitters,modulators,thermal imaging,bolometers,and photovoltaic devices.展开更多
Topological interface state(TIS)of elastic wave has attracted significant research interest due to its potential prospects in strengthening acoustic energy and enhancing the signal accuracy of damage identification an...Topological interface state(TIS)of elastic wave has attracted significant research interest due to its potential prospects in strengthening acoustic energy and enhancing the signal accuracy of damage identification and quantification.However,previous implementations on the interface modes of surface waves are limited to the non-adjustable frequency band and unalterable mode width.Here,we demonstrate the tunable TIS and topological resonance state(TRS)of Rayleigh wave by using a shape memory alloy(SMA)stubbed semi-infinite one-dimensional(1D)solid phononic crystals(PnCs),which simultaneously possesses the adjustable mode width.The mechanism of tunability stems from the phase transformation of the SMA between the martensite at low temperature and the austenite at high temperature.The tunable TIS of Rayleigh wave is realized by combining two bandgap-opened PnCs with different Zak phases.The TRS with adjustable mode width is achieved in the heterostructures by adding PnCs with Dirac point to the middle of two bandgap-opened PnCs with different Zak phases,which exhibits the extraordinary robustness in contrast to the ordinary Fabry–Perot resonance state.This research provides new possibilities for the highly adjustable Rayleigh wave manipulation and find promising applications such as tunable energy harvesters,wide-mode filters,and high-sensitivity Rayleigh wave detectors.展开更多
The defect chemistry is successfully modulated on free-standing and binder-free carbon cathodes for highly efficient Li-S redox reactions.Such rationally regulated defect engineering realizes the synchronization of io...The defect chemistry is successfully modulated on free-standing and binder-free carbon cathodes for highly efficient Li-S redox reactions.Such rationally regulated defect engineering realizes the synchronization of ion/electron-conductive and defect-rich networks on the threedimension carbon cathode,leading to its tunable activity for both relieving the shuttle phenomenon and accelerating the sulfur redox reaction kinetics.As expected,the defective carbon cathode harvests a high rate capacity of 1217.8 mAh g^(-1)at 0.2 C and a superior capacity retention of61.7%at 2 C after 500 cycles.Even under the sulfur mass loading of 11.1 mg cm^(-2),the defective cathode still holds a remarkable areal capacity of 8.5 mAh cm^(-2).展开更多
Dynamically tunable laser sources are highly promising for realizing visionary concepts of integrated photonic circuits and other applications. In this paper, a Ga N-based laser with an integrated PN junction heater o...Dynamically tunable laser sources are highly promising for realizing visionary concepts of integrated photonic circuits and other applications. In this paper, a Ga N-based laser with an integrated PN junction heater on Si is fabricated.The photoluminescence properties of the Ga N beam cavity are controlled by temperature, and the Joule heater provides electrically driven regulation of temperature. These two features of the cavity make it possible to realize convenient tuning of the lasing properties. The multi-functional Ga N beam cavity achieves optically pumped lasing with a single mode near 362.4 nm with a high Q-factor of 1394. The temperature of this device increases by 0–5℃ under the Joule heating effect. Then, electrical control of the lasing mode is demonstrated. The lasing resonant peak shows a continuous redshift of about 0.5 nm and the device also exhibits dynamic switching of its lasing mode. The lasing modulation can be ascribed to temperature-induced reduction of the bandgap. Our work may be of benefit for external optical modulation in future chip-based optoelectronic devices.展开更多
Chirp-rate-tunable microwave waveforms(CTMWs)with dynamically tunable parameters are of basic interest to many practical applications.Recently,photonic generation of microwave signals has made their bandwidths wider a...Chirp-rate-tunable microwave waveforms(CTMWs)with dynamically tunable parameters are of basic interest to many practical applications.Recently,photonic generation of microwave signals has made their bandwidths wider and more convenient for optical fiber transmission.An all-optical method for generation of multiband CTMWs is proposed and demonstrated on all-fiber architecture,relying on dual temporal cavity solitons with agile repetition rate.In the experiment,the triangular optical chirp microwave waveforms with bandwidth above0.45 GHz(ranging from 1.45 GHz to 1.9 GHz)are obtained,and the chirp rate reaches 0.9 GHz/ms.The reconfigurability is also demonstrated by adjusting the control signal.This all-optical approach provides a technical basis for compact,multi-band reconfigurable microwave photonics transmission and reception systems.展开更多
We propose a novel approach for generating a high-density,spatially periodic narrow electron beam comb(EBC)from a plasma grating induced by the interference of two intense laser pulses in subcritical-density plasma.We...We propose a novel approach for generating a high-density,spatially periodic narrow electron beam comb(EBC)from a plasma grating induced by the interference of two intense laser pulses in subcritical-density plasma.We employ particle-in-cell(PIC)simulations to investigate the effects of cross-propagating laser pulses with specific angles overlapping in a subcritical plasma.This overlap results in the formation of a transverse standing wave,leading to a spatially periodic high-density modulation known as a plasma grating.The electron density peak within the grating can reach several times the background plasma density.The charge imbalance between electrons and ions in the electron density peaks causes mutual repulsion among the electrons,resulting in Coulomb expansion and acceleration of the electrons.As a result,some electrons expand into vacuum,forming a periodic narrow EBC with an individual beam width in the nanoscale range.To further explore the formation of the nanoscale EBC,we conduct additional PIC simulations to study the dependence on various laser parameters.Overall,our proposed method offers a promising and controlled approach to generate tunable narrow EBCs with high density.展开更多
In quantum computation and quantum information processing, the manipulation and engineering of quantum systems to suit certain purposes are an ongoing task. One such example is quantum state transfer(QST), an essentia...In quantum computation and quantum information processing, the manipulation and engineering of quantum systems to suit certain purposes are an ongoing task. One such example is quantum state transfer(QST), an essential requirement for both quantum communication and large-scale quantum computation. Here we engineer a chain of four superconducting qubits with tunable couplers to realize the perfect state transfer(PST) protocol originally proposed in quantum spin networks and successfully demonstrate the efficient transfer of an arbitrary single-qubit state from one end of the chain to the other,achieving a high fidelity of 0.986 in just 25 ns. This demonstrated QST is readily to extend to larger chain and multi-node configurations, thus serving as a desirable tool for scalable quantum information processing.展开更多
Three-dimensional(3D)bioprinting has been used widely for the construction of hard tissues such as bone and cartilage.However,constructing soft tissues with complex structures remains a challenge.In this study,complex...Three-dimensional(3D)bioprinting has been used widely for the construction of hard tissues such as bone and cartilage.However,constructing soft tissues with complex structures remains a challenge.In this study,complex structures characterized by both tunable elastic modulus and porosity were printed using freeform reversible embedding of suspended hydrogels(FRESHs)printing methods.A mixture of alginate and gelatin was used as the main functional component of the bioink.Rheological analysis showed that this bioink possesses shear thinning and shear recovery properties,supporting both cryogenic and FRESH printing methods.Potential printing capabilities and limitations of cryogenic and FRESH printing were then analyzed by printability tests.A series of complex structures were printed by FRESH printing methods which could not be realized using conventional approaches.Mechanical tests and scanning electron microscopy analysis showed that the printed structure is of excellent flexibility and could be applied in various conditions by adjusting its mechanical modulus and porosity.L929 fibroblast cells maintained cell viability in cell-laden-printed structures,and the addition of collagen further improved the hydrogels’biocompatibility.Overall,all results provided useful insight into the building of human soft tissue organ blocks.展开更多
In order to improve the rejection capability of mismatched interferer signals,a new two-stage detector is proposed under homogeneous scenarios with unknown covariance matrix,which is obtained by cascading the adaptive...In order to improve the rejection capability of mismatched interferer signals,a new two-stage detector is proposed under homogeneous scenarios with unknown covariance matrix,which is obtained by cascading the adaptive matched filter(AMF)detector and the enhanced RAO(EnRAO)detector.The new detector has constant false alarm performance,and the closed-form expression of probability of false alarm and probability of detection is derived.The performance of the new detector is assessed,and analyzed in comparison with other detectors.The results show that,the proposed detector can provide enhanced rejection capability in the case of mismatch,but the performance of the detector is slightly lost under the condition of matching.展开更多
Wavelength-tunable organic semiconductor lasers based on mechanically stretchable polydimethylsiloxane (PDMS) gratings were developed. The intrinsic stretchability of PDMS was explored to modulate the period of the di...Wavelength-tunable organic semiconductor lasers based on mechanically stretchable polydimethylsiloxane (PDMS) gratings were developed. The intrinsic stretchability of PDMS was explored to modulate the period of the distributed feedback gratings for fine tuning the lasing wavelength. Notably, elastic lasers based on three typical light-emitting molecules show com-parable lasing threshold values analogous to rigid devices and a continuous wavelength tunability of about 10 nm by mechanic-al stretching. In addition, the stretchability provides a simple solution for dynamically tuning the lasing wavelength in a spec-tral range that is challenging to achieve for inorganic counterparts. Our work has provided a simple and efficient method of fab-ricating tunable organic lasers that depend on stretchable distributed feedback gratings, demonstrating a significant step in the advancement of flexible organic optoelectronic devices.展开更多
The 3D hollow hierarchi-cal architectures tend to be designed for inhibiting stack of MXene flakes to obtain satisfactory lightweight,high-e cient and broadband absorbers.Herein,the hollow NiCo compound@MXene networks...The 3D hollow hierarchi-cal architectures tend to be designed for inhibiting stack of MXene flakes to obtain satisfactory lightweight,high-e cient and broadband absorbers.Herein,the hollow NiCo compound@MXene networks were prepared by etching the ZIF 67 template and subsequently anchoring the Ti_(3)C_(2)Tx nanosheets through electrostatic self-assembly.The electromagnetic parameters and microwave absorption property can be distinctly or slightly regulated by adjusting the filler loading and decoration of Ti_(3)C_(2)Tx nanoflakes.Based on the synergistic e ectsof multi-components and special well-constructed structure,NiCo layered double hydroxides@Ti_(3)C_(2)Tx(LDHT-9)absorber remarkably achieves unexpected e ective absorption bandwidth(EAB)of 6.72 GHz with a thickness of 2.10 mm,covering the entire Ku-band.After calcination,transition metal oxide@Ti_(3)C_(2)Tx(TMOT-21)absorber near the percolation threshold possesses minimum reflection loss(RLmin)value of-67.22 dB at 1.70 mm within a filler loading of only 5 wt%.This work enlightens a simple strategy for constructing MXene-based composites to achieve high-e cient microwave absorbents with lightweight and tunable EAB.展开更多
We experimentally demonstrate an electrically triggered terahertz(THz) dual-band tunable band-pass filter based on Si_3 N_4–VO_2–Si_3 N_4 sandwich-structured hybrid metamaterials. The insulator–metal phase transiti...We experimentally demonstrate an electrically triggered terahertz(THz) dual-band tunable band-pass filter based on Si_3 N_4–VO_2–Si_3 N_4 sandwich-structured hybrid metamaterials. The insulator–metal phase transition of VO_2 film is induced by the Joule thermal effect of the top metal layer. The finite-integration-time-domain(FITD) method and finite element method(FEM) are used for numerical simulations. The sample is fabricated using a surface micromachining process,and characterized by a THz time-domain-spectrometer(TDS). When the bias current is 0.225 A, the intensity modulation depths at two central frequencies of 0.56 THz and 0.91 THz are about 81.7% and 81.3%, respectively. This novel design can achieve dynamically electric–thermo–optic modulation in the THz region, and has potential applications in the fields of THz communications, imaging, sensing, and astronomy exploration.展开更多
The lossy nature of indium tin oxide(ITO) at epsilon-near-zero(ENZ) wavelength is used to design an electrically tunable metasurface absorber. The metasurface unit cell is constructed of a circular resonator comprisin...The lossy nature of indium tin oxide(ITO) at epsilon-near-zero(ENZ) wavelength is used to design an electrically tunable metasurface absorber. The metasurface unit cell is constructed of a circular resonator comprising two ITO discs and a high dielectric constant perovskite barium strontium titanate(BST) film. The ENZ wavelength in the accumulation and depletion layers of ITO discs is controlled by applying a single bias voltage. The coupling of magnetic dipole resonance with the ENZ wavelength inside the accumulation layer of ITO film causes total absorption of reflected light. The reflection amplitude can achieve ~84 d B or ~99.99% modulation depth in the operation wavelength of 820 nm at a bias voltage of-2.5 V. Moreover, the metasurface is insensitive to the polarization of the incident light due to the circular design of resonators and the symmetrical design of bias connections.展开更多
Epilepsy is one of the most prevalent neurological disorders affecting 70 million people worldwide.The present work is focused on designing an efficient algorithm for automatic seizure detection by using electroenceph...Epilepsy is one of the most prevalent neurological disorders affecting 70 million people worldwide.The present work is focused on designing an efficient algorithm for automatic seizure detection by using electroencephalogram(EEG) as a noninvasive procedure to record neuronal activities in the brain.EEG signals' underlying dynamics are extracted to differentiate healthy and seizure EEG signals.Shannon entropy,collision entropy,transfer entropy,conditional probability,and Hjorth parameter features are extracted from subbands of tunable Q wavelet transform.Efficient decomposition level for different feature vector is selected using the Kruskal-Wallis test to achieve good classification.Different features are combined using the discriminant correlation analysis fusion technique to form a single fused feature vector.The accuracy of the proposed approach is higher for Q=2 and J=10.Transfer entropy is observed to be significant for different class combinations.Proposed approach achieved 100% accuracy in classifying healthy-seizure EEG signal using simple and robust features and hidden Markov model with less computation time.The proposed approach efficiency is evaluated in classifying seizure and non-seizure surface EEG signals.The system has achieved 96.87% accuracy in classifying surface seizure and nonseizure EEG segments using efficient features extracted from different J level.展开更多
文摘Tunable Airy beams with controllable propagation trajectories have sparked interest in various fields,such as optical manipulation and laser fabrication.Existing research approaches encounter challenges related to insufficient compactness and integration feasibility,or they require enhanced tunability to enable real-time dynamic manipulation of the propagation trajectory.In this work,we present a novel method that utilizes a dual metasurface system to surpass these limitations,significantly enhancing the practical potential of the Airy beam.Our approach involves encoding a cubic phase profile and two off-axis Fresnel lens phase profiles across the two metasurfaces.The validity of the proposed strategy has been confirmed through simulation and experimental results.The proposed meta-device addresses the existing limitations and lays the foundation for broadening the applicability of Airy beams across diverse domains,encompassing light-sheet microscopy,laser fabrication,optical tweezers,etc.
基金support from the National Natural Science Foundation of China(G.Nos.52173055,21961132024,and 51925302)the Ministry of Science and Technology of China(G.No.2021YFE0105100)+3 种基金the Textile Vision Basic Research Program(No.J202201)the International Cooperation Fund of Science and Technology Commission of Shanghai Municipality(G.No.21130750100)the Fundamental Research Funds for the Central Universitiesthe DHU Distinguished Young Professor Program(G.No.LZA2020001)。
文摘The seawater desalination based on solardriven interfacial evaporation has emerged as a promising technique to alleviate the global crisis on freshwater shortage.However,achieving high desalination performance on actual,oil-contaminated seawater remains a critical challenge,because the transport channels and evaporation interfaces of the current solar evaporators are easily blocked by the oil slicks,resulting in undermined evaporation rate and conversion efficiency.Herein,we propose a facile strategy for fabricating a modularized solar evaporator based on flexible MXene aerogels with arbitrarily tunable,highly ordered cellular/lamellar pore structures for high-efficiency oil interception and desalination.The core design is the creation of 1D fibrous MXenes with sufficiently large aspect ratios,whose superior flexibility and plentiful link forms lay the basis for controllable 3D assembly into more complicated pore structures.The cellular pore structure is responsible for effective contaminants rejection due to the multi-sieving effect achieved by the omnipresent,isotropic wall apertures together with underwater superhydrophobicity,while the lamellar pore structure is favorable for rapid evaporation due to the presence of continuous,large-area evaporation channels.The modularized solar evaporator delivers the best evaporation rate(1.48 kg m-2h-1)and conversion efficiency(92.08%)among all MXene-based desalination materials on oil-contaminated seawater.
基金supported by the National Key Research and Development Program of China(2021YFB3701603)National Science Foundation of China(51973030,52103075)+6 种基金Shanghai Rising-Star Program(20QA1400100)Science and Technology Commission of Shanghai Municipality(20JC1414900)China Postdoctoral Science Foundation(2022M710664,2022T150111)China Postdoctoral Science Foundation(2022M710663)the Fundamental Research Funds for the Central Universities“DHU”Distinguished Young Professor Program(LZB2021001)State Key Laboratory for Modification of Chemical Fibers and Polymer Materials,Donghua University。
文摘Solar-driven interfacial evaporation is an emerging technology for water desalination.Generally,double-layered structure with separate surface wettability properties is usually employed for evaporator construction.However,creating materials with tunable properties is a great challenge because the wettability of existing materials is usually monotonous.Herein,we report vinyltrimethoxysilane as a single molecular unit to hybrid with bacterial cellulose(BC)fibrous network,which can be built into robust aerogel with entirely distinct wettability through controlling assembly pathways.Siloxane groups or carbon atoms are exposed on the surface of BC nanofibers,resulting in either superhydrophilic or superhydrophobic aerogels.With this special property,single component-modified aerogels could be integrated into a double-layered evaporator for water desalination.Under 1 sun,our evaporator achieves high water evaporation rates of 1.91 and 4.20 kg m^(-2)h^(-1)under laboratory and outdoor solar conditions,respectively.Moreover,this aerogel evaporator shows unprecedented lightweight,structural robustness,long-term stability under extreme conditions,and excellent salt-resistance,highlighting the advantages in synthesis of aerogel materials from the single molecular unit.
基金Project supported by the National Key R&D Program of China (Grant Nos. 2017YFA0700503 and 2018YFA0209101)the National Natural Science Foundation of China (Grant Nos. 61821002, 11734005, 62075041, and 61704024)。
文摘Localized surface plasmon resonance(LSPR) has caused extensive concern and achieved widespread applications in optoelectronics. However, the weak coupling of plasmons and excitons in a nanometal/semiconductor system remains to be investigated via energy transfer. Herein, bandgap tunable perovskite films were synthesized to adjust the emission peaks,for further coupling with stable localized surface plasmons from gold nanoparticles. The degree of mismatch, using steadystate and transient photoluminescence(PL), was investigated systematically in two different cases of gold nanoparticles that were in direct contacting and insulated. The results demonstrated the process of tuning emission coupled to LSPR via wavelength-dependent photoluminescence intensity in the samples with an insulating spacer. In the direct contact case,the decreased radiative decay rate involves rapid plasmon resonance energy transfer to the perovskite semiconductor and non-radiative energy transfer to metal nanoparticles in the near-field range.
基金supported by the National Natural Science Foundation of China(52003203 and 52075422)the Rapid Manufacturing Engineering Technology Research Center of Shaanxi Province(2017HBGC-06)the Youth Innovation Team of Shaanxi Universities,and the K.C.Wong Education Foundation.
文摘Metamaterials have attracted increasing attention in recent years due to their powerful abilities in manipulating electromagnetic (EM) waves. However, most previously reported metamaterials are unable to actively control full-band EM waves. In this paper, we propose a thermo-tunable broadband metamaterial (T-TBM) using paraffin-based composites (PD-Cs) with different phase transition temperatures. Active control of the T-TBM reflection loss peaks from low to high frequency is realized by manipulating the solid–liquid state of the PD-Cs at different phase transition temperatures. The absorption peak bandwidth (where the reflection loss value is less than −30 dB) can be changed, while the broad bandwidth absorption (where the reflection loss value is less than −10 dB) is satisfied by adjusting the temperature of the T-TBM. It is shown that the stagnation of the phase transition temperature of the PD-Cs in the T-TBM provides a time window for actively controlling the EM wave absorption response under different thermal conditions. The device has a broad application prospect in the fields of EM absorption, intelligent metamaterials, multifunctional structural devices, and more.
基金support from the National Natural Science Foundation of China(61975046)。
文摘Transparent microwave absorbers that exhibit high optical transmittance and microwave absorption capability are ideal,although having a fixed absorption performance limits their applicability.Here,a simple,transparent,and thermally tunable microwave absorber is proposed,based on a patterned vanadium dioxide(VO_(2))film.Numerical calculations and experiments demonstrate that the proposed VO_(2)absorber has a high optical transmittance of 84.9%at 620 nm;its reflection loss at 15.06 GHz can be thermally tuned from–4.257 to–60.179 dB,and near-unity absorption is achieved at 523.750 K.Adjusting only the patterned VO_(2)film duty cycle can change the temperature of near-unity absorption.Our VO_(2)absorber has a simple composition,a high optical transmittance,a thermally tunable microwave absorption performance,a large modulation depth,and an adjustable temperature tuning range,making it promising for application in tunable sensors,thermal emitters,modulators,thermal imaging,bolometers,and photovoltaic devices.
基金the Doctoral Research Fund of University of South China(Grant No.210XQD016)the Outstanding Youth Foundation of the Hunan Education Department(Grant No.21B0406).
文摘Topological interface state(TIS)of elastic wave has attracted significant research interest due to its potential prospects in strengthening acoustic energy and enhancing the signal accuracy of damage identification and quantification.However,previous implementations on the interface modes of surface waves are limited to the non-adjustable frequency band and unalterable mode width.Here,we demonstrate the tunable TIS and topological resonance state(TRS)of Rayleigh wave by using a shape memory alloy(SMA)stubbed semi-infinite one-dimensional(1D)solid phononic crystals(PnCs),which simultaneously possesses the adjustable mode width.The mechanism of tunability stems from the phase transformation of the SMA between the martensite at low temperature and the austenite at high temperature.The tunable TIS of Rayleigh wave is realized by combining two bandgap-opened PnCs with different Zak phases.The TRS with adjustable mode width is achieved in the heterostructures by adding PnCs with Dirac point to the middle of two bandgap-opened PnCs with different Zak phases,which exhibits the extraordinary robustness in contrast to the ordinary Fabry–Perot resonance state.This research provides new possibilities for the highly adjustable Rayleigh wave manipulation and find promising applications such as tunable energy harvesters,wide-mode filters,and high-sensitivity Rayleigh wave detectors.
基金supported by the National Natural Science Foundation of China(52172239)Project of State Key Laboratory of Environment-Friendly Energy Materials+2 种基金Southwest University of Science and Technology(Grant Nos.21fksy24 and 18ZD320304)Chongqing Talents:Exceptional Young Talents Project(Grant No.CQYC201905041)Natural Science Foundation of Chongqing China(Grant No.cstc2021jcyj-jqX0031)。
文摘The defect chemistry is successfully modulated on free-standing and binder-free carbon cathodes for highly efficient Li-S redox reactions.Such rationally regulated defect engineering realizes the synchronization of ion/electron-conductive and defect-rich networks on the threedimension carbon cathode,leading to its tunable activity for both relieving the shuttle phenomenon and accelerating the sulfur redox reaction kinetics.As expected,the defective carbon cathode harvests a high rate capacity of 1217.8 mAh g^(-1)at 0.2 C and a superior capacity retention of61.7%at 2 C after 500 cycles.Even under the sulfur mass loading of 11.1 mg cm^(-2),the defective cathode still holds a remarkable areal capacity of 8.5 mAh cm^(-2).
基金the Natural Science Foundation of Jiangsu Province, China (Grant No. BK20210593)the Foundation of Jiangsu Provincial Double Innovation Doctor Program (Grant No. 30644)+2 种基金the National Natural Science Foundation of China (Grant No. 62204127)State Key Laboratory of Luminescence and Applications (Grant No. SKLA 202104)open research fund of Key Lab of Broadband Wireless Communication and Sensor Network Technology (Nanjing University of Posts and Telecommunications, Ministry of Education)。
文摘Dynamically tunable laser sources are highly promising for realizing visionary concepts of integrated photonic circuits and other applications. In this paper, a Ga N-based laser with an integrated PN junction heater on Si is fabricated.The photoluminescence properties of the Ga N beam cavity are controlled by temperature, and the Joule heater provides electrically driven regulation of temperature. These two features of the cavity make it possible to realize convenient tuning of the lasing properties. The multi-functional Ga N beam cavity achieves optically pumped lasing with a single mode near 362.4 nm with a high Q-factor of 1394. The temperature of this device increases by 0–5℃ under the Joule heating effect. Then, electrical control of the lasing mode is demonstrated. The lasing resonant peak shows a continuous redshift of about 0.5 nm and the device also exhibits dynamic switching of its lasing mode. The lasing modulation can be ascribed to temperature-induced reduction of the bandgap. Our work may be of benefit for external optical modulation in future chip-based optoelectronic devices.
基金the National Natural Science Foundation of China(Grant Nos.61675009 and 61325021)the Key Program of Beijing Municipal Natural Science Foundation(Grant No.KZ201910005006)。
文摘Chirp-rate-tunable microwave waveforms(CTMWs)with dynamically tunable parameters are of basic interest to many practical applications.Recently,photonic generation of microwave signals has made their bandwidths wider and more convenient for optical fiber transmission.An all-optical method for generation of multiband CTMWs is proposed and demonstrated on all-fiber architecture,relying on dual temporal cavity solitons with agile repetition rate.In the experiment,the triangular optical chirp microwave waveforms with bandwidth above0.45 GHz(ranging from 1.45 GHz to 1.9 GHz)are obtained,and the chirp rate reaches 0.9 GHz/ms.The reconfigurability is also demonstrated by adjusting the control signal.This all-optical approach provides a technical basis for compact,multi-band reconfigurable microwave photonics transmission and reception systems.
基金This work was supported by the National Natural Science Foundation of China(Grant Nos.12174410,11991072,11991074,12225411,and 12105353)the CAS Project for Young Scientists in Basic Research(Grant No.YSBR060)the State Key Laboratory Program of the Chinese Ministry of Science and Technology,and the CAS Youth Innovation Promotion Association(Grant Nos.Y201952 and 2022242).
文摘We propose a novel approach for generating a high-density,spatially periodic narrow electron beam comb(EBC)from a plasma grating induced by the interference of two intense laser pulses in subcritical-density plasma.We employ particle-in-cell(PIC)simulations to investigate the effects of cross-propagating laser pulses with specific angles overlapping in a subcritical plasma.This overlap results in the formation of a transverse standing wave,leading to a spatially periodic high-density modulation known as a plasma grating.The electron density peak within the grating can reach several times the background plasma density.The charge imbalance between electrons and ions in the electron density peaks causes mutual repulsion among the electrons,resulting in Coulomb expansion and acceleration of the electrons.As a result,some electrons expand into vacuum,forming a periodic narrow EBC with an individual beam width in the nanoscale range.To further explore the formation of the nanoscale EBC,we conduct additional PIC simulations to study the dependence on various laser parameters.Overall,our proposed method offers a promising and controlled approach to generate tunable narrow EBCs with high density.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 12034018 and 11625419)。
文摘In quantum computation and quantum information processing, the manipulation and engineering of quantum systems to suit certain purposes are an ongoing task. One such example is quantum state transfer(QST), an essential requirement for both quantum communication and large-scale quantum computation. Here we engineer a chain of four superconducting qubits with tunable couplers to realize the perfect state transfer(PST) protocol originally proposed in quantum spin networks and successfully demonstrate the efficient transfer of an arbitrary single-qubit state from one end of the chain to the other,achieving a high fidelity of 0.986 in just 25 ns. This demonstrated QST is readily to extend to larger chain and multi-node configurations, thus serving as a desirable tool for scalable quantum information processing.
基金supported by the National Natural Science Foundation of China(Nos.52275464 and 52075300)the Scientific Research Project for National High-Level Innovative Talents ofHebei Province Full-Time Introduction(No.2021HBQZYCXY004).
文摘Three-dimensional(3D)bioprinting has been used widely for the construction of hard tissues such as bone and cartilage.However,constructing soft tissues with complex structures remains a challenge.In this study,complex structures characterized by both tunable elastic modulus and porosity were printed using freeform reversible embedding of suspended hydrogels(FRESHs)printing methods.A mixture of alginate and gelatin was used as the main functional component of the bioink.Rheological analysis showed that this bioink possesses shear thinning and shear recovery properties,supporting both cryogenic and FRESH printing methods.Potential printing capabilities and limitations of cryogenic and FRESH printing were then analyzed by printability tests.A series of complex structures were printed by FRESH printing methods which could not be realized using conventional approaches.Mechanical tests and scanning electron microscopy analysis showed that the printed structure is of excellent flexibility and could be applied in various conditions by adjusting its mechanical modulus and porosity.L929 fibroblast cells maintained cell viability in cell-laden-printed structures,and the addition of collagen further improved the hydrogels’biocompatibility.Overall,all results provided useful insight into the building of human soft tissue organ blocks.
基金supported by the National Natural Science Foundation of China(No.61971412).
文摘In order to improve the rejection capability of mismatched interferer signals,a new two-stage detector is proposed under homogeneous scenarios with unknown covariance matrix,which is obtained by cascading the adaptive matched filter(AMF)detector and the enhanced RAO(EnRAO)detector.The new detector has constant false alarm performance,and the closed-form expression of probability of false alarm and probability of detection is derived.The performance of the new detector is assessed,and analyzed in comparison with other detectors.The results show that,the proposed detector can provide enhanced rejection capability in the case of mismatch,but the performance of the detector is slightly lost under the condition of matching.
基金financial support from the National Natural Science Foundation of China (21835003, 91833304,21422402, 62274097, 21674050, 62004106)the National Key Basic Research Program of China (2014CB648300,2017YFB0404501)+11 种基金the Natural Science Foundation of Jiangsu Province (BE2019120, BK20160888)Program for Jiangsu Specially-Appointed Professor (RK030STP15001)the Six Talent Peaks Project of Jiangsu Province (TD-XCL-009)the333 Project of Jiangsu Province (BRA2017402)the Natural Science Foundation of the Jiangsu Higher Education Institutions of China (20KJB140005)China Postdoctoral Science Foundation (2020M671553)the NUPT"1311 Project"and Scientific Foundation (NY217169, NY215062, NY215107,NY217087)the Leading Talent of Technological Innovation of National Ten-Thousands Talents Program of Chinathe Excellent Scientific and Technological Innovative Teams of Jiangsu Higher Education Institutions (TJ217038)the Postgraduate Research&Practice Innovation Program of Jiangsu Province (SJCX21-0297)the Synergetic Innovation Center for Organic Electronics and Information Displaysthe Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
文摘Wavelength-tunable organic semiconductor lasers based on mechanically stretchable polydimethylsiloxane (PDMS) gratings were developed. The intrinsic stretchability of PDMS was explored to modulate the period of the distributed feedback gratings for fine tuning the lasing wavelength. Notably, elastic lasers based on three typical light-emitting molecules show com-parable lasing threshold values analogous to rigid devices and a continuous wavelength tunability of about 10 nm by mechanic-al stretching. In addition, the stretchability provides a simple solution for dynamically tuning the lasing wavelength in a spec-tral range that is challenging to achieve for inorganic counterparts. Our work has provided a simple and efficient method of fab-ricating tunable organic lasers that depend on stretchable distributed feedback gratings, demonstrating a significant step in the advancement of flexible organic optoelectronic devices.
基金supported by the National Natural Science Foundation of China(No.52073010)Beijing Natural Science Foundation(2214069)。
文摘The 3D hollow hierarchi-cal architectures tend to be designed for inhibiting stack of MXene flakes to obtain satisfactory lightweight,high-e cient and broadband absorbers.Herein,the hollow NiCo compound@MXene networks were prepared by etching the ZIF 67 template and subsequently anchoring the Ti_(3)C_(2)Tx nanosheets through electrostatic self-assembly.The electromagnetic parameters and microwave absorption property can be distinctly or slightly regulated by adjusting the filler loading and decoration of Ti_(3)C_(2)Tx nanoflakes.Based on the synergistic e ectsof multi-components and special well-constructed structure,NiCo layered double hydroxides@Ti_(3)C_(2)Tx(LDHT-9)absorber remarkably achieves unexpected e ective absorption bandwidth(EAB)of 6.72 GHz with a thickness of 2.10 mm,covering the entire Ku-band.After calcination,transition metal oxide@Ti_(3)C_(2)Tx(TMOT-21)absorber near the percolation threshold possesses minimum reflection loss(RLmin)value of-67.22 dB at 1.70 mm within a filler loading of only 5 wt%.This work enlightens a simple strategy for constructing MXene-based composites to achieve high-e cient microwave absorbents with lightweight and tunable EAB.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11574059,61565004,and 11774288)the National Technology Major Special Project,China(Grant No.2017ZX02101007-003)+2 种基金the Natural Science Foundation of Guangxi,China(Grant Nos.2015GXNSFDA139039 and2017GXNSFBA198116)the Foundation from Guangxi Key Laboratory of Automatic Detection Technology and Instrument,China(Grant No.YQ16101)the Innovation of Guangxi Graduate Education,China(Grant Nos.2018YJCX70,2018YJCX67,and 2018YJCX74)
文摘We experimentally demonstrate an electrically triggered terahertz(THz) dual-band tunable band-pass filter based on Si_3 N_4–VO_2–Si_3 N_4 sandwich-structured hybrid metamaterials. The insulator–metal phase transition of VO_2 film is induced by the Joule thermal effect of the top metal layer. The finite-integration-time-domain(FITD) method and finite element method(FEM) are used for numerical simulations. The sample is fabricated using a surface micromachining process,and characterized by a THz time-domain-spectrometer(TDS). When the bias current is 0.225 A, the intensity modulation depths at two central frequencies of 0.56 THz and 0.91 THz are about 81.7% and 81.3%, respectively. This novel design can achieve dynamically electric–thermo–optic modulation in the THz region, and has potential applications in the fields of THz communications, imaging, sensing, and astronomy exploration.
基金supported by the Agency for Science, Technology and Research (A*STAR) under AME IRG Grant No. A2083c0058AME IAF-PP Grant No. 182 24 30030+1 种基金HBMS IAF-PP Grant No. H19H6a0025by MOE Tier 3 program LUNI170919a PUBMOE。
文摘The lossy nature of indium tin oxide(ITO) at epsilon-near-zero(ENZ) wavelength is used to design an electrically tunable metasurface absorber. The metasurface unit cell is constructed of a circular resonator comprising two ITO discs and a high dielectric constant perovskite barium strontium titanate(BST) film. The ENZ wavelength in the accumulation and depletion layers of ITO discs is controlled by applying a single bias voltage. The coupling of magnetic dipole resonance with the ENZ wavelength inside the accumulation layer of ITO film causes total absorption of reflected light. The reflection amplitude can achieve ~84 d B or ~99.99% modulation depth in the operation wavelength of 820 nm at a bias voltage of-2.5 V. Moreover, the metasurface is insensitive to the polarization of the incident light due to the circular design of resonators and the symmetrical design of bias connections.
文摘Epilepsy is one of the most prevalent neurological disorders affecting 70 million people worldwide.The present work is focused on designing an efficient algorithm for automatic seizure detection by using electroencephalogram(EEG) as a noninvasive procedure to record neuronal activities in the brain.EEG signals' underlying dynamics are extracted to differentiate healthy and seizure EEG signals.Shannon entropy,collision entropy,transfer entropy,conditional probability,and Hjorth parameter features are extracted from subbands of tunable Q wavelet transform.Efficient decomposition level for different feature vector is selected using the Kruskal-Wallis test to achieve good classification.Different features are combined using the discriminant correlation analysis fusion technique to form a single fused feature vector.The accuracy of the proposed approach is higher for Q=2 and J=10.Transfer entropy is observed to be significant for different class combinations.Proposed approach achieved 100% accuracy in classifying healthy-seizure EEG signal using simple and robust features and hidden Markov model with less computation time.The proposed approach efficiency is evaluated in classifying seizure and non-seizure surface EEG signals.The system has achieved 96.87% accuracy in classifying surface seizure and nonseizure EEG segments using efficient features extracted from different J level.
