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Mechanical Properties of Methane Hydrate-Bearing Interlayered Sediments 被引量:16
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作者 DONG Lin LI Yanlong +5 位作者 LIU Changling LIAO Hualin CHEN Guoqi CHEN Qiang LIU Lele HU Gaowei 《Journal of Ocean University of China》 SCIE CAS CSCD 2019年第6期1344-1350,共7页
The complex distribution of gas hydrate in sediments makes understanding the mechanical properties of hydrate-bearing sediments a challenging task.The mechanical behaviors of hydrate-bearing interlayered sediments are... The complex distribution of gas hydrate in sediments makes understanding the mechanical properties of hydrate-bearing sediments a challenging task.The mechanical behaviors of hydrate-bearing interlayered sediments are still poorly known.A series of triaxial shearing tests were conducted to investigate the strength parameters and deformation properties of methane hydrate-bearing interlayered sediments at the effective pressure of 1 MPa.The results indicate that the stress-strain curves of hydrate-bearing interlayered sediments are significantly different from that of hydrate-bearing sediments.The peak strength,Young's modulus,initial yielding modulus,and failure mode are deeply affected by the methane hydrate distribution.The failure behaviors and mechanism of strain softening and hardening patterns of the interlayered specimens are more complicated than those of the integrated specimens.This study compares the different mechanical behaviors between integrated and interlayered specimens containing gas hydrate,which can serve as a reference for the prediction and analysis of the deformation behaviors of natural gas hydrate reservoirs. 展开更多
关键词 gas HYDRATE interlayered SEDIMENTS MECHANICAL property TRIAXIAL SHEARING tests strength parameters
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Preparation and Microstructure of Al-pillared Interlayered Montmorillonite 被引量:2
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作者 曹明礼 《Journal of Wuhan University of Technology(Materials Science)》 SCIE EI CAS 2002年第4期13-16,共4页
Al-pillared interlayered montmorillonite (Al-PILM) was prepared using the artificial Na-montmorillonite from the Qingfengshan bentonite mine as a starting material mixed with Al-pillaring solutions.The microstructure ... Al-pillared interlayered montmorillonite (Al-PILM) was prepared using the artificial Na-montmorillonite from the Qingfengshan bentonite mine as a starting material mixed with Al-pillaring solutions.The microstructure of the materials was studied by an X-ray powder diffractometer and a Fourier transform infrared (FTIR) spectrometer.The results indicated that the basal spacing [d(001) value] of the materials was increased significantly to 1.9194 nm relative to Na-montmorillonite (1.2182 nm).After calcined for 2 h at 300℃,the basal spacing was stabilized at 1.8394 nm and the layered structure of the materials was not destroyed.Thermal analysis was conducted by a thermal gravimetry and differential thermal analysis (TG-DTA) instrument,it showed that Al-PILM lost physically adsorbed water below 230.6℃ and water formed by dehydroxylation of the pillars at around 497.1℃, with a peak of the phase transformation at 903.0℃. 展开更多
关键词 Al-pillared interlayered montmorillonite pillaring solution PREPARATION MICROSTRUCTURE
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Nacre-inspired MXene-based film for highly sensitive piezoresistive sensing over a broad sensing range 被引量:1
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作者 Gaofeng Wang Lingxian Meng +3 位作者 Xinyi Ji Xuying Liu Jiajie Liang Shuiren Liu 《Bio-Design and Manufacturing》 SCIE EI CAS CSCD 2024年第4期463-475,共13页
As the main component of wearable electronic equipment,flexible pressure sensors have attracted wide attention due to their excellent sensitivity and their promise with respect to applications in health monitoring,ele... As the main component of wearable electronic equipment,flexible pressure sensors have attracted wide attention due to their excellent sensitivity and their promise with respect to applications in health monitoring,electronic skin,and human-computer interactions.However,it remains a significant challenge to achieve epidermal sensing over a wide sensing range,with short response/recovery time and featuring seamless conformability to the skin simultaneously.This is critical since the capture of minute electrophysiological signals is important for health care applications.In this paper,we report the preparation of a nacre-like MXene/sodium carboxymethyl cellulose(CMC)nanocomposite film with a“brick-and-mortar”interior structure using a vacuum-induced self-assembly strategy.The synergistic behavior of the MXene“brick”and flexible CMC“mortar”contributes to attenuating interlamellar self-stacking and creates numerous variable conductive pathways on the sensing film.This resulted in a high sensitivity over a broad pressure range(i.e.,0.03-22.37 kPa:162.13 kPa^(-1);22.37-135.71 kPa:127.88 kPa^(-1);135.71-286.49 kPa:100.58 kPa^(-1)).This sensor also has a low detection limit(0.85 Pa),short response/recovery time(8.58 ms/34.34 ms),and good stability(2000 cycles).Furthermore,we deployed pressure sensors to distinguish among tiny particles,various physiological signals of the human body,space arrays,robot motion monitoring,and other related applications to demonstrate their feasibility for a variety of health and motion monitoring use cases. 展开更多
关键词 Flexible pressure sensor MXene BIOINSPIRED Physiological signals Interlayer spacing
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Evolution mechanism of lamellarαand interlayeredβduring hot compression of TC21 titanium alloy with a widmanst?tten structure 被引量:2
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作者 Xiaoyu ZHENG Ke WANG +2 位作者 Cheng ZHANG Renlong XIN Qing LIU 《Chinese Journal of Aeronautics》 SCIE EI CAS CSCD 2022年第3期475-483,共9页
TC21 titanium alloy,as an important metal to fabricate the aircraft structural components,has attracted great attentions recently.A TC21 titanium alloy with widmanst?tten structure was isothermally compressed.Based on... TC21 titanium alloy,as an important metal to fabricate the aircraft structural components,has attracted great attentions recently.A TC21 titanium alloy with widmanst?tten structure was isothermally compressed.Based on the microstructure observation,the evolution of initialβgrain,Grain Boundaryαphase(α;),lamellar a and interlayeredβwas systematically investigated.The results showed that,with the increasing of height reduction,theα;underwent an evolution process from bending/kinking to breaking inducing the corresponding blurring of initial coarse b grain outline.Meanwhile,a significant phase transformation from a to b took place at the terminations of brokenα;.The evolution of lamellarαand interlayeredβin the colony was closely related to their deformation compatibility.In the a colony,the interlayered b experienced a larger deformation amount than lamellarα.The higher distortion energy promoted the occurrence of Dynamic Recovery(DRV)and Dynamic Recrystallization(DRX)to generate many Low Angle Boundaries(LABs)and High Angle Boundaries(HABs)in interlayered b,which induced an apparent grain refinement of b phase.On the contrary,the lower distortion energy and low deformation temperature suppressed the occurrence of DRV/DRX and restrained the globularization of lamellarα.Furthermore,the microstructure observation clearly revealed that the shearing separation mechanism dominated the evolution of the a phase from lamellar to short bar-like morphology. 展开更多
关键词 Globularization Grain refinement Hot deformation interlayeredβ Lamellarα Titanium alloy
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Converting an O-vacancy-rich oxide into a multifunctional separator modifier for long-lifespan lithium metal batteries
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作者 Juntao Si Xiaoying Li +3 位作者 Yixuan Li Kuo Cao Yiran Zhu Chunhua Chen 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第10期371-378,I0007,共9页
The lithium metal anode is hailed as the desired "holy grail" for the forthcoming generation of highenergy-density batteries,given its astounding theoretical capacity and low potential.Nonetheless,the format... The lithium metal anode is hailed as the desired "holy grail" for the forthcoming generation of highenergy-density batteries,given its astounding theoretical capacity and low potential.Nonetheless,the formation and growth of dendrites seriously compromise battery life and safety.Herein,an yttriastabilized bismuth oxide(YSB) layer is fabricated on the polypropylene(PP) separator,where YSB reacts with Li anode in-situ in the cell to form a multi-component composite interlayer consisting of Li_(3)Bi,Li_(2)O,and Y_(2)O_(3).The interlayer can function not only as a redistributor to regulate Li^(+) distribution but also as an anion adsorber to increase the Li^(+) transference number from 0.37 to 0.79 for suppressing dendrite nucleation and growth.Consequently,compared with the cell with a baseline separator,those with modified separators exhibit prolonged lifespan in both Li/Li symmetrical cells and Li/Cu half-cells.Notably,the full cells coupled with ultrahigh-loading LiFePO_(4) display an excellent cycling performance of 1700 cycles with a high capacity retention of ~80% at 1 C,exhibiting great potential for practical applications.This work provides a feasible and effective new strategy for separator modification towards building a much-anticipated dendrite-free Li anode and realizing long-lifespan lithium metal batteries. 展开更多
关键词 Lithium metal battery SEPARATOR Dendrite-free Multifunctional interlayer Conversion-alloying reaction
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Tuning the crystallinity of titanium nitride on copper-embedded carbon nanofiber interlayers for accelerated electrochemical kinetics in lithium-sulfur batteries
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作者 Yinyu Xiang Liqiang Lu +4 位作者 Feng Yan Debarun Sengupta Petra Rudolf Ajay Giri Prakash Kottapalli Yutao Pei 《Carbon Energy》 SCIE EI CAS CSCD 2024年第6期40-55,共16页
The development of lithium-sulfur(Li-S)batteries is hindered by the disadvantages of shuttling of polysulfides and the sluggish redox kinetics of the conversion of sulfur species during discharge and charge.Herein,the... The development of lithium-sulfur(Li-S)batteries is hindered by the disadvantages of shuttling of polysulfides and the sluggish redox kinetics of the conversion of sulfur species during discharge and charge.Herein,the crystallinities of a titanium nitride(TiN)film on copper-embedded carbon nanofibers(Cu-CNFs)are regulated and the nanofibers are used as interlayers to resolve the aforementioned crucial issues.A low-crystalline TiN-coated Cu-CNF(L-TiN-Cu-CNF)interlayer is compared with its highly crystalline counterpart(H-TiN-Cu-CNFs).It is demonstrated that the L-TiN coating not only strengthens the chemical adsorption toward polysulfides but also greatly accelerates the electrochemical conversion of polysulfides.Due to robust carbon frameworks and enhanced kinetics,impressive highrate performance at 2 C(913 mAh g^(-1)based on sulfur)as well as remarkable cyclic stability up to 300 cycles(626 mAh g^(-1))with capacity retention of 46.5%is realized for L-TiN-Cu-CNF interlayer-configured Li-S batteries.Even under high loading(3.8 mg cm^(-2))of sulfur and relatively lean electrolyte(10μL electrolyte per milligram sulfur)conditions,the Li-S battery equipped with L-TiN-Cu-CNF interlayers delivers a high capacity of 1144 mAh g^(-1)with cathodic capacity of 4.25 mAh cm^(-2)at 0.1 C,providing a potential pathway toward the design of multifunctional interlayers for highly efficient Li-S batteries. 展开更多
关键词 CRYSTALLINITY electrochemical kinetics INTERLAYER lithium-sulfur batteries titanium nitride
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High mechanical strength Si anode synthesis with interlayer bonded expanded graphite structure for lithium-ion batteries
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作者 Wenhui Lai Jong Hak Lee +8 位作者 Lu Shi Yuqing Liu Yanhui Pu Yong Kang Ong Carlos Limpo Ting Xiong Yifan Rao Chorng Haur Sow Barbaros Ozyilmaz 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第6期253-263,I0007,共12页
Despite advancements in silicon-based anodes for high-capacity lithium-ion batteries,their widespread commercial adoption is still hindered by significant volume expansion during cycling,especially at high active mass... Despite advancements in silicon-based anodes for high-capacity lithium-ion batteries,their widespread commercial adoption is still hindered by significant volume expansion during cycling,especially at high active mass loadings crucial for practical use.The root of these challenges lies in the mechanical instability of the material,which subsequently leads to the structural failure of the electrode.Here,we present a novel synthesis of a composite combining expanded graphite and silicon nanoparticles.This composite features a unique interlayer-bonded graphite structure,achieved through the application of a modified spark plasma sintering method.Notably,this innovative structure not only facilitates efficient ion and electron transport but also provides exceptional mechanical strength(Vickers hardness:up to658 MPa,Young's modulus:11.6 GPa).This strength effectively accommodates silicon expansion,resulting in an impressive areal capacity of 2.9 mA h cm^(-2)(736 mA h g^(-1)) and a steady cycle life(93% after 100cycles).Such outsta nding performance is paired with features appropriate for large-scale industrial production of silicon batteries,such as active mass loading of at least 3.9 mg cm^(-2),a high-tap density electrode material of 1.68 g cm^(-3)(secondary clusters:1.12 g cm^(-3)),and a production yield of up to 1 kg per day. 展开更多
关键词 Lithium-ion battery Silicon anode Spark plasma sintering Interlayer bonding Mechanical strength Tap density
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Interlayer Magnetic Interaction in the CrI_(3)/CrSe_(2) Heterostructure
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作者 王秋皓 倪美燕 +3 位作者 李淑静 郑法伟 路洪艳 张平 《Chinese Physics Letters》 SCIE EI CAS CSCD 2024年第5期85-89,共5页
Based on first-principles calculations, we systematically study the stacking energy and interlayer magnetic interaction of the heterobilayer composed of CrI_(3) and CrSe_(2) monolayers. It is found that the stacking o... Based on first-principles calculations, we systematically study the stacking energy and interlayer magnetic interaction of the heterobilayer composed of CrI_(3) and CrSe_(2) monolayers. It is found that the stacking order plays a crucial role in the interlayer magnetic coupling. Among all possible stacking structures, the AA-stacking is the most stable heterostructure, exhibiting interlayer antiferromagnetic interactions. Interestingly, the interlayer magnetic interaction can be effectively tuned by biaxial strain. A 4.3% compressive strain would result in a ferromagnetic interlayer interaction in all stacking orders. These results reveal the magnetic properties of CrI_(3)/CrSe_(2) heterostructure, which is expected to be applied to spintronic devices. 展开更多
关键词 STRAIN STACKING INTERLAYER
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Stable Organic Solar Cells Enabled by Simultaneous Hole and Electron Interlayer Engineering
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作者 Wisnu Tantyo Hadmojo Furkan H.Isikgor +12 位作者 Yuanbao Lin Zhaoheng Ling Qiao He Hendrik Faber Emre Yengel Roshan Ali Abdus Samad Ryanda Enggar Anugrah Ardhi Sang Young Jeong Han Young Woo Udo Schwingenschlögl Martin Heeney Thomas D.Anthopoulos 《Energy & Environmental Materials》 SCIE EI CAS CSCD 2024年第5期313-320,共8页
The development of high-performance organic solar cells(OSCs)with high operational stability is essential to accelerate their commercialization.Unfortunately,our understanding of the origin of instabilities in state-o... The development of high-performance organic solar cells(OSCs)with high operational stability is essential to accelerate their commercialization.Unfortunately,our understanding of the origin of instabilities in state-of-the-art OSCs based on bulk heterojunction(BHJ)featuring non-fullerene acceptors(NFAs)remains limited.Herein,we developed NFA-based OSCs using different charge extraction interlayer materials and studied their storage,thermal,and operational stabilities.Despite the high power conversion efficiency(PCE)of the OSCs(17.54%),we found that cells featuring self-assembled monolayers(SAMs)as hole-extraction interlayers exhibited poor stability.The time required for these OSCs to reach 80%of their initial performance(T_(80))was only 6h under continuous thermal stress at 85℃in a nitrogen atmosphere and 1 h under maximum power point tracking(MPPT)in a vacuum.Inserting MoO_(x)between ITO and SAM enhanced the T_(80)to 50 and~15 h after the thermal and operational stability tests,respectively,while maintaining a PCE of 16.9%.Replacing the organic PDINN electron transport layer with ZnO NPs further enhances the cells'thermal and operational stability,boosting the T_(80)to 1000 and 170 h,respectively.Our work reveals the synergistic roles of charge-selective interlayers and device architecture in developing efficient and stable OSCs. 展开更多
关键词 INTERLAYERS metal oxide organic solar cells self-assembled monolayers stability
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Minimizing interfacial energy losses in inverted perovskite solar cells by a dipolar stereochemical 2D perovskite interface
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作者 Junjie Qian Jingjing He +10 位作者 Qihang Zhang Chenyue Zhu Shilin Chen Zhanpeng Wei Xuesong Leng Ziren Zhou Benben Shen Yu Peng Qiang Niu Shuang Yang Yu Hou 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第3期496-503,I0011,共9页
Inverted perovskite solar cells(PSCs) have attracted broad research and industrial interest owing to their suppressed hysteresis,cost-effectiveness,and easy-fabrication.However,the issue of non-radiative recombination... Inverted perovskite solar cells(PSCs) have attracted broad research and industrial interest owing to their suppressed hysteresis,cost-effectiveness,and easy-fabrication.However,the issue of non-radiative recombination losses at the n-type interface between the perovskite and fullerene has impeded further improvement of photovoltaic performance.Here,we modify the n-type interface of FAPbI_(3) perovskite films by constructing a stereochemical two-dimensional(2D) perovskite interlayer,in which the organic cations comprise both pyridine and ammonium groups.The pyridine N donor can create stable bonding with the surface-uncoordinated Pb on the perovskite,thereby passivating the shallow-level defects and enhancing the air stability of the film.Furthermore,the pyridine N donor also offers a positive polar interface to decrease the surface work function of the perovskite film,enabling n-type modification.Ultimately,we employ a p-i-n photovoltaic(PV) device with the positive dipole interlayer at perovskite/fullerene contact and achieve remarkable photoelectric conversion efficiency(PCE) of 22.0%. 展开更多
关键词 Perovskite solar cells Dipole interlayer STEREOCHEMISTRY Non-radiative recombination
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Peak structure in the interlayer conductance of Moirésuperlattices
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作者 Yizhou Tao Chao Liu +1 位作者 Mingwen Xiao Henan Fang 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第10期376-380,共5页
We investigate the peak structure in the interlayer conductance of Moirésuperlattices using a tunneling theory wedeveloped previously.The theoretical results predict that,due to the resonance of two different par... We investigate the peak structure in the interlayer conductance of Moirésuperlattices using a tunneling theory wedeveloped previously.The theoretical results predict that,due to the resonance of two different partial waves,the doublepeakstructure can appear in the curve of the interlayer conductance versus twist angle.Furthermore,we study the influencesof the model parameters,i.e.,the chemical potential of electrodes,the thickness of Moirésuperlattice,and the strength ofinterface potential,on the peak structure of the interlayer conductance.In particular,the parameter dependence of the peakstructure is concluded via a phase diagram,and the physical meanings of the phase diagram is formulized.Finally,thepotential applications of the present work is discussed. 展开更多
关键词 Moirésuperlattice interlayer conductance electronic transport twistronics
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Enhanced High-Temperature Cycling Stability of Garnet-Based All Solid-State Lithium Battery Using a Multi-Functional Catholyte Buffer Layer
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作者 Leqi Zhao Yijun Zhong +2 位作者 Chencheng Cao Tony Tang Zongping Shao 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第7期59-73,共15页
The pursuit of safer and high-performance lithium-ion batteries(LIBs)has triggered extensive research activities on solid-state batteries,while challenges related to the unstable electrode-electrolyte interface hinder... The pursuit of safer and high-performance lithium-ion batteries(LIBs)has triggered extensive research activities on solid-state batteries,while challenges related to the unstable electrode-electrolyte interface hinder their practical implementation.Polymer has been used extensively to improve the cathode-electrolyte interface in garnet-based all-solid-state LIBs(ASSLBs),while it introduces new concerns about thermal stability.In this study,we propose the incorporation of a multi-functional flame-retardant triphenyl phos-phate additive into poly(ethylene oxide),acting as a thin buffer layer between LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)cathode and garnet electro-lyte.Through electrochemical stability tests,cycling performance evaluations,interfacial thermal stability analysis and flammability tests,improved thermal stability(capacity retention of 98.5%after 100 cycles at 60℃,and 89.6%after 50 cycles at 80℃)and safety characteristics(safe and stable cycling up to 100℃)are demonstrated.Based on various materials characterizations,the mechanism for the improved thermal stability of the interface is proposed.The results highlight the potential of multi-functional flame-retardant additives to address the challenges associated with the electrode-electrolyte interface in ASSLBs at high temperature.Efficient thermal modification in ASSLBs operating at elevated temperatures is also essential for enabling large-scale energy storage with safety being the primary concern. 展开更多
关键词 Solid-state battery Cathode electrolyte interlayer Flame-retardant additive Cycling stability Interfacial stability
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Moiré superlattices arising from growth induced by screw dislocations in layered materials
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作者 田伏钰 Muhammad Faizan +2 位作者 贺欣 孙远慧 张立军 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第7期72-77,共6页
Moiré superlattices(MSLs) are modulated structures produced from homogeneous or heterogeneous two-dimensional layers stacked with a twist angle and/or lattice mismatch. Enriching the methods for fabricating MSL a... Moiré superlattices(MSLs) are modulated structures produced from homogeneous or heterogeneous two-dimensional layers stacked with a twist angle and/or lattice mismatch. Enriching the methods for fabricating MSL and realizing the unique emergent properties are key challenges in its investigation. Here we recommend that the spiral dislocation driven growth is another optional method for the preparation of high quality MSL samples. The spiral structure stabilizes the constant out-of-plane lattice distance, causing the variations in electronic and optical properties. Taking SnS_(2) MSL as an example, we find prominent properties including large band gap reduction(~ 0.4 e V) and enhanced optical activity. Firstprinciples calculations reveal that these unusual properties can be ascribed to the locally enhanced interlayer interaction associated with the Moiré potential modulation. We believe that the spiral dislocation driven growth would be a powerful method to expand the MSL family and broaden their scope of application. 展开更多
关键词 Moirésuperlattices interlayer interaction spiral dislocation layered materials
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Recent advances and perspectives in MXene-based cathodes for aqueous zinc-ion batteries
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作者 Aiduo Wu Tianhao Wang +4 位作者 Long Zhang Chen Chen Qiaomin Li Xuanhui Qu Yongchang Liu 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS CSCD 2024年第7期1752-1765,共14页
Aqueous zinc-ion batteries(AZIBs)show great potential for applications in grid-scale energy storage,given their intrinsic safety,cost effectiveness,environmental friendliness,and impressive electrochemical performance... Aqueous zinc-ion batteries(AZIBs)show great potential for applications in grid-scale energy storage,given their intrinsic safety,cost effectiveness,environmental friendliness,and impressive electrochemical performance.However,strong electrostatic interactions exist between zinc ions and host materials,and they hinder the development of advanced cathode materials for efficient,rapid,and stable Zn-ion storage.MXenes and their derivatives possess a large interlayer spacing,excellent hydrophilicity,outstanding electronic conductivity,and high redox activity.These materials are considered“rising star”cathode candidates for AZIBs.This comprehensive review discusses recent advances in MXenes as AZIB cathodes from the perspectives of crystal structure,Zn-storage mechanism,surface modification,interlayer engineering,and conductive network design to elucidate the correlations among their composition,structure,and electrochemical performance.This work also outlines the remaining challenges faced by MXenes for aqueous Zn-ion storage,such as the urgent need for improved toxic preparation methods,exploration of potential novel MXene cathodes,and suppression of layered MXene restacking upon cycling,and introduces the prospects of MXene-based cathode materials for high-performance AZIBs. 展开更多
关键词 aqueous zinc-ion batteries MXenes terminal groups interlayer engineering conductive network design
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Effect of interlayer bonded bilayer graphene on friction
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作者 李耀隆 田振国 +1 位作者 尹海峰 张任良 《Chinese Physics B》 SCIE EI CAS CSCD 2024年第8期389-395,共7页
We study the friction properties of interlayer bonded bilayer graphene by simulating the movement of a slider on the surface of bilayer graphene using molecular dynamics.The results show that the presence of the inter... We study the friction properties of interlayer bonded bilayer graphene by simulating the movement of a slider on the surface of bilayer graphene using molecular dynamics.The results show that the presence of the interlayer covalent bonds due to the local sp^(3) hybridization of carbon atoms in the bilayer graphene seriously reduces the frictional coefficient of the bilayer graphene surface to 30%,depending on the coverage of interlayer sp^(3) bonds and normal loads.For a certain coverage of interlayer sp3bonds,when the normal load of the slider reaches a certain value,the surface of this interlayer bonded bilayer graphene will lose the friction reduction effect on the slider.Our findings provide guidance for the regulation and manipulation of the frictional properties of bilayer graphene surfaces through interlayer covalent bonds,which may be useful for applications of friction related graphene based nanodevices. 展开更多
关键词 nanoscale friction molecular dynamic simulation bilayer graphene interlayer covalent bond
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Accelerating lithium-sulfur battery reaction kinetics and inducing 3D deposition of Li_(2)S using interactions between Fe_(3)Se_(4)and lithium polysulfides
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作者 Yihan Lin Liheng Li +5 位作者 Longjie Tan Yongliang Li Xiangzhong Ren Peixin Zhang Chuanxin He Lingna Sun 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第8期540-553,I0012,共15页
Although lithium-sulfur batteries(LSBs)exhibit high theoretical energy density,their practical application is hindered by poor conductivity of the sulfur cathode,the shuttle effect,and the irreversible deposition of L... Although lithium-sulfur batteries(LSBs)exhibit high theoretical energy density,their practical application is hindered by poor conductivity of the sulfur cathode,the shuttle effect,and the irreversible deposition of Li_(2)S.To address these issues,a novel composite,using electrospinning technology,consisting of Fe_(3)Se_(4)and porous nitrogen-doped carbon nanofibers was designed for the interlayer of LSBs.The porous carbon nanofiber structure facilitates the transport of ions and electrons,while the Fe_(3)Se_(4)material adsorbs lithium polysulfides(LiPSs)and accelerates its catalytic conversion process.Furthermore,the Fe_(3)Se_(4)material interacts with soluble LiPSs to generate a new polysulfide intermediate,Li_(x)FeS_(y)complex,which changes the electrochemical reaction pathway and facilitates the three-dimensional deposition of Li_(2)S,enhancing the reversibility of LSBs.The designed LSB demonstrates a high specific capacity of1529.6 mA h g^(-1)in the first cycle at 0.2 C.The rate performance is also excellent,maintaining an ultra-high specific capacity of 779.7 mA h g^(-1)at a high rate of 8 C.This investigation explores the mechanism of the interaction between the interlayer and LiPSs,and provides a new strategy to regulate the reaction kinetics and Li_(2)S deposition in LSBs. 展开更多
关键词 Lithium-sulfur batteries Polysulfide intermediates Li_(2)S electrodeposition INTERLAYERS Electrostatic spinning Adsorption Catalysis
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Experimental study on seismic reinforcement of bridge foundation on silty clay landslide with inclined interlayer
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作者 Lei Da Xiao Hanmo +3 位作者 Ran Jianhua Luo Bin Jiang Guanlu Xue Tianlang 《Earthquake Engineering and Engineering Vibration》 SCIE EI CSCD 2024年第1期193-207,共15页
A shaking table test for a bridge foundation reinforced by anti-slide piles on a silty clay landslide model with an inclined interlayer was performed.The deformation characteristics of the bridge foundation piles and ... A shaking table test for a bridge foundation reinforced by anti-slide piles on a silty clay landslide model with an inclined interlayer was performed.The deformation characteristics of the bridge foundation piles and anti-slide piles were analyzed in different loading conditions.The dynamic response law of a silty clay landslide with an inclined interlayer was summarized.The spacing between the rear anti-slide piles and bridge foundation should be reasonably controlled according to the seismic fortification requirements,to avoid the two peaks in the forced deformation of the bridge foundation piles.The“blocking effect”of the bridge foundation piles reduced the deformation of the forward anti-slide piles.The stress-strain response of silty clay was intensified as the vibration wave field appeared on the slope.Since the vibration intensified,the thrust distribution of the landslide underwent a process of shifting from triangle to inverted trapezoid,the difference in the acceleration response between the bearing platform and silty clay landslide tended to decrease,and the spectrum amplitude near the natural vibration frequency increased.The rear anti-slide piles were able to slow down the shear deformation of the soil in front of the piles and avoid excessive acceleration response of the bridge foundation piles. 展开更多
关键词 silty clay landslide inclined interlayer shaking table test anti-slide pile bridge foundation pile
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Numerical analysis on seismic performance of underground structures in liquefiable interlayer sites from centrifuge shaking table test
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作者 Yan Guanyu Xu Chengshun +2 位作者 Zhang Zihong Du Xiuli Wang Xuelai 《Earthquake Engineering and Engineering Vibration》 SCIE EI CSCD 2024年第4期781-798,共18页
When an underground structure passes through a liquefiable soil layer,the soil liquefaction may pose a significant threat to the structure.A centrifuge shaking table test was performed to research the seismic response... When an underground structure passes through a liquefiable soil layer,the soil liquefaction may pose a significant threat to the structure.A centrifuge shaking table test was performed to research the seismic response of underground structures in liquefiable interlayer sites,and a valid numerical model was obtained through simulation model test.Finally,the calibrated numerical model was used to perform further research on the influence of various distribution characteristics of liquefiable interlayers on the seismic reaction of underground structures.The key findings are as follows.The structure faces the most unfavorable condition once a liquefiable layer is located in the middle of the underground structure.When a liquefiable layer exists in the middle of the structure,the seismic reactions of both the underground structure and model site will increase with the rise of the thickness of the liquefiable interlayer.The inter-story drift of the structure in the non-liquefiable site is much smaller than that in the liquefiable interlayer site.The inter-story drift of the structure is not only associated with the site displacement and the soil-structure stiffness ratio but also closely associated with the slippage of the soil-structure contact interface under the condition of large deformation of the site. 展开更多
关键词 centrifuge shaking table test underground structure liquefiable interlayer sites seismic response validation of numerical model
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Performance-control-orientated hybrid metal additive manufacturing technologies:state of the art,challenges,and future trends
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作者 Jiming Lv Yuchen Liang +6 位作者 Xiang Xu Gang Xu Hongmei Zhang Haifei Lu Kaiyu Luo Jie Cai Jinzhong Lu 《International Journal of Extreme Manufacturing》 SCIE EI CAS CSCD 2024年第3期274-328,共55页
Metal additive manufacturing(AM)technologies have made significant progress in the basic theoretical field since their invention in the 1970s.However,performance instability during continuous processing,such as therma... Metal additive manufacturing(AM)technologies have made significant progress in the basic theoretical field since their invention in the 1970s.However,performance instability during continuous processing,such as thermal history,residual stress accumulation,and columnar grain epitaxial growth,consistently hinders their broad application in standardized industrial production.To overcome these challenges,performance-control-oriented hybrid AM(HAM)technologies have been introduced.These technologies,by leveraging external auxiliary processes,aim to regulate microstructural evolution and mechanical properties during metal AM.This paper provides a systematic and detailed review of performance-control-oriented HAM technology,which is categorized into two main groups:energy field-assisted AM(EFed AM,e.g.ultrasonic,electromagnetic,and heat)technologies and interlayer plastic deformation-assisted AM(IPDed AM,e.g.laser shock peening,rolling,ultrasonic peening,and friction stir process)technologies.This review covers the influence of external energy fields on the melting,flow,and solidification behavior of materials,and the regulatory effects of interlayer plastic deformation on grain refinement,nucleation,and recrystallization.Furthermore,the role of performance-control-oriented HAM technologies in managing residual stress conversion,metallurgical defect closure,mechanical property improvement,and anisotropy regulation is thoroughly reviewed and discussed.The review concludes with an analysis of future development trends in EFed AM and IPDed AM technologies. 展开更多
关键词 hybrid additive manufacturing in-situ/interlayer plastic deformation auxiliary energy fields microstructure customization mechanical properties enhancement
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A Transient-Pressure-Based Numerical Approach for Interlayer Identification in Sand Reservoirs
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作者 Hao Luo Haibo Deng +4 位作者 Honglin Xiao Shaoyang Geng Fu Hou Gang Luo Yaqi Li 《Fluid Dynamics & Materials Processing》 EI 2024年第3期641-659,共19页
Almost all sandstone reservoirs contain interlayers. The identification and characterization of these interlayers iscritical for minimizing the uncertainty associated with oilfield development and improving oil and ga... Almost all sandstone reservoirs contain interlayers. The identification and characterization of these interlayers iscritical for minimizing the uncertainty associated with oilfield development and improving oil and gas recovery.Identifying interlayers outside wells using identification methods based on logging data and machine learning isdifficult and seismic-based identification techniques are expensive. Herein, a numerical model based on seepageand well-testing theories is introduced to identify interlayers using transient pressure data. The proposed modelrelies on the open-source MATLAB Reservoir Simulation Toolbox. The effects of the interlayer thickness, position,and width on the pressure response are thoroughly investigated. A procedure for inverting interlayer parametersin the reservoir using the bottom-hole pressure is also proposed. This method uses only transient pressuredata during well testing and can effectively identify the interlayer distribution near the wellbore at an extremelylow cost. The reliability of the model is verified using effective oilfield examples. 展开更多
关键词 Sand reservoir interlayer identification transient pressure analysis numerical well test
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