Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency t...Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency transfer,measurement of fundamental physical constants,and high-precision ranging,achieving a series of milestone results in ground-based environments.With the continuous maturation and evolution of femtosecond lasers and related technologies,optical frequency combs are moving from ground-based applications to astronomical and space-based applications,playing an increasingly important role in atomic clocks,exoplanet observations,gravitational wave measurements,and other areas.This paper,focusing on astronomical and space-based applications,reviews research progress on astronomical frequency combs,optical clock time-frequency networks,gravitational waves,dark matter measurement,dual-comb large-scale absolute ranging,and high-resolution atmospheric spectroscopy.With enhanced performance and their gradual application in the field of space-based research,optical frequency combs will undoubtedly provide more powerful support for astronomical science and cosmic exploration in the future.展开更多
Optical frequency combbased Fourier transform spectroscopy has the features of broad spectral bandwidth,high sensitivity,andmultiplexed trace gas detection,which has valuable application potential in the fields of pre...Optical frequency combbased Fourier transform spectroscopy has the features of broad spectral bandwidth,high sensitivity,andmultiplexed trace gas detection,which has valuable application potential in the fields of precision spectroscopy and trace gas detection.Here,we report the development of a mid-infrared Fourier transform spectrometer based on an optical frequency comb combined with a Herriott-type multipass cell.Using this instrument,the broadband absorption spectra of several important molecules,including methane,acetylene,water molecules and nitrous oxide,are measured by near real-time data acquisition in the 2800-3500 cm^(-1)spectral region.The achieved minimum detectable absorption of the instrument is 4.4×10^(-8)cm^(-1)·Hz^(-1/2)per spectral element.Broadband spectra of H_(2)0 are fited using the Voigt profile multispectral fitting technique and the consistency of the concentration inversion is 1%.Our system also enables precise spectroscopic measurements,and it allows the determination of the spectral line positions and upper state constants of N_(2)O in the(0002)-(1000)band,with results in good agreement with those reported by Toth[Appl.Opt.30,5289(1991)].展开更多
Laser absorption spectroscopy has proven to be an effective approach for gas sensing, which plays an important rolein the fields of military, industry, medicine and basic research. This paper presents a multiplexed ga...Laser absorption spectroscopy has proven to be an effective approach for gas sensing, which plays an important rolein the fields of military, industry, medicine and basic research. This paper presents a multiplexed gas sensing system basedon optical frequency comb (OFC) calibrated frequency-modulated continuous-wave (FMCW) tuning nonlinearity. Thesystem can be used for multi-parameter synchronous measurement of gas absorption spectrum and multiplexed opticalpath. Multi-channel parallel detection is realized by combining wavelength division multiplexing (WDM) and frequencydivision multiplexing (FDM) techniques. By introducing nonlinear optical crystals, broadband spectrum detection is simultaneouslyachieved over a bandwidth of hundreds of nanometers. An OFC with ultra-high frequency stability is used asthe frequency calibration source, which guarantees the measurement accuracy. The test samples involve H13C14N, C_(2)H_(2)and Rb vapor cells of varying densities and 5 parallel measurement experiments are designed. The results show that themeasurement accuracies of spectral absorption line and the optical path are 150 MHz and 20 m, respectively. The schemeoffers the advantages of multiplexed, multi-parameter, wide spectrum and high resolution detection, which can realize theidentification of multi-gas components and the high-precision inversion of absorption lines under different environments.The proposed sensor demonstrates great potential in the field of high-resolution absorption spectrum measurement for gassensing applications.展开更多
The Fabry–Perot(FP) resonant cavity is widely used in laser and spectroscopic measurements due to its unique interference transfer function(ITF). In the ideal case of parallel incident light, the ITF of the FP resona...The Fabry–Perot(FP) resonant cavity is widely used in laser and spectroscopic measurements due to its unique interference transfer function(ITF). In the ideal case of parallel incident light, the ITF of the FP resonant cavity can be expressed by the Airy function. However, in reality, it is difficult to achieve perfect parallelism with collimated beams. In this article, a theoretical model is established for non-parallel light incidence, which assumes that the non-parallel incident light is a cone-shaped beam, and the cone angle is used to quantify the non-parallelism of the beam. The transmittance function of the FP resonant cavity under non-parallel light incidence is derived. The accuracy of the model is experimentally verified. Based on this model, the effects of divergence angle, tilt angle and FP cavity parameters(reflectivity, cavity length)on the ITF are studied. The reasons for the decrease in peak value, broadening and asymmetry of the interference peak under non-parallel light incidence are explained. It is suggested that a fine balance between the interference peak and the collimation effect of the incident light should be considered in the design and application of FP resonant cavities, especially for tilted applications such as angle-scanned spectroscopy. The research results of this article have certain significance for the design and application of FP resonant cavities.展开更多
Based on a semiconductor laser （SL） with incoherent optical feedback, a novel all-optical scheme for generating tunable and broadband microwave frequency combs （MFCs） is proposed and investigated numerically. The ...Based on a semiconductor laser （SL） with incoherent optical feedback, a novel all-optical scheme for generating tunable and broadband microwave frequency combs （MFCs） is proposed and investigated numerically. The results show that, under suitable operation parameters, the SL with incoherent optical feedback can be driven to operate at a regular pulsing state, and the generated MFCs have bandwidths broader than 40 GHz within a 10 dB amplitude variation. For a fixed bias current, the line spacing （or repetition frequency） of the MFCs can be easily tuned by varying the feedback delay time and the feedback strength, and the tuning range of the line spacing increases with the increase in the bias current. The linewidth of the MFCs is sensitive to the variation of the feedback delay time and the feedback strength, and a linewidth of tens of KHz can be achieved through finely adjusting the feedback delay time and the feedback strength. In addition, mappings of amplitude variation, repetition frequency, and linewidth of MFCs in the parameter space of the feedback delay time and the feedback strength are presented.展开更多
Optical frequency comb with evenly spaced lines over a broad bandwidth has revolutionized the fields of optical metrology and spectroscopy.Here,we propose a fast interleaved dual-comb spectroscopy with sub-femtometer-...Optical frequency comb with evenly spaced lines over a broad bandwidth has revolutionized the fields of optical metrology and spectroscopy.Here,we propose a fast interleaved dual-comb spectroscopy with sub-femtometer-resolution and absolute frequency,in which two electro-optic frequency combs are swept.Electrically-modulated stabilized laser enables ultrahigh resolution of 0.16 fm(or 20 k Hz in optical frequency)and single-shot measurement in 90 ms.Total 20 million points are recorded spanning 3.2 nm(or 400 GHz)bandwidth,corresponding to a spectral sampling rate of 2.5×10^(8)points/s under Nyquist-limitation.Besides,considering the trade-off between the measurement time and spectral resolution,a fast single-shot measurement is also realized in 1.6 ms with 8 fm(or 1 MHz)resolution.We demonstrate the 25-averaged result with 30.6 d B spectral measurement signal-to-noise ratio(SNR)by reducing the filter bandwidth in demodulation.The results show great prospect for precise measurement with flexibly fast refresh time,high spectral resolution,and high SNR.展开更多
Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study...Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study of signals during the generation of the Kerr optical frequency combs(OFCs). We find that the signals in different states, including the Turing pattern, the chaos, the single soliton state, and the multi-solitons state, can be distinguished according to different distributions of the eigenvalue spectrum. Specially, the eigenvalue spectrum of the single soliton pulse is composed of a pair of conjugate symmetric discrete eigenvalues and the quasi-continuous eigenvalue spectrum with eye-like structure.Moreover, we have successfully demonstrated that the number of discrete eigenvalue pairs in the eigenvalue spectrum corresponds to the number of solitons formed in a round-trip time inside the Kerr microresonator. This work shows that some characteristics of the time-domain signal can be well reflected in the nonlinear domain.展开更多
We review recent work on broadband RF channelizers based on integrated optical frequency Kerr micro-combs combined with passive micro-ring resonator filters,with microcombs having channel spacings of 200 and 49 GHz.Th...We review recent work on broadband RF channelizers based on integrated optical frequency Kerr micro-combs combined with passive micro-ring resonator filters,with microcombs having channel spacings of 200 and 49 GHz.This approach to realizing RF channelizers offers reduced complexity,size,and potential cost for a wide range of applications to microwave signal detection.展开更多
Frequency combs[1, 2] consisting of equally-spaced frequencylines can be fully described by two frequencies, i.e., carrieroffset (fCEO) and repetition rate (frep). Once the two frequenciesare stabilized, the frequency...Frequency combs[1, 2] consisting of equally-spaced frequencylines can be fully described by two frequencies, i.e., carrieroffset (fCEO) and repetition rate (frep). Once the two frequenciesare stabilized, the frequency comb is well defined. Frequencycombs can be used for various applications, i.e., metrology,spectroscopy, timing, communications, absolute distancemeasurements, and so on, due to their two importantcharacteristics, i.e., stabilized frequency lines and ultra-shortoptical pulses (if the mode-locking is obtained) as shown inFig. 1.展开更多
The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective f...The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective four wave-mixing in the active semiconductor gain medium. The low-noise Gaussian-like pulse can be obtained by locking the relaxation oscillation and compensating the gain asymmetry. The simulations suggest that pulse trains of width below 30 ps and repetition rate in GHz frequency can be generated simply by the optical injection locking of semiconductor lasers. Since the optical injection locking can broaden the spectrum and amplify the optical power simultaneously, it can be a good initial stage for generating optical frequency combs from dual-frequency lasers by multi-stage of spectral broadening in nonlinear waveguides.展开更多
This paper presents a novel approach to improve aliasing rejection in comb-based decimation filters. The method is established on certain palindromic polynomials with all zeros on the unit circle and the sharpening te...This paper presents a novel approach to improve aliasing rejection in comb-based decimation filters. The method is established on certain palindromic polynomials with all zeros on the unit circle and the sharpening technique. As a result, aliasing rejection and the passband characteristic are improved. The method is illustrated with various examples and compared with the methods from the literature. .展开更多
Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,t...Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,the temporal and spectral features of the HHG were shown to carry profound insight into frequency-comb emission dynamics.Here we present an ab initio investigation of the temporal and spectral coherence of the frequency comb emitted in HHG of He atom driven by few-cycle pulse trains.We find that the emission of frequency combs features a destructive and constructive coherences caused by the phase interference of HHG,leading to suppression and enhancement of frequency-comb emission.The results reveal intriguing and substantially different nonlinear optical response behaviors for frequency-comb emission via HHG.The dynamical origin of frequency-comb emission is clarified by analyzing the phase coherence in HHG processes in detail.Our results provide fresh insight into the experimental realization of selective enhancement of frequency comb in the VUV–XUV regimes.展开更多
基金support of the National Natural Sci-ence Foundation of China(NSFC)(62305373)the Strategic Priority Research Program of the Chinese Academy of Sciences(XDA1502040404,XDB2101040004).
文摘Optical frequency combs,as powerful tools for precision spectroscopy and research into optical frequency standards,have driven continuous progress and significant breakthroughs in applications such as time-frequency transfer,measurement of fundamental physical constants,and high-precision ranging,achieving a series of milestone results in ground-based environments.With the continuous maturation and evolution of femtosecond lasers and related technologies,optical frequency combs are moving from ground-based applications to astronomical and space-based applications,playing an increasingly important role in atomic clocks,exoplanet observations,gravitational wave measurements,and other areas.This paper,focusing on astronomical and space-based applications,reviews research progress on astronomical frequency combs,optical clock time-frequency networks,gravitational waves,dark matter measurement,dual-comb large-scale absolute ranging,and high-resolution atmospheric spectroscopy.With enhanced performance and their gradual application in the field of space-based research,optical frequency combs will undoubtedly provide more powerful support for astronomical science and cosmic exploration in the future.
基金supported by the National Natural Science Foundation China(No.42022051,No.U21A2028)Youth Innovation Promotion Association of the Chinese Academy of Sciences(No.Y202089)the HFIPS Director's Fund(No.YZJJ202101,No.BJPY2023A02).
文摘Optical frequency combbased Fourier transform spectroscopy has the features of broad spectral bandwidth,high sensitivity,andmultiplexed trace gas detection,which has valuable application potential in the fields of precision spectroscopy and trace gas detection.Here,we report the development of a mid-infrared Fourier transform spectrometer based on an optical frequency comb combined with a Herriott-type multipass cell.Using this instrument,the broadband absorption spectra of several important molecules,including methane,acetylene,water molecules and nitrous oxide,are measured by near real-time data acquisition in the 2800-3500 cm^(-1)spectral region.The achieved minimum detectable absorption of the instrument is 4.4×10^(-8)cm^(-1)·Hz^(-1/2)per spectral element.Broadband spectra of H_(2)0 are fited using the Voigt profile multispectral fitting technique and the consistency of the concentration inversion is 1%.Our system also enables precise spectroscopic measurements,and it allows the determination of the spectral line positions and upper state constants of N_(2)O in the(0002)-(1000)band,with results in good agreement with those reported by Toth[Appl.Opt.30,5289(1991)].
基金the National Natural Science Foun-dation of China(Grant No.52375546)the National Key Research and Development Program of China(Grant No.2022YFF0705701).
文摘Laser absorption spectroscopy has proven to be an effective approach for gas sensing, which plays an important rolein the fields of military, industry, medicine and basic research. This paper presents a multiplexed gas sensing system basedon optical frequency comb (OFC) calibrated frequency-modulated continuous-wave (FMCW) tuning nonlinearity. Thesystem can be used for multi-parameter synchronous measurement of gas absorption spectrum and multiplexed opticalpath. Multi-channel parallel detection is realized by combining wavelength division multiplexing (WDM) and frequencydivision multiplexing (FDM) techniques. By introducing nonlinear optical crystals, broadband spectrum detection is simultaneouslyachieved over a bandwidth of hundreds of nanometers. An OFC with ultra-high frequency stability is used asthe frequency calibration source, which guarantees the measurement accuracy. The test samples involve H13C14N, C_(2)H_(2)and Rb vapor cells of varying densities and 5 parallel measurement experiments are designed. The results show that themeasurement accuracies of spectral absorption line and the optical path are 150 MHz and 20 m, respectively. The schemeoffers the advantages of multiplexed, multi-parameter, wide spectrum and high resolution detection, which can realize theidentification of multi-gas components and the high-precision inversion of absorption lines under different environments.The proposed sensor demonstrates great potential in the field of high-resolution absorption spectrum measurement for gassensing applications.
基金Project supported by the National Natural Science Foundation of China (Grant No.U19A2044)the National Natural Science Foundation of China (Grant No.41975037)the Key Technologies Research and Development Program of Anhui Province (Grant No.202004i07020013)。
文摘The Fabry–Perot(FP) resonant cavity is widely used in laser and spectroscopic measurements due to its unique interference transfer function(ITF). In the ideal case of parallel incident light, the ITF of the FP resonant cavity can be expressed by the Airy function. However, in reality, it is difficult to achieve perfect parallelism with collimated beams. In this article, a theoretical model is established for non-parallel light incidence, which assumes that the non-parallel incident light is a cone-shaped beam, and the cone angle is used to quantify the non-parallelism of the beam. The transmittance function of the FP resonant cavity under non-parallel light incidence is derived. The accuracy of the model is experimentally verified. Based on this model, the effects of divergence angle, tilt angle and FP cavity parameters(reflectivity, cavity length)on the ITF are studied. The reasons for the decrease in peak value, broadening and asymmetry of the interference peak under non-parallel light incidence are explained. It is suggested that a fine balance between the interference peak and the collimation effect of the incident light should be considered in the design and application of FP resonant cavities, especially for tilted applications such as angle-scanned spectroscopy. The research results of this article have certain significance for the design and application of FP resonant cavities.
基金supported by the National Natural Science Foundation of China(Grant Nos.61178011,11204248,61475127,and 61275116)the Natural Science Foundation of Chongqing City,China(Grant Nos.2012jj B40011 and 2012jj A40012)the Open Fund of the State Key Lab of Millimeter Waves of China(Grant No.K201418)
文摘Based on a semiconductor laser （SL） with incoherent optical feedback, a novel all-optical scheme for generating tunable and broadband microwave frequency combs （MFCs） is proposed and investigated numerically. The results show that, under suitable operation parameters, the SL with incoherent optical feedback can be driven to operate at a regular pulsing state, and the generated MFCs have bandwidths broader than 40 GHz within a 10 dB amplitude variation. For a fixed bias current, the line spacing （or repetition frequency） of the MFCs can be easily tuned by varying the feedback delay time and the feedback strength, and the tuning range of the line spacing increases with the increase in the bias current. The linewidth of the MFCs is sensitive to the variation of the feedback delay time and the feedback strength, and a linewidth of tens of KHz can be achieved through finely adjusting the feedback delay time and the feedback strength. In addition, mappings of amplitude variation, repetition frequency, and linewidth of MFCs in the parameter space of the feedback delay time and the feedback strength are presented.
基金funding from National Natural Science Foundation of China(NSFC)under Grant Nos.61775132,61735015,61620106015supported by the Major Key Project of Peng Cheng Laboratory(PCL)。
文摘Optical frequency comb with evenly spaced lines over a broad bandwidth has revolutionized the fields of optical metrology and spectroscopy.Here,we propose a fast interleaved dual-comb spectroscopy with sub-femtometer-resolution and absolute frequency,in which two electro-optic frequency combs are swept.Electrically-modulated stabilized laser enables ultrahigh resolution of 0.16 fm(or 20 k Hz in optical frequency)and single-shot measurement in 90 ms.Total 20 million points are recorded spanning 3.2 nm(or 400 GHz)bandwidth,corresponding to a spectral sampling rate of 2.5×10^(8)points/s under Nyquist-limitation.Besides,considering the trade-off between the measurement time and spectral resolution,a fast single-shot measurement is also realized in 1.6 ms with 8 fm(or 1 MHz)resolution.We demonstrate the 25-averaged result with 30.6 d B spectral measurement signal-to-noise ratio(SNR)by reducing the filter bandwidth in demodulation.The results show great prospect for precise measurement with flexibly fast refresh time,high spectral resolution,and high SNR.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61475099 and 61922040)Program of State Key Laboratory of Quantum Optics and Quantum Optics Devices,China(Grant No.KF201701)the Key R&D Program of Guangdong Province,China(Grant No.2018B030325002)。
文摘Based on the nonlinear Schr?dinger equation(NLSE) with damping, detuning, and driving terms describing the evolution of signals in a Kerr microresonator, we apply periodic nonlinear Fourier transform(NFT) to the study of signals during the generation of the Kerr optical frequency combs(OFCs). We find that the signals in different states, including the Turing pattern, the chaos, the single soliton state, and the multi-solitons state, can be distinguished according to different distributions of the eigenvalue spectrum. Specially, the eigenvalue spectrum of the single soliton pulse is composed of a pair of conjugate symmetric discrete eigenvalues and the quasi-continuous eigenvalue spectrum with eye-like structure.Moreover, we have successfully demonstrated that the number of discrete eigenvalue pairs in the eigenvalue spectrum corresponds to the number of solitons formed in a round-trip time inside the Kerr microresonator. This work shows that some characteristics of the time-domain signal can be well reflected in the nonlinear domain.
文摘We review recent work on broadband RF channelizers based on integrated optical frequency Kerr micro-combs combined with passive micro-ring resonator filters,with microcombs having channel spacings of 200 and 49 GHz.This approach to realizing RF channelizers offers reduced complexity,size,and potential cost for a wide range of applications to microwave signal detection.
基金supported by the "Hundred-Talent" Program of Chinese Academy of Sciencesthe National Natural Science Foundation of China(61875220,61575214,61404150,61405233,and 61704181)+1 种基金the National Key R&D Program of China(2017YFF0106302 and 2017YFA0701005)Shanghai Municipal Commission of Science and Technology(17YF1430000)
文摘Frequency combs[1, 2] consisting of equally-spaced frequencylines can be fully described by two frequencies, i.e., carrieroffset (fCEO) and repetition rate (frep). Once the two frequenciesare stabilized, the frequency comb is well defined. Frequencycombs can be used for various applications, i.e., metrology,spectroscopy, timing, communications, absolute distancemeasurements, and so on, due to their two importantcharacteristics, i.e., stabilized frequency lines and ultra-shortoptical pulses (if the mode-locking is obtained) as shown inFig. 1.
基金Project supported by the National Natural Science Foundation of China(Grant No.62005215)。
文摘The optical injection locking of semiconductor lasers to dual-frequency lasers is studied by numerical simulations.The beat-note signals can be effectively transformed to optical frequency combs due to the effective four wave-mixing in the active semiconductor gain medium. The low-noise Gaussian-like pulse can be obtained by locking the relaxation oscillation and compensating the gain asymmetry. The simulations suggest that pulse trains of width below 30 ps and repetition rate in GHz frequency can be generated simply by the optical injection locking of semiconductor lasers. Since the optical injection locking can broaden the spectrum and amplify the optical power simultaneously, it can be a good initial stage for generating optical frequency combs from dual-frequency lasers by multi-stage of spectral broadening in nonlinear waveguides.
文摘This paper presents a novel approach to improve aliasing rejection in comb-based decimation filters. The method is established on certain palindromic polynomials with all zeros on the unit circle and the sharpening technique. As a result, aliasing rejection and the passband characteristic are improved. The method is illustrated with various examples and compared with the methods from the literature. .
基金the National Natural Science Foundation of China(Grant Nos.12074239 and 91850209)the Natural Science Foundation of Guangdong Province,China(Grant Nos.2020A1515010927 and 2020ST084)+1 种基金the Fund from the Department of Education of Guangdong Province,China(Grant Nos.2019KTSCX038 and 2020KCXTD012)the Fund from Shantou University(Grant No.NTF18030).
文摘Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition rates.In particular,the temporal and spectral features of the HHG were shown to carry profound insight into frequency-comb emission dynamics.Here we present an ab initio investigation of the temporal and spectral coherence of the frequency comb emitted in HHG of He atom driven by few-cycle pulse trains.We find that the emission of frequency combs features a destructive and constructive coherences caused by the phase interference of HHG,leading to suppression and enhancement of frequency-comb emission.The results reveal intriguing and substantially different nonlinear optical response behaviors for frequency-comb emission via HHG.The dynamical origin of frequency-comb emission is clarified by analyzing the phase coherence in HHG processes in detail.Our results provide fresh insight into the experimental realization of selective enhancement of frequency comb in the VUV–XUV regimes.
