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Synthesis of NO by rotating sliding arc discharge reactor with conical-spiral electrodes
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作者 Bingyan CHEN Qi LIU +7 位作者 Xu LI Chunyang ZHANG Xiangbin GUO Qingzhou YU Zhicheng TANG Xiang HE Wei SU Yongfeng JIANG 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第9期97-108,共12页
The present work investigates the potential applications of nitrogen oxides(NO_(x)),particularly nitric oxide(NO)and nitrogen dioxide(NO_(2)),generated through discharge plasma in diverse sectors such as medicine,nitr... The present work investigates the potential applications of nitrogen oxides(NO_(x)),particularly nitric oxide(NO)and nitrogen dioxide(NO_(2)),generated through discharge plasma in diverse sectors such as medicine,nitrogen fixation,energy,and environmental protection.In this study,a rotating sliding arc discharge reactor was initially employed to produce high concentrations of gaseous NO_(x),followed by the utilization of a molybdenum wire redox reactor for NO_(2)-to-NO conversion.The outcomes reveal that the discharge states and generations of NO_(x) are affected by varying parameters,including the applied energies,frequencies and airflow states(1.3-2.6 m/s are the laminar flow,2.6-5.2 m/s are the transition state,5.2-6.5 m/s are the turbulent flow),and the concentrations of NO_(x) within the arc discharge are higher than that in the spark discharge.Moreover,the concentrations of NO,NO_(2) and NO_(x) gradually increased,and the concentration ratios of NO/NO_(2) and NO_(x)/NO_(2) decreased with increasing the applied energy for one cycle from 14.8 mJ to 24.3 mJ.Meanwhile,the concentrations of NO,NO_(2) and NO_(x) gradually decreased,and the concentration ratios of NO/NO_(2) and NO_(x)/NO_(2) first decreased and then increased with increasing the applied frequencies from 5.0 kHz to 9.0 kHz.Further,the concentrations of NO,NO_(2) and NO_(x) gradually decreased,and the concentration ratios of NO/NO_(2) and NO_(x)/NO_(2) first increased and then decreased with increasing the air flow speeds from 1.3 m/s to 6.5 m/s.Lastly,the concentrations of NO increased and NO_(2) decreased with increasing temperature from 25℃ to 400℃ using molybdenum converted.These findings provide experimental support for the application of plasma in the fields of medicine,nitrogen fixation,energy and environmental protection. 展开更多
关键词 rotating sliding arc discharge NO_(x) synthesis of NO redox reaction
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Effect of power supply parameters on discharge characteristics and sterilization efficiency of magnetically driven rotating gliding arc
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作者 Shaohua QIN Meizhi WANG +2 位作者 Jun DU Lanlan NIE Jie PAN 《Plasma Science and Technology》 SCIE EI CAS CSCD 2024年第9期61-68,共8页
Plasma sterilization is a new generation of high-tech sterilization method that is fast,safe,and pollution free.It is widely used in medical,food,and environmental protection fields.Home air sterilization is an emergi... Plasma sterilization is a new generation of high-tech sterilization method that is fast,safe,and pollution free.It is widely used in medical,food,and environmental protection fields.Home air sterilization is an emerging field of plasma application,which puts higher requirements on the miniaturization,operational stability,and operating cost of plasma device.In this study,a novel magnetically driven rotating gliding arc(MDRGA)discharge device was used to sterilize Lactobacillus fermentation.Compared with the traditional gas-driven gliding arc,this device has a simple structure and a more stable gliding arc.Simulation using COMSOL Multiphysics showed that adding permanent magnets can form a stable magnetic field,which is conducive to the formation of gliding arcs.Experiments on the discharge performance,ozone concentration,and sterilization effect were conducted using different power supply parameters.The results revealed that the MDRGA process can be divided into three stages:starting,gliding,and extinguishing.Appropriate voltage was the key factor for stable arc gliding,and both high and low voltages were not conducive to stable arc gliding and ozone production.In this experimental setup,the sterilization effect was the best at 6.6 kV.A high modulation duty ratio was beneficial for achieving stable arc gliding.However,when the duty ratio exceeded a certain value,the improvement in the sterilization effect was slow.Therefore,considering the sterilization effect and energy factors comprehensively,we chose 80%as the optimal modulation duty ratio for this experimental device. 展开更多
关键词 PLASMA magnetically driven rotating gliding arc STERILIZATION
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Evolution of magnetically rotating arc into large area arc plasma 被引量:3
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作者 王城 李皖皖 +2 位作者 张晓宁 査俊 夏维东 《Chinese Physics B》 SCIE EI CAS CSCD 2015年第6期429-432,共4页
An arc channel tends to shrink due to its conductivity increasing with the increase of temperature. In this study, to generate large area arc plasma, we construct a magnetically rotating arc plasma generator, which ma... An arc channel tends to shrink due to its conductivity increasing with the increase of temperature. In this study, to generate large area arc plasma, we construct a magnetically rotating arc plasma generator, which mainly consists of a lanthanide tungsten cathode (13 mm in diameter), a concentric cylindrical graphite anode chamber (60 nun in diameter) and a solenoid coil for producing an axial magnet field. By controlling the cold gas flow, the magnetically rotating arc evolves from constricted mode to diffuse mode, which almost fills the whole arc chamber cross section. Results show that the diffuse arc plasma has better uniformity and stability. The formation mechanism of large area arc plasma is discussed in this paper. 展开更多
关键词 magnetically rotating arc diffuse arc dispersed arc
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The characteristics of welding currents in a rotating arc leadtandem GMAW process and the weld-seam tracking 被引量:3
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作者 Gao Yanfeng Xiao Jianhua 《China Welding》 EI CAS 2017年第2期1-10,共10页
Tandem gas metal arc welding ( T-GMAW) process shows a high deposition rate that up to three times o f the single electrode GMAW, so the welding speed could be significantly increased in this process. H... Tandem gas metal arc welding ( T-GMAW) process shows a high deposition rate that up to three times o f the single electrode GMAW, so the welding speed could be significantly increased in this process. However, the majority o f this process applications are based on the pre-programmed robotic welding, which does not allow them to track the seam real-time during welding. Rotating arc sensor, sensing the seam position by detecting the changing of welding currents, has been widely adopted in the automatic robot welding process. It is proposed in this paper to integrate the rotating arc sensor with a trailing torch to develop a new approach of rotating arc lead tandem gas metal arc welding (RLT-GMAW) process. The characteristics of the welding currents in the proposed new welding process were firstly studied, and then a self-turning fuzzy control seam tracking strategy was developed for the mobile robot automatic welding. The experimental results showed that the proposed RLT-GMAW process had an excellent seam tracking performance and high welding deposition rate. Even if there were some electromagnetic interactions between the two arcs, the deviation of the welding seam could also be reflected by the fluctuation of the welding currents on the leading arc once the correct welding parameters were selected. Based on the detected deviation, the welding tracking experiments showed that the proposed self-turning fuzzy controller had a good performance for the RLT-GMAW process seam tracking. 展开更多
关键词 tandem gas metal arc welding rotating arc sensing welding seam tracking welding current characteristics
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Characteristics of Atmospheric Pressure Rotating Gliding Arc Plasmas 被引量:2
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作者 张浩 朱凤森 +3 位作者 屠昕 薄拯 岑可法 李晓东 《Plasma Science and Technology》 SCIE EI CAS CSCD 2016年第5期473-477,共5页
In this work, a novel direct current (DC) atmospheric pressure rotating gliding arc (RGA) plasma reactor has been developed for plasma-assisted chemical reactions. The influence of the gas composition and the gas ... In this work, a novel direct current (DC) atmospheric pressure rotating gliding arc (RGA) plasma reactor has been developed for plasma-assisted chemical reactions. The influence of the gas composition and the gas flow rate on the arc dynamic behaviour and the formation of reactive species in the N2 and air gliding arc plasmas has been investigated by means of electrical signals, high speed photography, and optical emission spectroscopic diagnostics. Compared to conventional gliding arc reactors with knife-shaped electrodes which generally require a high flow rate (e.g., 10-20 L/min) to maintain a long arc length and reasonable plasma discharge zone, in this RGA system, a lower gas flow rate (e.g., 2 L/min) can also generate a larger effective plasma reaction zone with a longer arc length for chemical reactions. Two different motion patterns can be clearly observed in the N2 and air RGA plasmas. The time-resolved arc voltage signals show that three different arc dynamic modes, the arc restrike mode, takeover mode, and combined modes, can be clearly identified in the RGA plasmas. The occurrence of different motion and arc dynamic modes is strongly dependent on the composition of the working gas and gas flow rate. 展开更多
关键词 rotating gliding arc (RGA) gas flow rate optical emission spectroscopy motion behavior electrical characteristics
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A modified heat source model for rotating arc welding 被引量:2
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作者 郭宁 韩焱飞 +1 位作者 张琳琳 邹妍 《China Welding》 EI CAS 2011年第3期57-62,共6页
A modified mathematical model of heat source for rotating arc welding (RAW) process was developed for investigating the heat and temperature distribution. The characteristics of temperature field based on the comple... A modified mathematical model of heat source for rotating arc welding (RAW) process was developed for investigating the heat and temperature distribution. The characteristics of temperature field based on the complex welding motion trajectory were studied. In this work, a transient three-dimensional ( 3D ) model was established and computed by a finite element analysis computer program MARC as well as its subroutine. In RA'W process, the temperature changes in the style of stepladder. Moreover in the high temperature zone, there are multiple peak temperature points. These characteristics of temperature distribution are induced by the arc rotating which leads the repetitive heating or fasing during the welding process. In contrast with non-rotating arc (NRAW) process, the width of temperature distribution enlarges, and the peak temperature of weld pool decreases. Good agreement is shown between the computed results and experimental results of thermal cycle in RAW process. 展开更多
关键词 rotating arc process temperature distribution finite element analysis
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Study on weld formation in a novel rotating arc horizontal GMAW 被引量:1
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作者 郭宁 林三宝 +2 位作者 范成磊 张亚奇 杨春利 《China Welding》 EI CAS 2009年第2期41-45,共5页
A novel rotating arc horizontal welding process was developed for solving the sagging of the molten pool which bottlenecks the application and the development of the horizontal welding. The principle of the effect of ... A novel rotating arc horizontal welding process was developed for solving the sagging of the molten pool which bottlenecks the application and the development of the horizontal welding. The principle of the effect of the rotating arc on the molten pool is that the rotating arc process not only can reduce the welding heat input by prolonging the welding path in the same welding distance cawed by the arc rotation, but also disperse the arc force to affect the sidewall periodically to support the molten metal near the upper sidewall. The effects of the rotating speed and arc voltage on the weld formation were studied. The results indicate that there is an appropriate range of the rotating speed and the arc voltage to obtain the defect free horizontal welding. 展开更多
关键词 rotating arc horizontal welding weld formation
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Dynamic behavior of a rotating gliding arc plasma in nitrogen:effects of gas flow rate and operating current 被引量:1
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作者 张浩 朱凤森 +1 位作者 李晓东 杜长明 《Plasma Science and Technology》 SCIE EI CAS CSCD 2017年第4期42-47,共6页
The effects of feed gas flow rate and operating current on the electrical characteristics and dynamic behavior of a rotating gliding arc (RGA) plasma codriven by a magnetic field and tangential flow were investigate... The effects of feed gas flow rate and operating current on the electrical characteristics and dynamic behavior of a rotating gliding arc (RGA) plasma codriven by a magnetic field and tangential flow were investigated.The operating current has been shown to significantly affect the time-resolved voltage waveforms of the discharge,particularly at flow rate =21 min^-1.When the current was lower than 140 mA,sinusoidal waveforms with regular variation periods of 13.5-17.0 ms can be observed (flow rate =21 min^-1).The restrike mode characterized by serial sudden drops of voltage appeared under all studied conditions.Increasing the flow rate from 8 to 121 min^-1 (at the same current) led to a shift of arc rotation mode which would then result in a significant drop of discharge voltage (around 120-200 V).For a given flow rate,the reduction of current resulted in a nearly linear increase of voltage. 展开更多
关键词 rotating gliding arc (RGA) electrical characteristics gas flow rate operating current rotation mode
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Sensitivity analysis of rotating flux-cored arc welding process parameters 被引量:1
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作者 石永华 刘翠霞 《China Welding》 EI CAS 2011年第4期40-45,共6页
Empirical models were developed using curvilinear regression analysis to predict bead geometries of rotating fluxcored are welding (FCAW). Parameters, such as rotational frequerwy, rotational radius, torch height an... Empirical models were developed using curvilinear regression analysis to predict bead geometries of rotating fluxcored are welding (FCAW). Parameters, such as rotational frequerwy, rotational radius, torch height and welding current, are used as design variables. The objective function is formed using bead width and penetration. Experiments of rotating FCAW were conducted based on orthogonal experimental design of four process parameters. A sensitivity analysis was also conducted and the effects of four process parameters on bead geometries were compared. The results show that the sensitivity of rotational radius on bead width is much higher than those of rotational frequency, torch height and welding current on bead width. Welding current is insensitive to bead width. The sensivity of rotational frequerwy on weld penetration is higher than those of other three parameters. 展开更多
关键词 rotating arc welding weld bead geometry sensitivity analysis
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Application of RVM for prediction of bead shape in underwater rotating arc welding
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作者 杜健辉 石永华 +1 位作者 王国荣 黄国兴 《China Welding》 EI CAS 2010年第4期40-43,共4页
Bead sttape in underwater rotating arc welding was affected by several welding parameters. RVM ( relevance vector machine) was used to build a model to predict weld bead shape. The training data set of RVM eortsists... Bead sttape in underwater rotating arc welding was affected by several welding parameters. RVM ( relevance vector machine) was used to build a model to predict weld bead shape. The training data set of RVM eortsists of the welding parameters which are rotational frequency, rotational radius, height of torch and welding current and the features of the bead shape. The maximum error and mean error for prediction of width are 0. 10 mm and 0. 09 mm, respectively, and the maximum error and mean error for prediction of penetration are 0. 31 mm and 0. 12mm, respectively, which are showed that the prediction model can achieve higher prediction precision at reasonably small size of training data set. 展开更多
关键词 underwater welding relevance vector machine prediction model rotating arc sensor
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Rotating arc horizontal narrow gap welding of high strength quenched and tempered steel
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作者 郭宁 杨春利 +3 位作者 韩焱飞 贾传宝 杜永鹏 张琳琳 《China Welding》 EI CAS 2010年第4期31-35,共5页
Rotating arc borizontal narrow gap welding of quenched & tempered (Q&T) steel was innovatively performed for solving the bottleneck that the molten pool sagged due to the gravity. The shapely multilayer single pas... Rotating arc borizontal narrow gap welding of quenched & tempered (Q&T) steel was innovatively performed for solving the bottleneck that the molten pool sagged due to the gravity. The shapely multilayer single pass horizontal joint could be obtairzed by using the rotating are welding process. The cold crack was not observed in the joint without controlling the heat input and selecting the consumables intentionally. Microstructure of the joint could be divided into three zones: base metal zone (BMZ) , heat-affected zone ( HAZ) and weld zone (WZ). Because of the characteristic of the rotating arc horizontal welding process, the defects in the joints were slag inclztsion formed at the interlayer of lower side wall. Tbe tensile strength and hardness of HAZ and WZ were larger than those of BMZ. The impact toughness in WZ, HAZ and BM at 0 % is equal to 11.5, 212 and 236 J, respectively. 展开更多
关键词 horizontal welding rotating arc quenched and tempered steel narrow gap welding
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Grain refinement and improved properties through electromagnetic stirring in Al alloy MIG welds 被引量:3
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作者 常云龙 杨旭 +1 位作者 车小平 李多 《China Welding》 EI CAS 2008年第3期77-80,共4页
This paper described the effects of external excitatory parameters of current and frequency on the microstructure and mechanical properties of weld metal in MIG welding with longitudinal electromagnetic field. With a ... This paper described the effects of external excitatory parameters of current and frequency on the microstructure and mechanical properties of weld metal in MIG welding with longitudinal electromagnetic field. With a high speed video camera capturing the images of arc shape, the mechanism of arc rotation and how the periodic contraction and expansion of arc affected the movement of molten pool were investigated. The technique resulted in fine equiaxed grains in weld metal and optimum parameters of electromagnetic stirring were suggested based on the extent of refinement. Fine-grained weld metal exhibited better yield strength and significant improvement in elongation. 展开更多
关键词 grain refinement shape of rotating arc electromagnetic stirring MIG welding
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Simulation of Arc Rotation and Its Effects on Pressure of Expansion Volume in an Auto-Expansion SF_6 Circuit Breaker 被引量:1
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作者 张俊民 迟程缤 +2 位作者 关永刚 刘卫东 吴军辉 《Plasma Science and Technology》 SCIE EI CAS CSCD 2016年第3期287-291,共5页
A 3D Magnetohydrodynamics (MHD) arc model in conjunction with an arc move- ment model is applied to simulate the arc rotation as well as to solve its effect on the pressure in an auto-expansion circuit breaker. The ... A 3D Magnetohydrodynamics (MHD) arc model in conjunction with an arc move- ment model is applied to simulate the arc rotation as well as to solve its effect on the pressure in an auto-expansion circuit breaker. The rotation of the arc driven by an external electromagnetic force is simulated in the case with 200 kA of the short circuit current and 16 ms of arc duration. The arc rotating process and the speed of arc rotation have been obtained in the simulation. A comparison of the pressure in the expansion volume with and without an external magnetic field has been carried out based on the calculation results of two cases. The results of the simulation reveal that the arc rotation, which causes more energy exchange between the arc and its sur- rounding gas, can evidently bring about the pressurization in the expansion volume, which would contribute to more effective arc quenching at current zero and further reducing operation power. 展开更多
关键词 SF6 circuit breaker 3D arc model external magnetic field arc rotation
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