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Problems and Strategies in Applications of Advanced Process Control in China
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作者 Luo Xionglin Zuo Xin 《Petroleum Science》 SCIE CAS CSCD 2005年第3期44-49,共6页
Advanced Process Control (APC) is necessary for oil refining and chemical process in China, but some problems have emerged in the application of APC techniques in this field. This paper discusses the conditions of A... Advanced Process Control (APC) is necessary for oil refining and chemical process in China, but some problems have emerged in the application of APC techniques in this field. This paper discusses the conditions of APC application concerning process design, distributed control system (DCS) choice and regular control. It analyzes the problems and strategies in APC application. Some suggestions are proposed for the enterprise to benefit from APC application. 展开更多
关键词 China petrochemical process advanced process control application PROBLEM STRATEGY
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Mass Transfer-Promoted Fe^(2+)/Fe^(3+)Circulation Steered by 3D Flow-Through Co-Catalyst System Toward Sustainable Advanced Oxidation Processes
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作者 Weiyang Lv Hao Li +6 位作者 Jinhui Wang Lixin Wang Zenglong Wu Yuge Wang Wenkai Song Wenkai Cheng Yuyuan Yao 《Engineering》 SCIE EI CAS CSCD 2024年第5期264-275,共12页
Realizing fast and continuous generation of reactive oxygen species(ROSs)via iron-based advanced oxidation processes(AOPs)is significant in the environmental and biological fields.However,current AOPs assisted by co-c... Realizing fast and continuous generation of reactive oxygen species(ROSs)via iron-based advanced oxidation processes(AOPs)is significant in the environmental and biological fields.However,current AOPs assisted by co-catalysts still suffer from the poor mass/electron transfer and non-durable promotion effect,giving rise to the sluggish Fe^(2+)/Fe^(3+)cycle and low dynamic concentration of Fe^(2+)for ROS production.Herein,we present a three-dimensional(3D)macroscale co-catalyst functionalized with molybdenum disulfide(MoS_(2))to achieve ultra-efficient Fe^(2+)regeneration(equilibrium Fe^(2+)ratio of 82.4%)and remarkable stability(more than 20 cycles)via a circulating flow-through process.Unlike the conventional batch-type reactor,experiments and computational fluid dynamics simulations demonstrate that the optimal utilization of the 3D active area under the flow-through mode,initiated by the convectionenhanced mass/charge transfer for Fe^(2+)reduction and then strengthened by MoS_(2)-induced flow rotation for sufficient reactant mixing,is crucial for oxidant activation and subsequent ROS generation.Strikingly,the flow-through co-catalytic system with superwetting capabilities can even tackle the intricate oily wastewater stabilized by different surfactants without the loss of pollutant degradation efficiency.Our findings highlight an innovative co-catalyst system design to expand the applicability of AOPs based technology,especially in large-scale complex wastewater treatment. 展开更多
关键词 advanced oxidation processes 3D co-catalyst Flow-through mode Enhanced mass transfer Complex wastewater treatment
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UV-Based Advanced Oxidation Processes for Antibiotic Resistance Control: Efficiency, Influencing Factors, and Energy Consumption
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作者 Jiarui Han Wanxin Li +5 位作者 Yun Yang Xuanwei Zhang Siyu Bao Xiangru Zhang Tong Zhang Kenneth Mei Yee Leung 《Engineering》 SCIE EI CAS CSCD 2024年第6期27-39,共13页
Antibiotic resistant bacteria(ARB)with antibiotic resistance genes(ARGs)can reduce or eliminate the effectiveness of antibiotics and thus threaten human health.The United Nations Environment Programme considers antibi... Antibiotic resistant bacteria(ARB)with antibiotic resistance genes(ARGs)can reduce or eliminate the effectiveness of antibiotics and thus threaten human health.The United Nations Environment Programme considers antibiotic resistance the first of six emerging issues of concern.Advanced oxidation processes(AOPs)that combine ultraviolet(UV)irradiation and chemical oxidation(primarily chlorine,hydrogen peroxide,and persulfate)have attracted increasing interest as advanced water and wastewater treatment technologies.These integrated technologies have been reported to significantly elevate the efficiencies of ARB inactivation and ARG degradation compared with direct UV irradiation or chemical oxidation alone due to the generation of multiple reactive species.In this study,the performance and underlying mechanisms of UV/chlorine,UV/hydrogen peroxide,and UV/persulfate processes for controlling ARB and ARGs were reviewed based on recent studies.Factors affecting the process-specific efficiency in controlling ARB and ARGs were discussed,including biotic factors,oxidant dose,UV fluence,pH,and water matrix properties.In addition,the cost-effectiveness of the UV-based AOPs was evaluated using the concept of electrical energy per order.The UV/chlorine process exhibited a higher efficiency with lower energy consumption than other UV-based AOPs in the wastewater matrix,indicating its potential for ARB inactivation and ARG degradation in wastewater treatment.Further studies are required to address the trade-off between toxic byproduct formation and the energy efficiency of the UV/chlorine process in real wastewater to facilitate its optimization and application in the control of ARB and ARGs. 展开更多
关键词 advanced oxidation processes Ultraviolet/chlorine Ultraviolet/hydrogen peroxide Ultraviolet/persulfate Antibiotic resistant bacteria Antibiotic resistance genes
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Advanced Process and Electron Device Technology 被引量:1
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作者 Dan Zhang Xiaojing Su +21 位作者 Hao Chang Hao Xu Xiaolei Wang Xiaobin He Junjie Li Fei Zhao Qide Yao Yanna Luo Xueli Ma Hong Yang Yongliang Li Zhenhua Wu Yajuan Su Tao Yang Yayi Wei Anyan Du Huilong Zhu Junfeng Li Huaxiang Yin Jun Luo Tianchun Ye Wenwu Wang 《Tsinghua Science and Technology》 SCIE EI CAS CSCD 2022年第3期534-558,共25页
This article reviews advanced process and electron device technology of integrated circuits,including recent featuring progress and potential solutions for future development.In 5 years,for pushing the performance of ... This article reviews advanced process and electron device technology of integrated circuits,including recent featuring progress and potential solutions for future development.In 5 years,for pushing the performance of fin field-effect transistors(FinFET)to its limitations,several processes and device boosters are provided.Then,the three-dimensional(3 D)integration schemes with alternative materials and device architectures will pave paths for future technology evolution.Finally,it could be concluded that Moore’s law will undoubtedly continue in the next 15 years. 展开更多
关键词 advanced process gate-all-around devices three-dimensional(3D)integration high-mobility channel integrated circuits
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Application of advanced oxidation processes for removing salicylic acid from synthetic wastewaters 被引量:7
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作者 Djalma Ribeiro da Silva Carlos A.Martinez-Huítle 《Chinese Chemical Letters》 SCIE CAS CSCD 2010年第1期101-104,共4页
In this study,advanced oxidation processes(AOPs) such as anodic oxidation(AO),UV/H_2O_2 and Fenton processes(FP) were investigated for the degradation of salicylic acid(SA) in lab-scale experiments.Boron-doped diamond... In this study,advanced oxidation processes(AOPs) such as anodic oxidation(AO),UV/H_2O_2 and Fenton processes(FP) were investigated for the degradation of salicylic acid(SA) in lab-scale experiments.Boron-doped diamond(BDD) film electrodes using Ta as substrates were employed for AO of SA.In the case of FP and UV/H_2O_2,most favorable experimental conditions were determined for each process and these were used for comparing with AO process.The study showed that the FP was the most effective process under aci... 展开更多
关键词 advanced oxidation processes Salicylic acid(SA) Anodic oxidation Ta/BDD Electrocatalytic activity
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Chemical oxygen demand reduction in coffee wastewater through chemical flocculation and advanced oxidation processes 被引量:7
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作者 ZAYAS Pérez Teresa GEISSLER Gunther HERNANDEZ Fernando 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2007年第3期300-305,共6页
The removal of the natural organic matter present in coffee processing wastewater through chemical coagulation-flocculation and advanced oxidation processes (AOP) had been studied. The effectiveness of the removal o... The removal of the natural organic matter present in coffee processing wastewater through chemical coagulation-flocculation and advanced oxidation processes (AOP) had been studied. The effectiveness of the removal of natural organic matter using commercial flocculants and UV/H202, UV/O3 and UV/H2O2/O3 processes was determined under acidic conditions. For each of these processes, different operational conditions were explored to optimize the treatment efficiency of the coffee wastewater. Coffee wastewater is characterized by a high chemical oxygen demand (COD) and low total suspended solids. The outcomes of coffee wastewater treatment using coagulation-flocculation and photodegradation processes were assessed in terms of reduction of COD, color, and turbidity. It was found that a reduction in COD of 67% could be realized when the coffee wastewater was treated by chemical coagulation-flocculation with lime and coagulant T-1. When coffee wastewater was treated by coagulation-flocculation in combination with UV/H2O2, a COD reduction of 86% was achieved, although only after prolonged UV irradiation. Of the three advanced oxidation processes considered, UV/H2O2, UV/O3 and UV/H2O2/O3, we found that the treatment with UV/H2O2/O3 was the most effective, with an efficiency of color, turbidity and further COD removal of 87%, when applied to the flocculated coffee wastewater. 展开更多
关键词 advanced oxidation processes coagulation-flocculation: coffee wastewater chemical oxygen demand (COD)
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Degradation of Organic Pollutants by the Advanced Oxidation Processes 被引量:3
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作者 钟理 郭江海 +2 位作者 吕扬效 李小莹 高桂田 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 1999年第2期110-115,共6页
A kinetic model has been developed for the degradation of organic pollutants concerning with hydroperoxide ion as the initial step for generation of hydroxyl radical and its subsequent reaction mechanisms. Rate equati... A kinetic model has been developed for the degradation of organic pollutants concerning with hydroperoxide ion as the initial step for generation of hydroxyl radical and its subsequent reaction mechanisms. Rate equations were derived for depletion of ozone and pollutants in the peroxone oxidation process using ozone and hydrogen peroxide as combined oxidants. Kinetic data obtained experimentally from the hydrogen peroxide-ozone reaction and peroxone oxidation of nitrobenzene were analyzed by using the proposed rate equations. 展开更多
关键词 OXIDATION POLLUTANTS advanced oxidation processes
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Application of Spectral Angle Mapper Classification to Discriminate Hydrothermal Alteration in Southwest Birjand, Iran, Using Advanced Spaceborne Thermal Emission and Reflection Radiometer Image Processing 被引量:5
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作者 Maryam ABDI Mohammd H. KARIMPOUR 《Acta Geologica Sinica(English Edition)》 SCIE CAS CSCD 2012年第5期1289-1296,共8页
The purpose of this study is to evaluate the Spectral Angle Mapper (SAM) classification method for determining the optimum threshold (maximum spectral angle) to unveil the hydrothermal mineral assemblages related ... The purpose of this study is to evaluate the Spectral Angle Mapper (SAM) classification method for determining the optimum threshold (maximum spectral angle) to unveil the hydrothermal mineral assemblages related to mineral deposits. The study area indicates good potential for Cu-Au porphyry, epithermal gold deposits and hydrothermal alteration well developed in arid and semiarid climates, which makes this region significant for Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) image processing analysis. Given that achieving an acceptable mineral mapping requires knowing the alteration patterns, petrochemistry and petrogenesis of the igneous rocks while considering the effect of weathering, overprinting of supergene alteration, overprinting of hypogene alteration and host rock spectral mixing, SAM classification was implemented for argillic, sericitic, propylitic, alunitization, silicification and iron oxide zones of six previously known mineral deposits: Maherabad, a Cu-Au porphyry system; Sheikhabad, an upper part of Cu-Au porphyry system; Khoonik, an Intrusion related Au system; Barmazid, a low sulfidation epithermal system; Khopik, a Cu-Au porphyry system; and Hanish, an epithermal Au system. Thus, the investigation showed that although the whole alteration zones are affected by mixing, it is also possible to produce a favorable hydrothermal mineral map by such complementary data as petrology, petrochemistry and alteration patterns. 展开更多
关键词 hydrothermal alteration Spectral Angle Mapper advanced Spaceborne Thermal Emission and Reflection Radiometer image process Iran
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The Inception of Jungian Advanced Motor Processing (JAMP) —A 21st Century Approach to Treating Trauma 被引量:1
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作者 Lahab Al-Samarrai 《Journal of Behavioral and Brain Science》 2022年第4期116-130,共15页
Jungian Advanced Motor Processing (JAMP) is a mode of treatment developed in May of 2020 by Dr. Lahab Al-Samarrai during the COVID-19 pandemic. Dr. Al-Samarrai had many students who reported increased anxiety, negativ... Jungian Advanced Motor Processing (JAMP) is a mode of treatment developed in May of 2020 by Dr. Lahab Al-Samarrai during the COVID-19 pandemic. Dr. Al-Samarrai had many students who reported increased anxiety, negative thoughts, fearful thoughts, and self-defeating thoughts. These students needed symptom relief more quickly than conventional talk therapy typically provides. Dr. Al-Samarrai developed a treatment modality incorporating light, bilateral audible beats, and positive affirmations. So far, more than 100 subjects have undergone JAMP, and this paper is a case study of one such subject. The research currently being compiled on JAMP, the subject of a future paper, to date shows positive improvement after receiving 5 - 6 sessions, and demonstrated decreases in both somatic symptoms and post-traumatic symptoms ranging from 45 - 55 percent. This paper will share the following: 1) Description of the underlying theoretical components supporting the treatment;2) Description of the treatment;3) Discussion of the case of Grace and her experience with JAMP. 展开更多
关键词 Jungian advanced Motor processing TRAUMA Treatment
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The First Pacific Rim International Conference on Advanced Materials and Processing 被引量:1
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作者 Hangzhou China, 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 1993年第1期77-78,共2页
The First Pacific Rim International Confer-ence on Advanced Materials and Processing(PRICM-1)organized by The Chinese Society ofMetals(CSM),and co-sponsored by the Japan In-stitute of Metals(JIM),the Korean Institute ... The First Pacific Rim International Confer-ence on Advanced Materials and Processing(PRICM-1)organized by The Chinese Society ofMetals(CSM),and co-sponsored by the Japan In-stitute of Metals(JIM),the Korean Institute ofMetals(KIM)and The Mineral,Metals & Materi-als Society of the United States(TMS),was held inShangri-La Hotel,Hangzhou,China on June24-27,1992.It was the first large international conference 展开更多
关键词 The First Pacific Rim International Conference on advanced Materials and processing
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Acid precipitation coupled membrane-dispersion advanced oxidation process(MAOP)to treat crystallization mother liquor of pulp wastewater
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作者 Rongzong Li Zhaoyang Li +3 位作者 Qian Jiang Zhaoxiang Zhong Ming Zhou Weihong Xing 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2020年第7期1911-1917,共7页
Treatment to crystallization mother liquor containing high concentration of organic and inorganic substances is a challenge in zero liquid discharge of industrial wastewater.Acid precipitation coupled membrane-dispers... Treatment to crystallization mother liquor containing high concentration of organic and inorganic substances is a challenge in zero liquid discharge of industrial wastewater.Acid precipitation coupled membrane-dispersion advanced oxidation process(MAOP)was proposed for organics degradation before salt crystallization by evaporation.With acid-MAOP treatment CODCrin mother liquor of pulping wastewater was eliminated by 55.2%from ultrahigh initial concentration up to 12,500 mg·L^-1.The decolorization rate was 96.5%.Recovered salt was mainly NaCl(83.3 wt%)having whiteness 50 brighter than industrial baysalt of whiteness 45.The oxidation conditions were optimized as CO3=0.11 g·L^-1 and CH2O2=2.0 g·L^-1 with dispersing rate 0.53 ml·min^-1 for 100 min reaction toward acidified liquor of p H=2.Acidification has notably improved evaporation efficiency during crystallization.Addition of H2O2 made through membrane dispersion has eliminated hydroxyl radical"quench effect"and enhanced the degradation capacity,in particular,the breakage of carbon-chloride bonds(of both aliphatic and aromatic).As a result,the proposed coupling method has improved organic pollutant reduction so as the purity of salt from the wastewater mixture which can facilitate water and salt recycling in industry. 展开更多
关键词 advanced oxidation process Crystallization mother liquor Ceramic membrane dispersion Pulping wastewater
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Advanced oxidation processes of decomposing dichloroacetic acid and trichloroacetic acid in water
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作者 汪昆平 JUNJI Hirotsuji 《Journal of Chongqing University》 CAS 2008年第3期171-178,共8页
We studied the decomposition of two haloacetic acids (HAAs),dichloroacetic acid (DCAA) and trichloroacetic acid (TCAA),in water by single oxidants ozone (O3) and ultraviolet radiation (UV) and the advanced oxidation p... We studied the decomposition of two haloacetic acids (HAAs),dichloroacetic acid (DCAA) and trichloroacetic acid (TCAA),in water by single oxidants ozone (O3) and ultraviolet radiation (UV) and the advanced oxidation processes (AOPs) constituted by the combinations of O3/UV,H2O2/UV,O3 /H2O2,and O3/H2O2/UV. The concentrations of HAAs were analyzed at specified time intervals to track their decomposition. Except for O3 and UV,the four combined oxidation processes remarkably enhance the decomposition of DCAA and TCAA owing to the generated very reactive hydroxyl radicals. The fastest decomposition process is O3/H2O2/UV,closely followed by O3/UV. DCAA is much easier to decompose than TCAA. The kinetics of HAA decomposition by O3/UV can be described well by a pseudo first-order reaction model under a constant initial dissolved O3 concentration and fixed UV radiation. Humic acids and HCO3-in the reaction system both decrease the decomposition rate constants for DCAA and TCAA. The amount of H2O2 accumulates in the presence of humic acids in the O3/UV process. 展开更多
关键词 OZONIZATION ultraviolet radiation OZONE advanced oxidation process haloacetic acid
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Preliminary Announcement for the 1st Pacific Rim International Conference on Advanced Materials and Processing(PRICM-1)
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《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 1990年第5期378-378,共1页
The Joint Conference Organizing Committee of The Chinese Society of Metals(CSM),The Japan Insti-tute of Metals(JIM),The Korean Institute of Metals(KIM)and The Minerals,Metals & Materials Society(TMS)announces The ... The Joint Conference Organizing Committee of The Chinese Society of Metals(CSM),The Japan Insti-tute of Metals(JIM),The Korean Institute of Metals(KIM)and The Minerals,Metals & Materials Society(TMS)announces The First Pacific Rim International Conference on Advanced Materials and Processing(PRICM-1)which will be held in Hangzhou,China,in the last week of June,1992 lasting about four days.It is agreed that the PRICM-1 will be organized by The Chinese Society of Metals. 展开更多
关键词 Co PRICM-1 Preliminary Announcement for the 1st Pacific Rim International Conference on advanced Materials and processing
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Effects of Advanced Oxidation Processes on the Decomposition Properties of Organic Compounds with Different Molecular Structures in Water
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作者 Harufumi Suzuki Shoichi Yamagiwa +1 位作者 Sadao Araki Hideki Yamamoto 《Journal of Water Resource and Protection》 2016年第9期823-834,共13页
Studies to decompose persistent organic pollutants in wastewater from chemical factories by using Advanced Oxidation Processes (AOPs) have recently been performed. Oxidation reactions involving ozone and &bull;OH ... Studies to decompose persistent organic pollutants in wastewater from chemical factories by using Advanced Oxidation Processes (AOPs) have recently been performed. Oxidation reactions involving ozone and &bull;OH radicals and cleavage caused by UV are the main decomposition reactions that occur in AOPs using ozone and UV. The mechanisms through which organic compounds are decomposed in AOPs are complicated and difficult to understand because various decomposition reactions occur simultaneously. The Total Organic Carbon (TOC) removal efficiencies achieved in several different AOPs were evaluated in this study. The TOC removal efficiencies were different for organic compounds with different chemical structures. The TOC was more effectively removed when aromatic compounds were treated using the O<sub>3</sub>-UV-TiO<sub>2</sub> process than when using the other AOPs, and the TOC was removed more effectively by the O<sub>3</sub>-UV process than by the UV-TiO<sub>2</sub> process. However, the TOC was removed more effectively when open-chain compounds were treated using the UV-TiO<sub>2</sub> process than using the O<sub>3</sub>-UV process, and the UV-TiO<sub>2</sub> and O<sub>3</sub>-UV-TiO<sub>2</sub> processes resulted in similar TOC removal efficiencies. Therefore, it is necessary to use the O<sub>3</sub>-UV-TiO<sub>2</sub> process to decompose aromatic compounds as quickly as possible. On the other hand, the UV-TiO<sub>2</sub> process degraded the open-chain compounds most effectively, and the O<sub>3</sub>-UV-TiO<sub>2</sub> process did not need to decompose open-chain compounds. Moreover, the TOC of aromatic compounds was removed more slowly than that of open-chain compounds. The TOC removal efficiency increased with decreasing the number of carbon atoms in the molecule. The TOC removal efficiencies increased in order of the organic compounds containing methyl groups, aldehyde groups and carboxyl groups. The removal of the TOC when organic compounds were treated using the O<sub>3</sub>-UV-TiO<sub>2</sub> process followed pseudo-zero-order kinetics. 展开更多
关键词 advanced Oxidation process OZONE Hydroxyl Radical Decomposition Efficiency Water Treatment
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South China University of fechnology Advanced Metallic Materials Research and Processing Technology Center
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《China Foundry》 SCIE CAS 2004年第S1期67-67,共1页
A dvanced Metallic Materials Research and Processing Technology Center was found in December 1998. As a unit under The College of Mechanical Engineering, the Center is an expansion of the former Cast and Composite Mat... A dvanced Metallic Materials Research and Processing Technology Center was found in December 1998. As a unit under The College of Mechanical Engineering, the Center is an expansion of the former Cast and Composite Materials Research Group, which was found in the early eighties of last century. The Center is focusing in the basic and applied research, and development of advanced metallic materials and their processing technology. It also functions as an organization 展开更多
关键词 South China University of fechnology advanced Metallic Materials Research and processing Technology Center HIGH
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Advances of embedded resistive random access memory in industrial manufacturing and its potential applications
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作者 Zijian Wang Yixian Song +7 位作者 Guobin Zhang Qi Luo Kai Xu Dawei Gao Bin Yu Desmond Loke Shuai Zhong Yishu Zhang 《International Journal of Extreme Manufacturing》 SCIE EI CAS CSCD 2024年第3期175-214,共40页
Embedded memory,which heavily relies on the manufacturing process,has been widely adopted in various industrial applications.As the field of embedded memory continues to evolve,innovative strategies are emerging to en... Embedded memory,which heavily relies on the manufacturing process,has been widely adopted in various industrial applications.As the field of embedded memory continues to evolve,innovative strategies are emerging to enhance performance.Among them,resistive random access memory(RRAM)has gained significant attention due to its numerousadvantages over traditional memory devices,including high speed(<1 ns),high density(4 F^(2)·n^(-1)),high scalability(~nm),and low power consumption(~pJ).This review focuses on the recent progress of embedded RRAM in industrial manufacturing and its potentialapplications.It provides a brief introduction to the concepts and advantages of RRAM,discusses the key factors that impact its industrial manufacturing,and presents the commercial progress driven by cutting-edge nanotechnology,which has been pursued by manysemiconductor giants.Additionally,it highlights the adoption of embedded RRAM in emerging applications within the realm of the Internet of Things and future intelligent computing,with a particular emphasis on its role in neuromorphic computing.Finally,the review discusses thecurrent challenges and provides insights into the prospects of embedded RRAM in the era of big data and artificial intelligence. 展开更多
关键词 embedded resistive random access memory industrial manufacturing intelligent computing advanced process node
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Review of advanced oxidation processes for treating hospital sewage to achieve decontamination and disinfection 被引量:2
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作者 Si-Ying Yu Zhi-Hui Xie +9 位作者 Xiaoyu Wu Yun-Zhe Zheng Yang Shi Zhao-Kun Xiong Peng Zhou Yang Liu Chuan-Shu He Zhi-Cheng Pan Kai-Jun Wang Bo Lai 《Chinese Chemical Letters》 SCIE CAS CSCD 2024年第1期140-152,共13页
Hospital sewage contains various harmful pharmaceutical contaminants(e.g.,antibiotics,anti-inflammatory agents,and painkillers)and pathogens(e.g.,bacteria,viruses,and parasites),whose direct discharge into the environ... Hospital sewage contains various harmful pharmaceutical contaminants(e.g.,antibiotics,anti-inflammatory agents,and painkillers)and pathogens(e.g.,bacteria,viruses,and parasites),whose direct discharge into the environment will induce diseases and pose a powerful threat to human health and safety,and environmental ecology.In recent years,advanced oxidation processes(AOPs),particularly photocatalysis,electrocatalysis,and ozone catalysis have been developed as widespread and effective techniques for hospital sewage treatments.However,there is a lack of systematic comparison and review of the prior studies on hospital sewage treatment using AOPs systems.This review elaborates on the mechanisms,removal efficiencies,and advantages/disadvantages of these AOPs systems for hospital wastewater decontamination and disinfection.Meanwhile,some novel and potential technologies such as photo-electrocatalysis,electro-peroxone,Fenton/Fenton-like,and piezoelectric catalysis are also included and summarized.Moreover,we further summarize and compare the capacity of these AOPs to treat the actual hospital wastewater under the impact of the water matrix and pH,and estimate the economic cost of these technologies for practical application.Finally,the future development directions of AOPs for hospital wastewater decontamination and disinfection have been prospected.Overall,this study provides a comparison and overview of these AOP systems in an attempt to raise extensive concerns about hospital wastewater decontamination and disinfection technologies and guide researchers to discover the future directions of technologies optimization,which would be a crucial step forward in the field of hospital sewage treatment. 展开更多
关键词 Hospital sewage treatment advanced oxidation processes Pharmaceutical contaminants DISINFECTION DECONTAMINATION
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Flue gas analysis for biomass and coal co‑fring in fuidized bed:process simulation and validation 被引量:2
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作者 Daulet Zhakupov Lyazzat Kulmukanova +1 位作者 Yerbol Sarbassov Dhawal Shah 《International Journal of Coal Science & Technology》 EI CAS CSCD 2022年第4期71-81,共11页
Coal-conversion technologies,although used ubiquitously,are often discredited due to high pollutant emissions,thereby emphasizing a dire need to optimize the combustion process.The co-fring of coal/biomass in a fuidiz... Coal-conversion technologies,although used ubiquitously,are often discredited due to high pollutant emissions,thereby emphasizing a dire need to optimize the combustion process.The co-fring of coal/biomass in a fuidized bed reactor has been an efcient way to optimize the pollutants emission.Herein,a new model has been designed in Aspen Plus®to simultaneously include detailed reaction kinetics,volatile compositions,tar combustion,and hydrodynamics of the reactor.Validation of the process model was done with variations in the fuel including high-sulfur Spanish lignite,high-ash Ekibastuz coal,wood pellets,and locally collected municipal solid waste(MSW)and the temperature ranging from 1073 to 1223 K.The composition of the exhaust gases,namely,CO/CO_(2)/NO/SO_(2)were determined from the model to be within 2%of the experimental observations.Co-combustion of local MSW with Ekibastuz coal had fue gas composition ranging from 1000 to 5000 ppm of CO,16.2%–17.2%of CO_(2),200–550 ppm of NO,and 130–210 ppm of SO_(2).A sensitivity analysis on co-fring of local biomass and Ekibastuz coal demonstrated the optimal operating temperature for fuidized bed reactor at 1148 K with the recommended biomass-to-coal ratio is 1/4,leading to minimum emissions of CO,NO,and SO_(2). 展开更多
关键词 Biomass cofring Fluidized-bed combustion advanced process simulation Flue-gas emissions Fuel utilization Aspen plus
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Fabrication of pollution-free coal gangue-based catalytic material utilizing ferrous chloride as activator for efficient peroxymonosulfate activation
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作者 Zhiming Sun Xinlin Wang +3 位作者 Shaoran Jia Jialin Liang Xiaotian Ning Chunquan Li 《International Journal of Coal Science & Technology》 EI CAS CSCD 2024年第1期103-118,共16页
Novel coal gangue-based persulfate catalyst(CG-FeCl_(2))was successfully synthesized by the means of calcinating under nitrogen atmosphere with the addition of ferrous chloride tetrahydrate(FeCl_(2)·_(4)H_(2)O).T... Novel coal gangue-based persulfate catalyst(CG-FeCl_(2))was successfully synthesized by the means of calcinating under nitrogen atmosphere with the addition of ferrous chloride tetrahydrate(FeCl_(2)·_(4)H_(2)O).The phase transformation of the prepared materials and gas products during the heating process are thoroughly investigated.It is suggested that ferrous chloride participated in the phase transformation and formed Si-O-Fe bonds.And the main gaseous products are H_(2)O,H_(2),and HCl during the heating process.Besides,the ability of CG-FeCl_(2) to activate peroxymonosulfate(PMS)for catalytic degradation of polycyclic aromatic hydrocarbons(PAHs)and phenol was deeply studied.More than 95%of naphthyl,phenanthrene and phenol were removed under optimizied conditions.In addition,1O_(2),·OH,and SO_(4)·−were involved in the CG-FeCl_(2)/PMS system from the free radical scavenging experiment,where 1O_(2) played a major role during the oxidation process.Furthermore,CG-FeCl_(2)/PMS system exhibited superior stability in a relatively wide pH range and the presence of common anion from related degradation experiments.Overall,the novel CG-FeCl_(2) is an efficient and environmentally friendly catalyst,displaying potential application prospect in the field of PAHs and phenol-contaminated wastewater treatment. 展开更多
关键词 Coal gangue Persulfate activation advanced oxidation processes Polycyclic aromatic hydrocarbons Phenol Ferrous chloride
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Simultaneous Degradation, Dehalogenation, and Detoxification of Halogenated Antibiotics by Carbon Dioxide Radical Anions
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作者 Yanzhou Ding Xia Yu +8 位作者 Shuguang Lyu Huajun Zhen Wentao Zhao Cheng Peng Jiaxi Wang Yiwen Zhu Chengfei Zhu Lei Zhou Qian Sui 《Engineering》 SCIE EI CAS CSCD 2024年第6期78-86,共9页
Despite the extensive application of advanced oxidation processes(AOPs)in water treatment,the efficiency of AOPs in eliminating various emerging contaminants such as halogenated antibiotics is constrained by a number ... Despite the extensive application of advanced oxidation processes(AOPs)in water treatment,the efficiency of AOPs in eliminating various emerging contaminants such as halogenated antibiotics is constrained by a number of factors.Halogen moieties exhibit strong resistance to oxidative radicals,affecting the dehalogenation and detoxification efficiencies.To address these limitations of AOPs,advanced reduction processes(ARPs)have been proposed.Herein,a novel nucleophilic reductant—namely,the carbon dioxide radical anion(CO_(2)^(·-))—is introduced for the simultaneous degradation,dehalogenation,and detoxification of florfenicol(FF),a typical halogenated antibiotic.The results demonstrate that FF is completely eliminated by CO_(2)^(·-),with approximately 100%of Cland 46%of Freleased after 120 min of treatment.Simultaneous detoxification is observed,which exhibits a linear response to the release of free inorganic halogen ions(R^(2)=0.97,p<0.01).The formation of halogen-free products is the primary reason for the superior detoxification performance of this method,in comparison with conventional hydroxyl-radical-based AOPs.Products identification and density functional theory(DFT)calculations reveal the underlying dehalogenation mechanism,in which the chlorine moiety of FF is more susceptible than other moieties to nucleophilic attack by CO_(2)^(·-).Moreover,CO_(2)^(·-)-based ARPs exhibit superior dehalogenation efficiencies(>75%)in degrading a series of halogenated antibiotics,including chloramphenicol(CAP),thiamphenicol(THA),diclofenac(DLF),triclosan(TCS),and ciprofloxacin(CIP).The system shows high tolerance to the pH of the solution and the presence of natural water constituents,and demonstrates an excellent degradation performance in actual groundwater,indicating the strong application potential of CO_(2)^(·-)-based ARPs in real life.Overall,this study elucidates the feasibility of CO_(2)^(·-)for the simultaneous degradation,dehalogenation,and detoxification of halogenated antibiotics and provides a promising method for their regulation during water or wastewater treatment. 展开更多
关键词 Carbon dioxide radical anions advanced reduction processes Halogenated antibiotics DEHALOGENATION DETOXIFICATION
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