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Anomalous refinement and uniformization of grains in metallic thin films 被引量:1
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作者 Lei Wang Shu Wang +8 位作者 Xiaofeng Wang Jianming Zhang Jianjie Dong Bin Wei Haiguang Yang Zhongchang Wang Ziyang Zhang ChuanFei Guo Qian Liu 《Nano Research》 SCIE EI CSCD 2023年第12期13358-13365,共8页
When a laser beam writes on a metallic film,it usually coarsens and deuniformizes grains because of Ostwald ripening,similar to the case of annealing.Here we show an anomalous refinement effect of metal grains:A metal... When a laser beam writes on a metallic film,it usually coarsens and deuniformizes grains because of Ostwald ripening,similar to the case of annealing.Here we show an anomalous refinement effect of metal grains:A metallic silver film with large grains melts and breaks into uniform,close-packed,and ultrafine(~10 nm)grains by laser direct writing with a nanoscale laser spot size and nanosecond pulse that causes localized heating and adaptive shock-cooling.This method exhibits high controllability in both grain size and uniformity,which lies in a linear relationship between the film thickness(h)and grain size(D),D∝h.The linear relationship is significantly different from the classical spinodal dewetting theory obeying a nonlinear relationship(D∝h5/3)in common laser heating.We also demonstrate the application of such a silver film with a grain size of~10.9 nm as a surface-enhanced Raman scattering chip,exhibiting superhigh spatial-uniformity and low detection limit down to 10-15 M.This anomalous refinement effect is general and can be extended to many other metallic films. 展开更多
关键词 laser direct writing anomalous refinement localized heating RIPENING linear relationship
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Intrinsic two-dimensional multiferroicity in CrNCl_(2) monolayer 被引量:2
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作者 Wei Shen Yuanhui Pan +3 位作者 Shengnan Shen Hui Li Siyuan Nie Jie Mei 《Chinese Physics B》 SCIE EI CAS CSCD 2021年第11期570-574,共5页
Two-dimensional multiferroics,which simultaneously possess ferroelectricity and magnetism in a single phase,are well-known to possess great potential applications in nanoscale memories and spintronics.On the basis of ... Two-dimensional multiferroics,which simultaneously possess ferroelectricity and magnetism in a single phase,are well-known to possess great potential applications in nanoscale memories and spintronics.On the basis of first-principles calculations,a CrNCl_(2) monolayer is reported as an intrinsic multiferroic.The CrNCl_(2) has an antiferromagnetic ground state,with a N´eel temperature of about 88 K,and it exhibits an in-plane spontaneous polarization of 200 pC/m.The magnetic moments of CrNCl_(2) mainly come from the dxy orbital of the Cr cation,but the plane of the dxy orbital is perpendicular to the direction of the ferroelectric polarization,which hardly suppresses the occurrence of ferroelectricity.Therefore,the multiferroic exits in the CrNCl_(2).In addition,like CrNCl_(2),the CrNBr_(2) is an intrinsic multiferroic with antiferromagneticferroelectric ground state while CrNI_(2) is an intrinsic multiferroic with ferromagnetic-ferroelectric ground state.These findings enrich the multiferroics in the two-dimensional system and enable a wide range of applications in nanoscale devices. 展开更多
关键词 two-dimensional multiferroic CrNCl_(2)monolayer magnetism ferroelectricity
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Growth of 2D MoP single crystals on liquid metals by chemical vapor deposition
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作者 Feifei Cao Shuting Zheng +7 位作者 Jingjing Liang Zhi Li Bin Wei Yiran Ding Zhongchang Wang Mengqi Zeng Nan Xu Lei Fu 《Science China Materials》 SCIE EI CAS CSCD 2021年第5期1182-1188,共7页
Two-dimensional(2 D) transition metal phosphides(TMPs) are predicted with many novel properties and various applications. As a member of TMPs family, molybdenum phosphide(MoP) exhibits many exotic physicochemical prop... Two-dimensional(2 D) transition metal phosphides(TMPs) are predicted with many novel properties and various applications. As a member of TMPs family, molybdenum phosphide(MoP) exhibits many exotic physicochemical properties. However, the synthesis of high-quality2 D MoP single crystals is not reported due to the lack of reliable fabrication method, which limits the exploration of 2 D MoP. Here, we report the growth of high-quality ultrathin MoP single crystals with thickness down to 10 nm on liquid metals via chemical vapor deposition(CVD). The smooth surface of liquid Ga is regarded as a suitable growth substrate for producing 2 D MoP single crystals. The Mo source diffuses toward the Ga surface due to the high surface energy to react with phosphorus source, thus to fabricate ultrathin MoP single crystals. Then, we study the second harmonic generation(SHG) of 2 D MoP for the first time due to its intrinsic noncentrosymmetric structure. Our study provides an new approach to synthesize and explore other 2 D TMPs for future applications. 展开更多
关键词 2D materials transition metal phosphides molybdenum phosphides liquid metals chemical vapor deposition
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A nanoconcrete welding strategy for constructing high-performance wound dressing
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作者 Yingshuai Wang Yanxia Zhu +5 位作者 Penghe Zhao Bin Wei Mingjian Fan Danyang Chen Zhaokui Jin Qianjun He 《Bioactive Materials》 SCIE 2022年第8期31-41,共11页
Engineering biomaterials to meet specific biomedical applications raises high requirements of mechanical performances,and simultaneous strengthening and toughening of polymer are frequently necessary but very challeng... Engineering biomaterials to meet specific biomedical applications raises high requirements of mechanical performances,and simultaneous strengthening and toughening of polymer are frequently necessary but very challenging in many cases.In this work,we propose a new concept of nanoconcrete welding polymer chains,where mesoporous CaCO3(mCaCO_(3))nanoconcretes which are composed of amorphous and nanocrystalline phases are developed to powerfully weld polymer chains through siphoning-induced occlusion,hydration-driven crystallization and dehydration-driven compression of nanoconcretes.The mCaCO_(3) nanoconcrete welding technology is verified to be able to remarkably augment strength,toughness and anti-fatigue performances of a model polymer poly(3-hydroxybutyrate-co-3-hydroxyvalerate)-based porous membrane.Mechanistically,we have revealed polymer-occluded nanocrystal structure and welding-derived microstress which is much stronger than interfacial Van der Waals force,thus efficiently preventing the generation of microcracks and repairing initial microcracks by microcracks-induced hydration,crystallization and polymer welding of mCaCO_(3) nanoconcretes.Constructed porous membrane is used as wound dressing,exhibiting a special nanoplates-constructed surface topography as well as a porous structure with plentiful oriented,aligned and opened pore channels,improved hydrophilicity,water vapor permeability,anti-bacterial and cell adherence,in support of wound healing and skin structural/functional repairing.The proposed nanoconcrete-welding-polymer strategy breaks a new pathway for improving the mechanical performances of polymers. 展开更多
关键词 Tissue engineering Mechanical performances Calcium carbonate Mesoporous materials Organic/inorganic nanocomposite Wound dressing
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