This work reports spectroscopic studies of uranium containing plasma generated in air and argon environments. The 532 nm Q-switched Nd:YAG laser generates the optical breakdown plasma, which was recorded by a spectro...This work reports spectroscopic studies of uranium containing plasma generated in air and argon environments. The 532 nm Q-switched Nd:YAG laser generates the optical breakdown plasma, which was recorded by a spectrometer and an intensified charge coupled device having a resolution of 25 pm. Neutral and ionized uranium lines in the wavelength range of 385.8-391.9 nm indicate significant width and shift variations during the first few microseconds. Electron temperature and density of the plasma are determined using the Boltzmann plot and the Saha-Boltzmann equation at various time delay. The study reveals the power law decay pattern of electron temperature and density, which changes to exponential decay pattern if large gate- width is used to acquire the signal, due to an averaging effect.展开更多
基金supported by the fund obtained from DAE-BARC(ⅫPlan)
文摘This work reports spectroscopic studies of uranium containing plasma generated in air and argon environments. The 532 nm Q-switched Nd:YAG laser generates the optical breakdown plasma, which was recorded by a spectrometer and an intensified charge coupled device having a resolution of 25 pm. Neutral and ionized uranium lines in the wavelength range of 385.8-391.9 nm indicate significant width and shift variations during the first few microseconds. Electron temperature and density of the plasma are determined using the Boltzmann plot and the Saha-Boltzmann equation at various time delay. The study reveals the power law decay pattern of electron temperature and density, which changes to exponential decay pattern if large gate- width is used to acquire the signal, due to an averaging effect.