Fast photography and optical emission spectroscopy are implemented in a 5 mm neon gap dielectric barrier discharge(DBD) at atmospheric pressure with quartz glass used as the dielectric layer. Results show that it star...Fast photography and optical emission spectroscopy are implemented in a 5 mm neon gap dielectric barrier discharge(DBD) at atmospheric pressure with quartz glass used as the dielectric layer. Results show that it starts with a Townsend discharge and ends at a sub-normal glow discharge in neon DBD. Based on the Townsend discharge, the first ionization coefficient of neon is measured. The measurements are consistent with those at low pressure. Optical emission spectroscopy indicates that the spectra are mainly composed of atomic lines of neon, molecular bands and molecular ion bands originating from inevitable gas impurities(mainly nitrogen).Moreover, spectral lines emitted from atomic neon corresponding to the transitions(2p^5 3p→2p^5 3s) are predominant. Although the second positive system of N_2(C^3Π_u→B^3Π_g) is observed, their intensities are too weak compared with neon's spectrum. The molecular nitrogen ion line of 391.4 nm is observed. It reveals that Penning ionization between high energy neon excited states and the inevitable gas impurities plays an important role in the value of the αcoefficient.展开更多
The dielectric barrier discharge characteristics in helium at atmospheric pressure are simulated based on a one- dimensional fluid model. Under some discharge conditions, the results show that one discharge pulse per ...The dielectric barrier discharge characteristics in helium at atmospheric pressure are simulated based on a one- dimensional fluid model. Under some discharge conditions, the results show that one discharge pulse per half voltage cycle usually appears when the amplitude of external voltage is low, while a glow-like discharge occurs at high voltage. For the one discharge pulse per half voltage cycle, the maximum of electron density appears near the anode at the beginning of the discharge, which corresponds to a Townsend discharge mode. The maxima of the electron density and the intensity of electric field appear in the vicinity of the cathode when the discharge current increases to some extent, which indicates the formation of a cathode-fall region. Therefore, the discharge has a transition from the Townsend mode to the glow discharge mode during one discharge pulse, which is consistent with previous experimental results.展开更多
The Townsend discharge mechanism has been explored in a planar microelectronic gas discharge device （MGDD） with different applied voltages U and interelectrode distance d under various pressures in air. The anode an...The Townsend discharge mechanism has been explored in a planar microelectronic gas discharge device （MGDD） with different applied voltages U and interelectrode distance d under various pressures in air. The anode and the cathode of the MGDD are formed by a transparent SnO2 covered glass and a GaAs semiconductor, respectively. In the experiments, the discharge is found to be unstable just below the breakdown voltage Ub, whereas the discharge passes through a homo- geneous stable Townsend mode beyond the breakdown voltage. The measurements are made by an electrical circuit and a CCD camera by recording the currents and light emission （LE） intensities. The intensity profiles, which are converted from the 3D light emission images along the semiconductor diameter, have been analysed for different system parameters. Dif- ferent instantaneous conductivity ~t regimes are found below and beyond the Townsend region. These regimes govern the current and spatio-temporal LE stabilities in the plasma system. It has been proven that the stable LE region increases up to 550 Torr as a function of pressure for small d. If the active area of the semiconductor becomes larger and the interlectrode distance d becomes smaller, the stable LE region stays nearly constant with pressure.展开更多
Prediction models were proposed to estimate the reduced Townsend ionization coefficient and ionization cross-section.A shape function of the reduced Townsend ionization coefficient curves was derived from the ionizati...Prediction models were proposed to estimate the reduced Townsend ionization coefficient and ionization cross-section.A shape function of the reduced Townsend ionization coefficient curves was derived from the ionization collision probability model.The function had three parameters:the first ionization potential energy,A_(α),and B_(α).A_(α)and B_(α)were related to the molecule symmetry and size.The polarization of molecules could characterize the molecule symmetry.The multi-layer molecular cross-section(MMCS)was proposed to describe the contributions of electrons and molecule radius on different molecule surfaces to collisions.A prediction model of the ionization cross-section was also proposed based on Aα.The molecule parameters were calculated by the Becke3–Lee–Yang–Parr(B3LYP)method and the 6–311G**basis set.We used available data of 30 and 23 gases,respectively,to build the prediction models of reduced Townsend ionization coefficients and ionization cross-sections.The relationships between the molecular parameters Aαand Bαand the ionization cross-section were built up via nonlinear fittings.The determination coefficients R^(2)of Aα,Bα,and the ionization cross-section were 0.877,0.887,and 0.838,respectively.The results showed that the accuracy of models was positively correlated with the molecule symmetry and reduced electric field.This was mainly related to the accuracy of the MMCS model in predicting Aα.The MMCS model needed to be improved to describe the collision direction selectivity caused by the molecule asymmetry.Under a high reduced electric field,that error of Aαhad less influence on the prediction results.However,the prediction results for single atoms with high symmetry were poor.This may be due to the absolute error of the model close to single atoms’reduced Townsend ionization coefficients.The models could provide the basis for gas insulation prediction and discharge calculations,especially for symmetric molecules under a high electric field.展开更多
We present here an investigation of the self-pulsing phenomenon of negative corona and parallel-plate discharge in argon within one frame of a one-dimensional fluid model in cylinder–cylinder electrode geometry.The t...We present here an investigation of the self-pulsing phenomenon of negative corona and parallel-plate discharge in argon within one frame of a one-dimensional fluid model in cylinder–cylinder electrode geometry.The transition from corona to parallel-plate discharge is obtained by changing the inner and outer radii of the electrodes.The model reproduces the self-pulsing waveform well and provides the spatiotemporal behaviors of the charged particles and electric field during the pulse.The self-pulsing shows a common feature that occurs in various configurations and that does not depend on a specific electrode structure.The self-pulsing is the transformation between a weak-current Townsend mode and a large-current normal glow mode.The behavior of the positive ions is the dominant factor in the formation of the pulse.展开更多
This paper describes the realization of a homogeneous dielectric barrier discharge(DBD)in argon at atmospheric pressure.The effect of the morphology of the dielectric surface(especially the dielectric surface covered ...This paper describes the realization of a homogeneous dielectric barrier discharge(DBD)in argon at atmospheric pressure.The effect of the morphology of the dielectric surface(especially the dielectric surface covered by hollow ceramic beads(99%Al_(2)O_(3))with different diameters)on discharge is investigated.With different dielectrics,the argon DBD presents two discharge modes:a filamentary mode and a homogeneous mode.Fast photography shows that the filamentary mode operates in a streamer discharge,and the homogeneous mode operates in a Townsend discharge regime.It is found that a homogeneous discharge can be generated within a certain voltage range.The voltage amplitude range decreases,and the breakdown voltage increases with the increase in the mean diameter of the ceramic beads.Waveforms of the total current and optical emission signal present stochastic pulses per half voltage cycle for the filamentary mode,whereas there is one single hump per half voltage cycle for the homogeneous mode.In the homogeneous mode,the intensity of the optical emission decreases with the mean diameter of the ceramic beads.The optical emission spectrum is mainly composed of atomic lines of argon and the second positive system of molecular nitrogen.It reveals that the electron density decreases with the increasing mean diameter of the ceramic beads.The vibrational temperature increases with the increasing mean diameter of the ceramic beads.It is believed that a large number of microdischarges are formed,and smaller ceramic beads have a larger activation surface area and more point discharge.Electrons liberated in the shallow well and electrons generated from microdischarges can increase the secondary electron emission coefficient of the cathode and provide initial electrons for discharge continuously.Therefore,the breakdown electric field is reduced,which contributes to easier generation of homogeneous discharge.This is confirmed by the simulation results.展开更多
基金supported by Postdoctoral Project of Hebei University, National Natural Science Foundation of China (Nos. 11575050, 11875121, 51977057)Hebei Natural Science Fund (Nos. A2017201099, A2020201008)。
文摘Fast photography and optical emission spectroscopy are implemented in a 5 mm neon gap dielectric barrier discharge(DBD) at atmospheric pressure with quartz glass used as the dielectric layer. Results show that it starts with a Townsend discharge and ends at a sub-normal glow discharge in neon DBD. Based on the Townsend discharge, the first ionization coefficient of neon is measured. The measurements are consistent with those at low pressure. Optical emission spectroscopy indicates that the spectra are mainly composed of atomic lines of neon, molecular bands and molecular ion bands originating from inevitable gas impurities(mainly nitrogen).Moreover, spectral lines emitted from atomic neon corresponding to the transitions(2p^5 3p→2p^5 3s) are predominant. Although the second positive system of N_2(C^3Π_u→B^3Π_g) is observed, their intensities are too weak compared with neon's spectrum. The molecular nitrogen ion line of 391.4 nm is observed. It reveals that Penning ionization between high energy neon excited states and the inevitable gas impurities plays an important role in the value of the αcoefficient.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 10805013 and 51077035)the Funds for Distinguished Young Scientists of Hebei University, China (Grant No. A2012201045)+2 种基金the Key Project of Ministry of Education of China (Grant No. 210014)the Natural Science Foundation of Hebei province, China (Grant Nos. A2009000149 and A2011201132)the Outstanding Youth Project of Education Department of China (Grant No. Y2011120)
文摘The dielectric barrier discharge characteristics in helium at atmospheric pressure are simulated based on a one- dimensional fluid model. Under some discharge conditions, the results show that one discharge pulse per half voltage cycle usually appears when the amplitude of external voltage is low, while a glow-like discharge occurs at high voltage. For the one discharge pulse per half voltage cycle, the maximum of electron density appears near the anode at the beginning of the discharge, which corresponds to a Townsend discharge mode. The maxima of the electron density and the intensity of electric field appear in the vicinity of the cathode when the discharge current increases to some extent, which indicates the formation of a cathode-fall region. Therefore, the discharge has a transition from the Townsend mode to the glow discharge mode during one discharge pulse, which is consistent with previous experimental results.
基金Project supported by Gazi University BAP Research Project, Turkey （Grant Nos. 05/2012-47 and 05/2012-72）.
文摘The Townsend discharge mechanism has been explored in a planar microelectronic gas discharge device （MGDD） with different applied voltages U and interelectrode distance d under various pressures in air. The anode and the cathode of the MGDD are formed by a transparent SnO2 covered glass and a GaAs semiconductor, respectively. In the experiments, the discharge is found to be unstable just below the breakdown voltage Ub, whereas the discharge passes through a homo- geneous stable Townsend mode beyond the breakdown voltage. The measurements are made by an electrical circuit and a CCD camera by recording the currents and light emission （LE） intensities. The intensity profiles, which are converted from the 3D light emission images along the semiconductor diameter, have been analysed for different system parameters. Dif- ferent instantaneous conductivity ~t regimes are found below and beyond the Townsend region. These regimes govern the current and spatio-temporal LE stabilities in the plasma system. It has been proven that the stable LE region increases up to 550 Torr as a function of pressure for small d. If the active area of the semiconductor becomes larger and the interlectrode distance d becomes smaller, the stable LE region stays nearly constant with pressure.
基金supported by National Natural Science Foundation of China(No.U1966211)National Key R&D Program of China(No.2021YFB2401400)。
文摘Prediction models were proposed to estimate the reduced Townsend ionization coefficient and ionization cross-section.A shape function of the reduced Townsend ionization coefficient curves was derived from the ionization collision probability model.The function had three parameters:the first ionization potential energy,A_(α),and B_(α).A_(α)and B_(α)were related to the molecule symmetry and size.The polarization of molecules could characterize the molecule symmetry.The multi-layer molecular cross-section(MMCS)was proposed to describe the contributions of electrons and molecule radius on different molecule surfaces to collisions.A prediction model of the ionization cross-section was also proposed based on Aα.The molecule parameters were calculated by the Becke3–Lee–Yang–Parr(B3LYP)method and the 6–311G**basis set.We used available data of 30 and 23 gases,respectively,to build the prediction models of reduced Townsend ionization coefficients and ionization cross-sections.The relationships between the molecular parameters Aαand Bαand the ionization cross-section were built up via nonlinear fittings.The determination coefficients R^(2)of Aα,Bα,and the ionization cross-section were 0.877,0.887,and 0.838,respectively.The results showed that the accuracy of models was positively correlated with the molecule symmetry and reduced electric field.This was mainly related to the accuracy of the MMCS model in predicting Aα.The MMCS model needed to be improved to describe the collision direction selectivity caused by the molecule asymmetry.Under a high reduced electric field,that error of Aαhad less influence on the prediction results.However,the prediction results for single atoms with high symmetry were poor.This may be due to the absolute error of the model close to single atoms’reduced Townsend ionization coefficients.The models could provide the basis for gas insulation prediction and discharge calculations,especially for symmetric molecules under a high electric field.
基金supported in part by the Electrostatic Research Foundation of Liu Shanghe Academicians and Experts Workstation,Beijing Orient Institute of Measurement and Test(No.BOIMTLSHJD20221002)。
文摘We present here an investigation of the self-pulsing phenomenon of negative corona and parallel-plate discharge in argon within one frame of a one-dimensional fluid model in cylinder–cylinder electrode geometry.The transition from corona to parallel-plate discharge is obtained by changing the inner and outer radii of the electrodes.The model reproduces the self-pulsing waveform well and provides the spatiotemporal behaviors of the charged particles and electric field during the pulse.The self-pulsing shows a common feature that occurs in various configurations and that does not depend on a specific electrode structure.The self-pulsing is the transformation between a weak-current Townsend mode and a large-current normal glow mode.The behavior of the positive ions is the dominant factor in the formation of the pulse.
基金supported by National Natural Science Foundation of China(Nos.11875121,51977057,11575050,11875014)the Hebei Province Natural Science Foundation(No.A2022201036)。
文摘This paper describes the realization of a homogeneous dielectric barrier discharge(DBD)in argon at atmospheric pressure.The effect of the morphology of the dielectric surface(especially the dielectric surface covered by hollow ceramic beads(99%Al_(2)O_(3))with different diameters)on discharge is investigated.With different dielectrics,the argon DBD presents two discharge modes:a filamentary mode and a homogeneous mode.Fast photography shows that the filamentary mode operates in a streamer discharge,and the homogeneous mode operates in a Townsend discharge regime.It is found that a homogeneous discharge can be generated within a certain voltage range.The voltage amplitude range decreases,and the breakdown voltage increases with the increase in the mean diameter of the ceramic beads.Waveforms of the total current and optical emission signal present stochastic pulses per half voltage cycle for the filamentary mode,whereas there is one single hump per half voltage cycle for the homogeneous mode.In the homogeneous mode,the intensity of the optical emission decreases with the mean diameter of the ceramic beads.The optical emission spectrum is mainly composed of atomic lines of argon and the second positive system of molecular nitrogen.It reveals that the electron density decreases with the increasing mean diameter of the ceramic beads.The vibrational temperature increases with the increasing mean diameter of the ceramic beads.It is believed that a large number of microdischarges are formed,and smaller ceramic beads have a larger activation surface area and more point discharge.Electrons liberated in the shallow well and electrons generated from microdischarges can increase the secondary electron emission coefficient of the cathode and provide initial electrons for discharge continuously.Therefore,the breakdown electric field is reduced,which contributes to easier generation of homogeneous discharge.This is confirmed by the simulation results.
