Flow visualization was used to investigate experimentally the evolution process from symmetrical shedding to staggered shedding of the starting vortex and the phenomenon of secondary separation on an elliptic cylinder...Flow visualization was used to investigate experimentally the evolution process from symmetrical shedding to staggered shedding of the starting vortex and the phenomenon of secondary separation on an elliptic cylinder at moderate Reynolds numbers.The vortex structure of the flow separation was studied.The temporal variation of separation angle and length of wake vortex were given. The photographs and experimental results provided basis for further investigation of the complicated feature of the starting process of unsteady separated flows around an elliptic cylinder.展开更多
For a cyclone, it is possible to improve separation efficiency and reduce pressure drop by increasing the cyclone height. However, an exceeded height increase could result in a dramatical drop in separation efficiency...For a cyclone, it is possible to improve separation efficiency and reduce pressure drop by increasing the cyclone height. However, an exceeded height increase could result in a dramatical drop in separation efficiency. In this study, experimental and computational fluid dynamics simulation results exhibit that the introduction of an apex cone at the dust outlet could avoid the risk of separation efficiency drop but lead to a continuous reducing of the pressure drop. Generally, the optimal cyclone height should be closely related to the natural vortex length. While, when the vortex end contracts into the separation space in the cyclone with an exceeded height, severe back-mixing of particles always occurs, which will result in the decrease of separation efficiency. Herein, it is found that when an apex cone is installed at the dust outlet, the vortex end can be grasped by the cone so as to weaken the back-mixing of particles.Meanwhile, the introduction of this apex cone can enhance the secondary separation to capture the back-mixed particles again so as to protect the efficiency. In addition, it is found that the enhanced secondary separation could come from either the stagnant current of axial velocity in the center or the improved tangential velocity of inner vortex whereas the forcibly extending the length of vortex to exceed its natural length will not significantly increase efficiency.展开更多
A zeolitic imidazolate hybrid membrane(Co-IM-mIM) containing two imidazolate ligands deposited on a macroporous α-alumina support was prepared by pre-depositing and secondary growth technique. XRD, TGA and SEM charac...A zeolitic imidazolate hybrid membrane(Co-IM-mIM) containing two imidazolate ligands deposited on a macroporous α-alumina support was prepared by pre-depositing and secondary growth technique. XRD, TGA and SEM characterizations demonstrate that a stable and thin, but dense and pure-phase Co-IM-mIM membrane can be obtained on the macroporous-alumina discs in Teflon-lined autoclave at 120 °C after pre-depositing by dip-coating at room temperature. No visible cracks, pinholes or other defects were observed on the membrane layer. The gas separation studies of Co-IM-mIM membrane were carried out at 25 °C and 1×10~5 Pa, showing ideal selectivity of 6.95, 5.25, 3.40 for H_2/CO_2, H_2/N_2 and H_2/CH_4, respectively, and a permeance of 17.37× 10^(-6) mol/(m^2·s·Pa) for H_2. The influence of temperature and trans-membrane pressure on hydrogen separation and permeation was also carried out. The gas permeation and selectivity demonstrate that this membrane may have potential applications for efficient H_2 separation.展开更多
The funnel flow of high-temperature circulating ash and coal in moving bed with height restrictions directly influences the efficiency of coal pyrolysis and scale-up design of reactor.It is one of the technical bottle...The funnel flow of high-temperature circulating ash and coal in moving bed with height restrictions directly influences the efficiency of coal pyrolysis and scale-up design of reactor.It is one of the technical bottlenecks in the use of moving bed.In order to provide data support for the particle flow and pyrolysis model close to the actual working conditions in the future,this study describes the flow characteristics of solid-solid mixed particles in a cold two-dimensional moving bed.The results indicate that flow char-acteristics of mixed particles in the quartz sand-coal system are better than those in the cold circulating ash-coal system.The optimized conditions were obtained,the insert half angle is 20° and a heat carrier to coal ratio of 6:1.As the mixture progressed downstream,secondary separation of the heat carrier and coal become apparent.Furthermore,mixture residence time has been investigated to explore the relationship between regional residence time and to predict accurately the actual pyrolysis progress in pyrolyzer.展开更多
基金The project supported by the National Natural Science Foundation of China.
文摘Flow visualization was used to investigate experimentally the evolution process from symmetrical shedding to staggered shedding of the starting vortex and the phenomenon of secondary separation on an elliptic cylinder at moderate Reynolds numbers.The vortex structure of the flow separation was studied.The temporal variation of separation angle and length of wake vortex were given. The photographs and experimental results provided basis for further investigation of the complicated feature of the starting process of unsteady separated flows around an elliptic cylinder.
基金sponsored by the National Natural Science Foundation of China (21506139 and U1710101)。
文摘For a cyclone, it is possible to improve separation efficiency and reduce pressure drop by increasing the cyclone height. However, an exceeded height increase could result in a dramatical drop in separation efficiency. In this study, experimental and computational fluid dynamics simulation results exhibit that the introduction of an apex cone at the dust outlet could avoid the risk of separation efficiency drop but lead to a continuous reducing of the pressure drop. Generally, the optimal cyclone height should be closely related to the natural vortex length. While, when the vortex end contracts into the separation space in the cyclone with an exceeded height, severe back-mixing of particles always occurs, which will result in the decrease of separation efficiency. Herein, it is found that when an apex cone is installed at the dust outlet, the vortex end can be grasped by the cone so as to weaken the back-mixing of particles.Meanwhile, the introduction of this apex cone can enhance the secondary separation to capture the back-mixed particles again so as to protect the efficiency. In addition, it is found that the enhanced secondary separation could come from either the stagnant current of axial velocity in the center or the improved tangential velocity of inner vortex whereas the forcibly extending the length of vortex to exceed its natural length will not significantly increase efficiency.
基金Project(21376274)supported by the National Natural Science Foundation ChinaProject(2015BAL04B02)supported by the National Key Technology R&D Program of China
文摘A zeolitic imidazolate hybrid membrane(Co-IM-mIM) containing two imidazolate ligands deposited on a macroporous α-alumina support was prepared by pre-depositing and secondary growth technique. XRD, TGA and SEM characterizations demonstrate that a stable and thin, but dense and pure-phase Co-IM-mIM membrane can be obtained on the macroporous-alumina discs in Teflon-lined autoclave at 120 °C after pre-depositing by dip-coating at room temperature. No visible cracks, pinholes or other defects were observed on the membrane layer. The gas separation studies of Co-IM-mIM membrane were carried out at 25 °C and 1×10~5 Pa, showing ideal selectivity of 6.95, 5.25, 3.40 for H_2/CO_2, H_2/N_2 and H_2/CH_4, respectively, and a permeance of 17.37× 10^(-6) mol/(m^2·s·Pa) for H_2. The influence of temperature and trans-membrane pressure on hydrogen separation and permeation was also carried out. The gas permeation and selectivity demonstrate that this membrane may have potential applications for efficient H_2 separation.
基金supported by the National Natural Science Foundation of China(grant numbers:22078177,21776164,21376142)Natural Science Foundation of Shandong Province(grant number:ZR2020QB186).
文摘The funnel flow of high-temperature circulating ash and coal in moving bed with height restrictions directly influences the efficiency of coal pyrolysis and scale-up design of reactor.It is one of the technical bottlenecks in the use of moving bed.In order to provide data support for the particle flow and pyrolysis model close to the actual working conditions in the future,this study describes the flow characteristics of solid-solid mixed particles in a cold two-dimensional moving bed.The results indicate that flow char-acteristics of mixed particles in the quartz sand-coal system are better than those in the cold circulating ash-coal system.The optimized conditions were obtained,the insert half angle is 20° and a heat carrier to coal ratio of 6:1.As the mixture progressed downstream,secondary separation of the heat carrier and coal become apparent.Furthermore,mixture residence time has been investigated to explore the relationship between regional residence time and to predict accurately the actual pyrolysis progress in pyrolyzer.