Rational design of photocatalyst to maximize the use of sunlight is one of the issues to be solved in photocatalysis technology.In this study,the CuFe_(2)O_(4)@C/Cd_(0.9)Zn_(0.1)S(CFO@C/CZS)S-scheme photocatalyst with...Rational design of photocatalyst to maximize the use of sunlight is one of the issues to be solved in photocatalysis technology.In this study,the CuFe_(2)O_(4)@C/Cd_(0.9)Zn_(0.1)S(CFO@C/CZS)S-scheme photocatalyst with photothermal effect was synthesized by ultrasonic self-assembly combined with calcination.The dark CFO@C absorbed visible light and partly converted into heat to promote the hydrogen evolution reaction.The presence of heterojunctions inhibited the photogenerated electron-hole recombination.The graphite-carbon layer provided a stable channel for electron transfer,and the presence of magnetic CFO made recycle easier.Under the action of photothermal assistance and heterojunction,the hydrogen evolution rate of the optimal CFO@C/CZS was 80.79 mmol g^(-1) h^(-1),which was 2.55 times and 260.61 times of that of pure CZS and CFO@C,respectively.Notably,the composite samples also exhibit excellent stability and a wide range of environmental adaptability.Through experimental tests and first-principles simulation calculation methods,the plausible mechanism of photoactivity enhancement was proposed.This work provided a feasible strategy of photothermal assistance for the development of heterojunction photocatalysts with distinctive hydrogen evolution.展开更多
Majorana quantum computation offers a potential approach to securely manipulating and storing quantum data in a topological manner that may effectively resist the decoherence induced by local noise. However, actual Ma...Majorana quantum computation offers a potential approach to securely manipulating and storing quantum data in a topological manner that may effectively resist the decoherence induced by local noise. However, actual Majorana qubit setups are susceptible to noise. In this study, from a quantum dynamics perspective, we develop a noise model for Majorana qubits that accounts for quasi-particle poisoning and Majorana overlapping with fluctuation. Furthermore, we focus on Majorana parity readout methodologies, specifically those leveraging an ancillary quantum dot, and carry out an indepth exploration of continuous measurement techniques founded on the quantum jump model of a quantum point contact.Utilizing these methodologies, we proceed to analyze the influence of noise on the afore-mentioned noise model, employing numerical computation to evaluate the power spectrum and frequency curve. In the culmination of our study, we put forward a strategy to benchmark the presence and detailed properties of noise in Majorana qubits.展开更多
We study the exceptional-point(EP) structure and the associated quantum dynamics in a system consisting of a non-Hermitian qubit and a Hermitian qubit. We find that the system possesses two sets of EPs, which divide t...We study the exceptional-point(EP) structure and the associated quantum dynamics in a system consisting of a non-Hermitian qubit and a Hermitian qubit. We find that the system possesses two sets of EPs, which divide the systemparameter space into PT-symmetry unbroken, partially broken and fully broken regimes, each with distinct quantumdynamics characteristics. Particularly, in the partially broken regime, while the PT-symmetry is generally broken in the whole four-dimensional Hilbert space, it is preserved in a two-dimensional subspace such that the quantum dynamics in the subspace are similar to those in the PT-symmetry unbroken regime. In addition, we reveal that the competition between the inter-qubit coupling and the intra-qubit driving gives rise to a complex pattern in the EP variation with system parameters.展开更多
We study how can an angular momentum coherent state |τ> keeps its form-invariant during time evolution governed by the Hamiltonian H = f(t)J++ f^*(t)J-+ g(t)Jz. We discuss this topic in the context of boson realiz...We study how can an angular momentum coherent state |τ> keeps its form-invariant during time evolution governed by the Hamiltonian H = f(t)J++ f^*(t)J-+ g(t)Jz. We discuss this topic in the context of boson realization of |τ>. By employing the entangled state representation |ζ> and deriving a new binomial theorem involving two-subscript Hermite polynomials, we derive the wave function <ζ|τ>, which turns out to be a single-subscript Hermite polynomial. Based on this result the maintenance of angular momentum coherent state during time evolution is examined, and the value of τ(t) is totally determined by the parameters involved in the Hamiltonian.展开更多
To probe the behavior of hydrogen bonds in solid energetic materials, we conduct ReaxFF and SCC-DFTB molecular dynamics simulations of crystalline TATB, RDX, and DATB. By comparing the intra- and inter-molecular hydro...To probe the behavior of hydrogen bonds in solid energetic materials, we conduct ReaxFF and SCC-DFTB molecular dynamics simulations of crystalline TATB, RDX, and DATB. By comparing the intra- and inter-molecular hydrogen bond- ing rates, we find that the crystal structures are stabilized by inter-molecular hydrogen bond networks. Under high-pressure, the inter- and intra-molecular hydrogen bonds in solid TATB and DATB are nearly equivalent. The hydrogen bonds in solid TATB and DATB are much shorter than in solid RDX, which suggests strong hydrogen bond interactions existing in these energetic materials. Stretching of the C-H bond is observed in solid RDX, which may lead to further decomposition and even detonation.展开更多
Using the thermal-entangled state representation and the operator-ordering method, we investigate Wigner function(WF) for the squeezed negative binomial state(SNBS) and the analytical evolution law of density operator...Using the thermal-entangled state representation and the operator-ordering method, we investigate Wigner function(WF) for the squeezed negative binomial state(SNBS) and the analytical evolution law of density operator in the amplitude decay channel.The results show that the analytical WF is related to the square of the module of single-variable Hermite polynomials, which leads to a new two-variable special function and its generating function, and the parameters s and γplay opposite roles in the WF distributions.Besides, after undergoing this channel, the initial pure SNBS evolves into a new mixed state related to two operator Hermite polynomials within normal ordering, and fully loses its nonclassicality and decays to vacuum at long decay time.展开更多
By using the parameter differential method of operators,we recast the combination function of coordinate and momentum operators into its normal and anti-normal orderings,which is more ecumenical,simpler,and neater tha...By using the parameter differential method of operators,we recast the combination function of coordinate and momentum operators into its normal and anti-normal orderings,which is more ecumenical,simpler,and neater than the existing ways.These products are very useful in obtaining some new differential relations and useful mathematical integral formulas.Further,we derive the normally ordered form of the operator(fQ+gP)^-n with n being an arbitrary positive integer by using the parameter tracing method of operators together with the intermediate coordinate-momentum representation.In addition,general mutual transformation rules of the normal and anti-normal orderings,which have good universality,are derived and hence the anti-normal ordering of(fQ+gP)^-n is also obtained.Finally,the application of some new identities is given.展开更多
Using a swarm intelligence structure search method combining with first-principles calculations,three new structures of Zn-I and Hg-I compounds are discovered and pressure-composition phase diagrams are determined.An ...Using a swarm intelligence structure search method combining with first-principles calculations,three new structures of Zn-I and Hg-I compounds are discovered and pressure-composition phase diagrams are determined.An interesting phenomenon is found,that is,the compounds that are stable at 0 GPa in both systems will decompose into their constituent elements under certain pressure,which is contrary to the general intuition that pressure always makes materials more stability and density.A detailed analysis of the decomposition mechanism reveals the increase of formation enthalpy with the increase of pressure due to contributions from bothΔU andΔ[P V].Pressure-dependent studies of theΔV demonstrate that denser materials tend to be stabilized at higher pressures.Additionally,charge transfer calculations show that external pressure is more effective in regulating the ionic bond of Hg-I,resulting in a lower decomposition pressure for HgI_(2)than for ZnI_(2).These findings have important implications for designs and syntheses of new materials,as they challenge the conventional understanding on how pressure affects stability.展开更多
Effective path planning is crucial for mobile robots to quickly reach rescue destination and complete rescue tasks in a post-disaster scenario.In this study,we investigated the post-disaster rescue path planning probl...Effective path planning is crucial for mobile robots to quickly reach rescue destination and complete rescue tasks in a post-disaster scenario.In this study,we investigated the post-disaster rescue path planning problem and modeled this problem as a variant of the travel salesman problem(TSP)with life-strength constraints.To address this problem,we proposed an improved iterated greedy(IIG)algorithm.First,a push-forward insertion heuristic(PFIH)strategy was employed to generate a high-quality initial solution.Second,a greedy-based insertion strategy was designed and used in the destruction-construction stage to increase the algorithm’s exploration ability.Furthermore,three problem-specific swap operators were developed to improve the algorithm’s exploitation ability.Additionally,an improved simulated annealing(SA)strategy was used as an acceptance criterion to effectively prevent the algorithm from falling into local optima.To verify the effectiveness of the proposed algorithm,the Solomon dataset was extended to generate 27 instances for simulation.Finally,the proposed IIG was compared with five state-of-the-art algorithms.The parameter analysiswas conducted using the design of experiments(DOE)Taguchi method,and the effectiveness analysis of each component has been verified one by one.Simulation results indicate that IIGoutperforms the compared algorithms in terms of the number of rescue survivors and convergence speed,proving the effectiveness of the proposed algorithm.展开更多
The Cs_(2)NaInCl_(6) double perovskite is one of the most promising lead-free perovskites due to its exceptional stability and straightforward synthesis.However,it faces challenges related to inefficient photoluminesc...The Cs_(2)NaInCl_(6) double perovskite is one of the most promising lead-free perovskites due to its exceptional stability and straightforward synthesis.However,it faces challenges related to inefficient photoluminescence.Doping and high pressure are employed to tailor the optical properties of Cs_(2)NaInCl_(6).Herein,Sb^(3+)doped Cs_(2)NaInCl_(6)(Sb^(3+):Cs_(2)NaInCl_(6)) was synthesized and it exhibits blue emission with a photoluminescence quantum yield of up to 37.3%.Further,by employing pressure tuning,a blue stable emission under a very wide range from 2.7 GPa to 9.8 GPa is realized in Sb^(3+):Cs_(2)NaInCl_(6).Subsequently,the emission intensity of Sb^(3+):Cs_(2)NaInCl_(6) experiences a significant increase(3.3 times)at 19.0 GPa.It is revealed that the pressure-induced distinct emissions can be attributed to the carrier self-trapping and detrapping between Cs_(2)NaInCl_(6) and Sb^(3+).Notably,the lattice compression in the cubic phase inevitably modifies the band gap of Sb^(3+):Cs_(2)NaInCl_(6).Our findings provide valuable insights into effects of the high pressure in further boosting unique emission characteristics but also offer promising opportunities for development of doped double perovskites with enhanced optical functionalities.展开更多
Two-dimensional(2D)topological materials have recently garnered significant interest due to their profound physical properties and promising applications for future quantum nanoelectronics.Achieving various topologica...Two-dimensional(2D)topological materials have recently garnered significant interest due to their profound physical properties and promising applications for future quantum nanoelectronics.Achieving various topological states within one type of materials is,however,seldom reported.Based on first-principles calculations and tightbinding models,we investigate topological electronic states in a novel family of 2D halogenated tetragonal stanene(T-SnX,X=F,Cl,Br,I).All the four monolayers are found to be unusual topological nodal-line semimetals(NLSs),protected by a glide mirror symmetry.When spin-orbit coupling(SOC)is turned on,T-SnF and TSnCl are still ascertained as topological NLSs due to the remaining band inversion,primarily composed of Sn pxy orbitals,while T-Sn Br and T-SnI become quantum spin Hall insulators.The phase transition is ascribed to moving up in energy of Sn s orbitals and increasing of SOC strengths.The topology origin in the materials is uniformly rationalized through elementary band representations.The robust and diverse topological states found in the 2D T-SnX monolayers position them as an excellent material platform for development of innovative topological electronics.展开更多
We propose a density-matrix-formalism based scheme to study polarization mode dispersion(PMD)monitoring and compensation in optical fiber communication systems.Compared to traditional monitoring and compensation schem...We propose a density-matrix-formalism based scheme to study polarization mode dispersion(PMD)monitoring and compensation in optical fiber communication systems.Compared to traditional monitoring and compensation schemes based on the PMD vector in the Stokes space,the scheme we proposed requires no auxiliary matrices and can be handily extended to any higher-dimensional modal space,which is advantageous in mode-division multiplexing(MDM)systems.A 28 GBaud polarization division multiplexing quadrature phase-shift keying(PDM-QPSK)coherent simulation system is built to demonstrate that our scheme can implement the monitoring and compensation of 170 ps large differential-group-delay(DGD)that far exceeds the typical DGDs in practical optical communication systems.The results verify the effectiveness of the density-matrix-formalism based scheme in PMD monitoring and compensation,thus pave the way for further applications of the scheme in more general MDM optical communication systems.展开更多
Hydrogel is frequently used as a solid electrolyte for all solid-state supercapacitors(SCs)because of its liquid-like ion-transport property and high conformability.However,due to the higher water content,the hydrogel...Hydrogel is frequently used as a solid electrolyte for all solid-state supercapacitors(SCs)because of its liquid-like ion-transport property and high conformability.However,due to the higher water content,the hydrogel electrolyte undergoes inevitable freezing and/or dehydration with climate change.Herein,polypyrrole/carbon all-solid-state SCs(PCSCs)were developed based on a hierarchical polypyrrole/carbon nanotube electrode and a highly stretchable double-network polymer hydrogel electrolyte with LiCl/ethylene glycol as a mixed solvent.The PCSCs showed excellent electrochemical performance and cycle stability with a wide operating temperature.The specific capacitances could reach 202.2 and 112.3 mF cm^(−2) at current densities of 0.5 and 3.0 mA cm^(−2),respectively.Meanwhile,the PCSCs showed outstanding mechanical properties in maintaining a high areal capacitance under deformations of bending and tension.The excellent water retention of the device also ensured the stable electrochemical performance of PCSCs in a wide temperature range(30–80℃),which could potentially represent a reliable application in various harsh environments.展开更多
We solve the fermionic master equation for a thermal bath to obtain its explicit Kraus operator solutions via the fermionic state approach. The normalization condition of the Kraus operators is proved. The matrix repr...We solve the fermionic master equation for a thermal bath to obtain its explicit Kraus operator solutions via the fermionic state approach. The normalization condition of the Kraus operators is proved. The matrix representation for these solutions is obtained, which is incongruous with the result in the book completed by Nielsen and Chuang [Quan- tum Computation and Quantum Information, Cambridge University Press, 2000]. As especial cases, we also present the Kraus operator solutions to master equations for describing the amplitude-decay model and the diffusion process at finite temperature.展开更多
By extending the usual Weyl transformation to the s-parameterized Weyl transformation with s being a real parameter,we obtain the s-parameterized quantization scheme which includes P–Q quantization, Q–P quantization...By extending the usual Weyl transformation to the s-parameterized Weyl transformation with s being a real parameter,we obtain the s-parameterized quantization scheme which includes P–Q quantization, Q–P quantization, and Weyl ordering as its three special cases. Some operator identities can be derived directly by virtue of the s-parameterized quantization scheme.展开更多
The group V–VI semiconductor material getchellite (crystalline AsSbS_(3)) has garnered extensive attention due to itswonderful electronic and optical properties. The pressure engineering is one of the most effective ...The group V–VI semiconductor material getchellite (crystalline AsSbS_(3)) has garnered extensive attention due to itswonderful electronic and optical properties. The pressure engineering is one of the most effective methods to modulatecrystal structure and physical properties of semiconductor materials. In this study, the structural behavior, optical and electricalproperties of AsSbS_(3) under high pressure have been investigated systematically by in situ high-pressure experimentsfor the first time. The monoclinic structure of AsSbS_(3) remains stable up to 47.0 GPa without phase transition. The graduallattice contraction with increasing pressure results in a continuous narrowing of the bandgap then leads to pressure-inducedmetallization of AsSbS_(3) at 31.5 GPa. Our research presents a high-pressure strategy for tuning the crystal structure andphysical properties of AsSbS_(3) to expand its potential applications in electronic and optoelectronic fields.展开更多
We present a theoretical study of the influence of a single silver sphere on the fluorescence of radix angelica dahurica, which is a kind of traditional Chinese medicine. The enhancement factors of the excitation and ...We present a theoretical study of the influence of a single silver sphere on the fluorescence of radix angelica dahurica, which is a kind of traditional Chinese medicine. The enhancement factors of the excitation and the relaxation processes are deduced. The excitation can be enhanced more than 100 times at 315 nm. The enhancement factor of the emission can reach up to 9 at a center wavelength of 400 nm.展开更多
we preset the design and rabrication of a novel auai-iunction hign contrast gratings that can De usea as a polarizationselective beam splitter with transverse magnetic polarization,which performs two independent funct...we preset the design and rabrication of a novel auai-iunction hign contrast gratings that can De usea as a polarizationselective beam splitter with transverse magnetic polarization,which performs two independent functions,i.e.,reflection focusing and power equalization at a wavelength of 1550 nm.This dual-function grating profile is optimized by the rigorous coupled-wave analysis and the finite-element method.Simple analytical expressions of phase and modal guideline for the beam splitter design are given.The beam splitter based on the grating structure is experimentally studied at a distance of 160 μm from the reflection plane,the results are consistent with the theoretical results basically.展开更多
We investigate the Hugoniot curve, shock-particle velocity relations, and Chapman-Jouguet conditions of the hot dense system through molecular dynamics （MD） simulations. The detailed pathways from crystal nitrometha...We investigate the Hugoniot curve, shock-particle velocity relations, and Chapman-Jouguet conditions of the hot dense system through molecular dynamics （MD） simulations. The detailed pathways from crystal nitromethane to reacted state by shock compression are simulated. The phase transition of N2 and CO mixture is found at about 10 GPa, and the main reason is that the dissociation of the C-O bond and the formation of C-C bond start at 10.0-11.0 GPa. The unreacted state simulations of nitromethane are consistent with shock Hugoniot data. The complete pathway from unreacted to reacted state is discussed. Through chemical species analysis, we find that the C-N bond breaking is the main event of the shock-induced nitromethane decomposition.展开更多
We theoretically introduce two new photon-modulated atomic coherent states(ACSs)via using the Schwinger bosonic representation of the angular momentum operators(the sequential operations J±n)on an ACS,and investi...We theoretically introduce two new photon-modulated atomic coherent states(ACSs)via using the Schwinger bosonic representation of the angular momentum operators(the sequential operations J±n)on an ACS,and investigate their nonclassicality using the Wigner distribution,photon number distribution,and entanglement entropy.It is found that photonmodulated ACSs possess more stronger nonclassicality than the original ACS in certain regions ofτ,the nonclassicality enhances with increasing number n of the operations J±and the operation J+(-)n enhances the entanglement in the region of small(large)τ.展开更多
基金supported by the Shandong Provincial Natural Science Foundation(ZR2022ME179,ZR2021QE086)the Shandong Provincial Key Research and Development Program(Public Welfare Science and Technology Research)(2019GGX103010)+2 种基金the Science and Technology Planning Project of Higher School in Shandong Province(J18KA243)the Liaocheng Key Research and Development Program(Policy guidance category)(2022YDSF90)the Liaocheng University High-level Talents&PhD Research Startup Foundation(318051619)。
文摘Rational design of photocatalyst to maximize the use of sunlight is one of the issues to be solved in photocatalysis technology.In this study,the CuFe_(2)O_(4)@C/Cd_(0.9)Zn_(0.1)S(CFO@C/CZS)S-scheme photocatalyst with photothermal effect was synthesized by ultrasonic self-assembly combined with calcination.The dark CFO@C absorbed visible light and partly converted into heat to promote the hydrogen evolution reaction.The presence of heterojunctions inhibited the photogenerated electron-hole recombination.The graphite-carbon layer provided a stable channel for electron transfer,and the presence of magnetic CFO made recycle easier.Under the action of photothermal assistance and heterojunction,the hydrogen evolution rate of the optimal CFO@C/CZS was 80.79 mmol g^(-1) h^(-1),which was 2.55 times and 260.61 times of that of pure CZS and CFO@C,respectively.Notably,the composite samples also exhibit excellent stability and a wide range of environmental adaptability.Through experimental tests and first-principles simulation calculation methods,the plausible mechanism of photoactivity enhancement was proposed.This work provided a feasible strategy of photothermal assistance for the development of heterojunction photocatalysts with distinctive hydrogen evolution.
基金supported by the Innovation Program for Quantum Science and Technology (Grant No.2021ZD0302400)the National Natural Science Foundation of China (Grants No.11974198)the Natural Science Foundation of Shandong Province of China (Grant No.ZR2021MA091)。
文摘Majorana quantum computation offers a potential approach to securely manipulating and storing quantum data in a topological manner that may effectively resist the decoherence induced by local noise. However, actual Majorana qubit setups are susceptible to noise. In this study, from a quantum dynamics perspective, we develop a noise model for Majorana qubits that accounts for quasi-particle poisoning and Majorana overlapping with fluctuation. Furthermore, we focus on Majorana parity readout methodologies, specifically those leveraging an ancillary quantum dot, and carry out an indepth exploration of continuous measurement techniques founded on the quantum jump model of a quantum point contact.Utilizing these methodologies, we proceed to analyze the influence of noise on the afore-mentioned noise model, employing numerical computation to evaluate the power spectrum and frequency curve. In the culmination of our study, we put forward a strategy to benchmark the presence and detailed properties of noise in Majorana qubits.
基金partly funded by the Natural Science Foundation of Shandong Province of China (Grant Nos. ZR2021MA091 and ZR2018MA044)Introduction and Cultivation Plan of Youth Innovation Talents for Universities of Shandong Province (Research and Innovation Team on Materials Modification and Optoelectronic Devices at extreme conditions)。
文摘We study the exceptional-point(EP) structure and the associated quantum dynamics in a system consisting of a non-Hermitian qubit and a Hermitian qubit. We find that the system possesses two sets of EPs, which divide the systemparameter space into PT-symmetry unbroken, partially broken and fully broken regimes, each with distinct quantumdynamics characteristics. Particularly, in the partially broken regime, while the PT-symmetry is generally broken in the whole four-dimensional Hilbert space, it is preserved in a two-dimensional subspace such that the quantum dynamics in the subspace are similar to those in the PT-symmetry unbroken regime. In addition, we reveal that the competition between the inter-qubit coupling and the intra-qubit driving gives rise to a complex pattern in the EP variation with system parameters.
基金Project supported by the National Natural Science Foundation of China(Grant No.11347026)the Natural Science Foundation of Shandong Province,China(Grant Nos.ZR2016AM03 and ZR2017MA011)
文摘We study how can an angular momentum coherent state |τ> keeps its form-invariant during time evolution governed by the Hamiltonian H = f(t)J++ f^*(t)J-+ g(t)Jz. We discuss this topic in the context of boson realization of |τ>. By employing the entangled state representation |ζ> and deriving a new binomial theorem involving two-subscript Hermite polynomials, we derive the wave function <ζ|τ>, which turns out to be a single-subscript Hermite polynomial. Based on this result the maintenance of angular momentum coherent state during time evolution is examined, and the value of τ(t) is totally determined by the parameters involved in the Hamiltonian.
基金Project supported by the National Natural Science Foundation of China(Grant No.11176020)the Fund from the China Academy of Engineering Physics,China(Grant No.2011A0302014)
文摘To probe the behavior of hydrogen bonds in solid energetic materials, we conduct ReaxFF and SCC-DFTB molecular dynamics simulations of crystalline TATB, RDX, and DATB. By comparing the intra- and inter-molecular hydrogen bond- ing rates, we find that the crystal structures are stabilized by inter-molecular hydrogen bond networks. Under high-pressure, the inter- and intra-molecular hydrogen bonds in solid TATB and DATB are nearly equivalent. The hydrogen bonds in solid TATB and DATB are much shorter than in solid RDX, which suggests strong hydrogen bond interactions existing in these energetic materials. Stretching of the C-H bond is observed in solid RDX, which may lead to further decomposition and even detonation.
基金Project supported by the National Natural Science Foundation of China(Grant No.11347026)the Natural Science Foundation of Shandong Province,China(Grant Nos.ZR2016AM03 and ZR2017MA011)
文摘Using the thermal-entangled state representation and the operator-ordering method, we investigate Wigner function(WF) for the squeezed negative binomial state(SNBS) and the analytical evolution law of density operator in the amplitude decay channel.The results show that the analytical WF is related to the square of the module of single-variable Hermite polynomials, which leads to a new two-variable special function and its generating function, and the parameters s and γplay opposite roles in the WF distributions.Besides, after undergoing this channel, the initial pure SNBS evolves into a new mixed state related to two operator Hermite polynomials within normal ordering, and fully loses its nonclassicality and decays to vacuum at long decay time.
基金Project supported by the National Natural Science Foundation of China(Grant No.11347026)the Natural Science Foundation of Shandong Province,China(Grant Nos.ZR2016AM03 and ZR2017MA011)the Natural Science Foundation of Heze University,China(Grant Nos.XY17KJ09 and XY18PY13).
文摘By using the parameter differential method of operators,we recast the combination function of coordinate and momentum operators into its normal and anti-normal orderings,which is more ecumenical,simpler,and neater than the existing ways.These products are very useful in obtaining some new differential relations and useful mathematical integral formulas.Further,we derive the normally ordered form of the operator(fQ+gP)^-n with n being an arbitrary positive integer by using the parameter tracing method of operators together with the intermediate coordinate-momentum representation.In addition,general mutual transformation rules of the normal and anti-normal orderings,which have good universality,are derived and hence the anti-normal ordering of(fQ+gP)^-n is also obtained.Finally,the application of some new identities is given.
基金supported by the National Natural Science Foundation of China(Grant Nos.11974154,11604133,and 11874318)the Taishan Scholars Special Funding for Construction Projectsthe Natural Science Foundation of Shandong Province(Grant No.ZR2022MA023)。
文摘Using a swarm intelligence structure search method combining with first-principles calculations,three new structures of Zn-I and Hg-I compounds are discovered and pressure-composition phase diagrams are determined.An interesting phenomenon is found,that is,the compounds that are stable at 0 GPa in both systems will decompose into their constituent elements under certain pressure,which is contrary to the general intuition that pressure always makes materials more stability and density.A detailed analysis of the decomposition mechanism reveals the increase of formation enthalpy with the increase of pressure due to contributions from bothΔU andΔ[P V].Pressure-dependent studies of theΔV demonstrate that denser materials tend to be stabilized at higher pressures.Additionally,charge transfer calculations show that external pressure is more effective in regulating the ionic bond of Hg-I,resulting in a lower decomposition pressure for HgI_(2)than for ZnI_(2).These findings have important implications for designs and syntheses of new materials,as they challenge the conventional understanding on how pressure affects stability.
基金supported by the Opening Fund of Shandong Provincial Key Laboratory of Network based Intelligent Computing,the National Natural Science Foundation of China(52205529,61803192)the Natural Science Foundation of Shandong Province(ZR2021QE195)+1 种基金the Youth Innovation Team Program of Shandong Higher Education Institution(2023KJ206)the Guangyue Youth Scholar Innovation Talent Program support received from Liaocheng University(LCUGYTD2022-03).
文摘Effective path planning is crucial for mobile robots to quickly reach rescue destination and complete rescue tasks in a post-disaster scenario.In this study,we investigated the post-disaster rescue path planning problem and modeled this problem as a variant of the travel salesman problem(TSP)with life-strength constraints.To address this problem,we proposed an improved iterated greedy(IIG)algorithm.First,a push-forward insertion heuristic(PFIH)strategy was employed to generate a high-quality initial solution.Second,a greedy-based insertion strategy was designed and used in the destruction-construction stage to increase the algorithm’s exploration ability.Furthermore,three problem-specific swap operators were developed to improve the algorithm’s exploitation ability.Additionally,an improved simulated annealing(SA)strategy was used as an acceptance criterion to effectively prevent the algorithm from falling into local optima.To verify the effectiveness of the proposed algorithm,the Solomon dataset was extended to generate 27 instances for simulation.Finally,the proposed IIG was compared with five state-of-the-art algorithms.The parameter analysiswas conducted using the design of experiments(DOE)Taguchi method,and the effectiveness analysis of each component has been verified one by one.Simulation results indicate that IIGoutperforms the compared algorithms in terms of the number of rescue survivors and convergence speed,proving the effectiveness of the proposed algorithm.
基金supported by the National Key Research and Development Program of China(Grant Nos.2021YFA1400200 and2021YFA0718701)the National Natural Science Foundation of China(Grant Nos.U2032127,11904322,12104411,12174347)+4 种基金the Natural Science Foundation of Henan province of China(Grant No.202300410356)the China Postdoctoral Science Foundation(Grant Nos.2019M652560 and 2020M682326)the CAS Interdisciplinary Innovation Team(Grant No.JCTD-2019-01)the Postdoctoral Research Grant in Henan Province(Grant No.1902013)the Science Foundation for Highlevel Talents of Wuyi University(Grant No.2021AL019)。
文摘The Cs_(2)NaInCl_(6) double perovskite is one of the most promising lead-free perovskites due to its exceptional stability and straightforward synthesis.However,it faces challenges related to inefficient photoluminescence.Doping and high pressure are employed to tailor the optical properties of Cs_(2)NaInCl_(6).Herein,Sb^(3+)doped Cs_(2)NaInCl_(6)(Sb^(3+):Cs_(2)NaInCl_(6)) was synthesized and it exhibits blue emission with a photoluminescence quantum yield of up to 37.3%.Further,by employing pressure tuning,a blue stable emission under a very wide range from 2.7 GPa to 9.8 GPa is realized in Sb^(3+):Cs_(2)NaInCl_(6).Subsequently,the emission intensity of Sb^(3+):Cs_(2)NaInCl_(6) experiences a significant increase(3.3 times)at 19.0 GPa.It is revealed that the pressure-induced distinct emissions can be attributed to the carrier self-trapping and detrapping between Cs_(2)NaInCl_(6) and Sb^(3+).Notably,the lattice compression in the cubic phase inevitably modifies the band gap of Sb^(3+):Cs_(2)NaInCl_(6).Our findings provide valuable insights into effects of the high pressure in further boosting unique emission characteristics but also offer promising opportunities for development of doped double perovskites with enhanced optical functionalities.
基金supported by the National Natural Science Foundation of China(Grant Nos.12174059,11874117,11904101,and 11604134)the Natural Science Foundation of Shanghai(Grant No.21ZR140820)。
文摘Two-dimensional(2D)topological materials have recently garnered significant interest due to their profound physical properties and promising applications for future quantum nanoelectronics.Achieving various topological states within one type of materials is,however,seldom reported.Based on first-principles calculations and tightbinding models,we investigate topological electronic states in a novel family of 2D halogenated tetragonal stanene(T-SnX,X=F,Cl,Br,I).All the four monolayers are found to be unusual topological nodal-line semimetals(NLSs),protected by a glide mirror symmetry.When spin-orbit coupling(SOC)is turned on,T-SnF and TSnCl are still ascertained as topological NLSs due to the remaining band inversion,primarily composed of Sn pxy orbitals,while T-Sn Br and T-SnI become quantum spin Hall insulators.The phase transition is ascribed to moving up in energy of Sn s orbitals and increasing of SOC strengths.The topology origin in the materials is uniformly rationalized through elementary band representations.The robust and diverse topological states found in the 2D T-SnX monolayers position them as an excellent material platform for development of innovative topological electronics.
基金supported by the National Natural Science Foundation of China(No.61501214)the Natural Science Foundation of Shandong Province(Nos.ZR2022MF284 and ZR2018MA044).
文摘We propose a density-matrix-formalism based scheme to study polarization mode dispersion(PMD)monitoring and compensation in optical fiber communication systems.Compared to traditional monitoring and compensation schemes based on the PMD vector in the Stokes space,the scheme we proposed requires no auxiliary matrices and can be handily extended to any higher-dimensional modal space,which is advantageous in mode-division multiplexing(MDM)systems.A 28 GBaud polarization division multiplexing quadrature phase-shift keying(PDM-QPSK)coherent simulation system is built to demonstrate that our scheme can implement the monitoring and compensation of 170 ps large differential-group-delay(DGD)that far exceeds the typical DGDs in practical optical communication systems.The results verify the effectiveness of the density-matrix-formalism based scheme in PMD monitoring and compensation,thus pave the way for further applications of the scheme in more general MDM optical communication systems.
基金NSF of Jiangsu Province,Grant/Award Number:BK20190688NSF of Jiangsu Higher Education Institutions,Grant/Award Number:21KJB430039+1 种基金NSF of Shandong Province,Grant/Award Number:ZR2020KB018Taishan Scholars”Construction Special Fund of Shandong Province,and the Industrial Alliance Fund of Shandong Provincial Key Laboratory,Grant/Award Number:SDKL016038。
文摘Hydrogel is frequently used as a solid electrolyte for all solid-state supercapacitors(SCs)because of its liquid-like ion-transport property and high conformability.However,due to the higher water content,the hydrogel electrolyte undergoes inevitable freezing and/or dehydration with climate change.Herein,polypyrrole/carbon all-solid-state SCs(PCSCs)were developed based on a hierarchical polypyrrole/carbon nanotube electrode and a highly stretchable double-network polymer hydrogel electrolyte with LiCl/ethylene glycol as a mixed solvent.The PCSCs showed excellent electrochemical performance and cycle stability with a wide operating temperature.The specific capacitances could reach 202.2 and 112.3 mF cm^(−2) at current densities of 0.5 and 3.0 mA cm^(−2),respectively.Meanwhile,the PCSCs showed outstanding mechanical properties in maintaining a high areal capacitance under deformations of bending and tension.The excellent water retention of the device also ensured the stable electrochemical performance of PCSCs in a wide temperature range(30–80℃),which could potentially represent a reliable application in various harsh environments.
基金supported by the National Natural Science Foundation of China(Grant No.11347026)the Natural Science Foundation of Shandong Province+1 种基金China(Grant Nos.ZR2013AM012 and ZR2012AM004)the Research Fund for the Doctoral Program and Scientific Research Project of Liaocheng University,Shandong Province,China
文摘We solve the fermionic master equation for a thermal bath to obtain its explicit Kraus operator solutions via the fermionic state approach. The normalization condition of the Kraus operators is proved. The matrix representation for these solutions is obtained, which is incongruous with the result in the book completed by Nielsen and Chuang [Quan- tum Computation and Quantum Information, Cambridge University Press, 2000]. As especial cases, we also present the Kraus operator solutions to master equations for describing the amplitude-decay model and the diffusion process at finite temperature.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11147009,11347026,and 11244005)the Natural Science Foundation of Shandong Province,China(Grant Nos.ZR2013AM012 and ZR2012AM004)the Natural Science Foundation of Liaocheng University,China
文摘By extending the usual Weyl transformation to the s-parameterized Weyl transformation with s being a real parameter,we obtain the s-parameterized quantization scheme which includes P–Q quantization, Q–P quantization, and Weyl ordering as its three special cases. Some operator identities can be derived directly by virtue of the s-parameterized quantization scheme.
基金Project supported by the National Natural Science Foundation of China(Grant No.42274123)the Special Construction Project Fund for Shandong Provincial Taishan Scholars.
文摘The group V–VI semiconductor material getchellite (crystalline AsSbS_(3)) has garnered extensive attention due to itswonderful electronic and optical properties. The pressure engineering is one of the most effective methods to modulatecrystal structure and physical properties of semiconductor materials. In this study, the structural behavior, optical and electricalproperties of AsSbS_(3) under high pressure have been investigated systematically by in situ high-pressure experimentsfor the first time. The monoclinic structure of AsSbS_(3) remains stable up to 47.0 GPa without phase transition. The graduallattice contraction with increasing pressure results in a continuous narrowing of the bandgap then leads to pressure-inducedmetallization of AsSbS_(3) at 31.5 GPa. Our research presents a high-pressure strategy for tuning the crystal structure andphysical properties of AsSbS_(3) to expand its potential applications in electronic and optoelectronic fields.
基金supported by the National Natural Science Foundation of China(Grant Nos.61405085 and 61275147)the Research Fund for the Doctoral Program of Liaocheng University,China+1 种基金the Key Project of Science and Technology of Shandong Province of China(Grant No.2010GGX10127)the Shandong Province Natural Science Foundation of China(Grant Nos.ZR2013EML006 and ZR2012AL11)
文摘We present a theoretical study of the influence of a single silver sphere on the fluorescence of radix angelica dahurica, which is a kind of traditional Chinese medicine. The enhancement factors of the excitation and the relaxation processes are deduced. The excitation can be enhanced more than 100 times at 315 nm. The enhancement factor of the emission can reach up to 9 at a center wavelength of 400 nm.
基金Project supported by the Open Fund of the State Key Laboratory of Information Photonics and Optical CommunicationBeijing University of Posts and Telecommunications,China(Grant No.IPOC2019A009)the National Natural Science Foundation of China(Grant Nos.61501214 and 61501213)。
文摘we preset the design and rabrication of a novel auai-iunction hign contrast gratings that can De usea as a polarizationselective beam splitter with transverse magnetic polarization,which performs two independent functions,i.e.,reflection focusing and power equalization at a wavelength of 1550 nm.This dual-function grating profile is optimized by the rigorous coupled-wave analysis and the finite-element method.Simple analytical expressions of phase and modal guideline for the beam splitter design are given.The beam splitter based on the grating structure is experimentally studied at a distance of 160 μm from the reflection plane,the results are consistent with the theoretical results basically.
基金supported by the National Natural Science Foundation of China(Grant No.11374217)the Shandong Provincial Natural Science Foundation,China(Grant No.ZR2014BQ008)
文摘We investigate the Hugoniot curve, shock-particle velocity relations, and Chapman-Jouguet conditions of the hot dense system through molecular dynamics （MD） simulations. The detailed pathways from crystal nitromethane to reacted state by shock compression are simulated. The phase transition of N2 and CO mixture is found at about 10 GPa, and the main reason is that the dissociation of the C-O bond and the formation of C-C bond start at 10.0-11.0 GPa. The unreacted state simulations of nitromethane are consistent with shock Hugoniot data. The complete pathway from unreacted to reacted state is discussed. Through chemical species analysis, we find that the C-N bond breaking is the main event of the shock-induced nitromethane decomposition.
基金Project supported by the National Natural Science Foundation of China(Grant No.11347026)the Natural Science Foundation of Shandong Province,China(Grant Nos.ZR2016AM03 and ZR2017MA011)。
文摘We theoretically introduce two new photon-modulated atomic coherent states(ACSs)via using the Schwinger bosonic representation of the angular momentum operators(the sequential operations J±n)on an ACS,and investigate their nonclassicality using the Wigner distribution,photon number distribution,and entanglement entropy.It is found that photonmodulated ACSs possess more stronger nonclassicality than the original ACS in certain regions ofτ,the nonclassicality enhances with increasing number n of the operations J±and the operation J+(-)n enhances the entanglement in the region of small(large)τ.
