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Design and performance study of a dielectric-filled cavity beam current monitor for HUST-PTF
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作者 Ji-Qing Li Kuan-Jun Fan +3 位作者 Zheng-Zheng Liu Jian Wang Qu-Shan Chen Jin-Feng Yang 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2023年第8期75-85,共11页
To guarantee the exact proton dose applied to patients and ensure treatment safety while disrupting and destroying tumor cells,it is essential to accurately monitor the proton beam current in real time during patient ... To guarantee the exact proton dose applied to patients and ensure treatment safety while disrupting and destroying tumor cells,it is essential to accurately monitor the proton beam current in real time during patient treatment.Because clinical treatment requires a proton beam current in the∼nA range,nondestructive beam current monitors(BCMs)are preferred to minimize the degradation of beam quality.However,this poses significant challenges in accurately monitoring such extremely low beam intensities.This study proposes a cavity-type BCM equipped with a dielectric plate to reduce its dimensions and achieve sufficient measurement sensitivity for practical requirements.A prototype cavity BCM was fabricated,and off-line testing was performed using a metal wire to simulate the beam to study its performance.Both the simulation and experi-mental results showed that the cavity BCM could measure ultralow proton beam currents with a resolution up to 0.03 nA. 展开更多
关键词 Proton therapy Beam current Cavity BCM NONDESTRUCTIVE
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Effect of PEGylation on the physicochemical and pharmacokinetic characteristics of bovine serum albumin-encapsulated liposome 被引量:2
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作者 Yuko Okamoto Kazuaki Taguchi +3 位作者 Keishi Yamasaki Mina Sakuragi Shun’ichi Kuroda Masaki Otagiri 《Asian Journal of Pharmaceutical Sciences》 SCIE CAS 2016年第1期112-113,共2页
There is now little doubt that PEGylation is useful and is in widespread use because it provides a prolonged half-life,a higher stability and a lowerimmunogenicity[1].However,it is of concern that PEGylation may affec... There is now little doubt that PEGylation is useful and is in widespread use because it provides a prolonged half-life,a higher stability and a lowerimmunogenicity[1].However,it is of concern that PEGylation may affect the physicochemical and pharmacokinetic characteristics of protein-encapsulated liposome.Thus,we prepared the bovine serum albumin(BSA)-encapsulated liposome(BSA-liposome)with or without PEG and then compared their physicochemical and pharmacokinetic characteristics(Fig.1).BSA-liposomes were prepared by the thin-film hydration method. 展开更多
关键词 LIPOSOME PEGYLATION BOVINE serum ALBUMIN
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Understanding of the activity difference between nanogold and bulk gold by relativistic effects 被引量:1
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作者 Keju Sun Masanori Kohyama +1 位作者 Shingo Tanaka Seiji Takeda 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2015年第4期485-489,共5页
It is a challenge to thoroughly understand the astonishing difference in catalytic activity between nanogold and bulk gold for some oxidation reactions. In this work,the Au–O interactions in various surroundings were... It is a challenge to thoroughly understand the astonishing difference in catalytic activity between nanogold and bulk gold for some oxidation reactions. In this work,the Au–O interactions in various surroundings were investigated by DFT calculations and compared with the Ag–O interactions. We have found the three points.First,only Au–O bond can be significantly strengthened by the linear O–Au–O structure. Second,the Au–O bond is always stronger than the Ag–O bond when the bonds are embedded in common surroundings. Third,the Au–O bond becomes weaker than the Ag–O bond when the number of neighboring Au atoms becomes large,because the Au–O interactions are suppressed by the presence of neighboring gold atoms. The origin of these three points can be attributed to wider spatial extension of d orbitals of gold,induced by strong relativistic effects. The strong relativistic effects make nanogold with smaller coordinate numbers highly active due to the ease in forming strong Au–O bonds,especially for the O–Au–O bond,whereas gold atoms in bulk with larger coordination numbers chemically inert due to the strong suppression by neighboring gold atoms destabilizing the O–Au–O bond. 展开更多
关键词 NANOGOLD Au–O interactions Relativistic effects DFT calculations
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The Surface Coating of Commercial LiFePO_4 by Utilizing ZIF-8 for High Electrochemical Performance Lithium Ion Battery 被引量:10
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作者 XiaoLong Xu CongYu Qi +5 位作者 ZhenDong Hao Hao Wang JinTing Jiu JingBing Liu Hui Yan Katsuaki Suganuma 《Nano-Micro Letters》 SCIE EI CAS 2018年第1期3-11,共9页
The requirement of energy-storage equipment needs to develop the lithium ion battery(LIB) with high electrochemical performance. The surface modification of commercial LiFePO_4(LFP) by utilizing zeolitic imidazolate f... The requirement of energy-storage equipment needs to develop the lithium ion battery(LIB) with high electrochemical performance. The surface modification of commercial LiFePO_4(LFP) by utilizing zeolitic imidazolate frameworks-8(ZIF-8) offers new possibilities for commercial LFP with high electrochemical performances.In this work, the carbonized ZIF-8(C_(ZIF-8)) was coated on the surface of LFP particles by the in situ growth and carbonization of ZIF-8. Transmission electron microscopy indicates that there is an approximate 10 nm coating layer with metal zinc and graphite-like carbon on the surface of LFP/C_(ZIF-8) sample. The N_2 adsorption and desorptionisotherm suggests that the coating layer has uniform and simple connecting mesopores. As cathode material, LFP/C_(ZIF-8) cathode-active material delivers a discharge specific capacity of 159.3 m Ah g^(-1) at 0.1 C and a discharge specific energy of 141.7 m Wh g^(-1) after 200 cycles at 5.0 C(the retention rate is approximate 99%). These results are attributed to the synergy improvement of the conductivity,the lithium ion diffusion coefficient, and the degree of freedom for volume change of LFP/C_(ZIF-8) cathode. This work will contribute to the improvement of the cathode materials of commercial LIB. 展开更多
关键词 LIFEPO4 Zeolitic imidazolate frameworks-8 Surface coating CATHODE Lithium ion battery
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Elucidation of the early infection machinery of hepatitis B virus by using bio-nanocapsule 被引量:1
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作者 Qiushi Liu Masaharu Somiya Shun'ichi Kuroda 《World Journal of Gastroenterology》 SCIE CAS 2016年第38期8489-8496,共8页
Currently, hepatitis B virus(HBV), upon attaching to human hepatocytes, is considered to interact first with heparan sulfate proteoglycan(HSPG) via an antigenic loop of HBV envelope S protein. Then, it is promptly tra... Currently, hepatitis B virus(HBV), upon attaching to human hepatocytes, is considered to interact first with heparan sulfate proteoglycan(HSPG) via an antigenic loop of HBV envelope S protein. Then, it is promptly transferred to the sodium taurocholate cotransporting polypeptide(NTCP) via the myristoylated N-terminal sequence of pre-S1 region(from Gly-2 to Gly-48, HBV genotype D), and it finally enters the cell by endocytosis. However, it is not clear how HSPG passes HBV to NTCP and how NTCP contributes to the cellular entry of HBV. Owing to the poor availability and the difficulty of manipulations, including fluorophore encapsulation, it has been nearly impossible to perform biochemical and cytochemical analyses using a substantial amount of HBV. A bio-nanocapsule(BNC), which is a hollow nanoparticle consisting of HBV envelope L protein, was efficiently synthesized in Saccharomyces cerevisiae. Since BNC could encapsulate payloads(drugs, genes, proteins) and specifically enter human hepatic cells utilizing HBV-derived infection machinery, it could be used as a model of HBV infection to elucidate the early infection machinery. Recently, it was demonstrated that the N-terminal sequence of pre-S1 region(from Asn-9 to Gly-24) possesses low p H-dependent fusogenic activity, which might play a crucial role in the endosomal escape of BNC payloads and in the uncoating process of HBV. In this minireview, we describe a model in which each domain of the HBV L protein contributes to attachment onto human hepatic cells through HSPG, initiation of endocytosis, interaction with NTCP in endosomes, and consequent provocation of membrane fusion followed by endosomal escape. 展开更多
关键词 Bio-nanocapsule Endosomal escape Hepatitis B virus Heparan sulfate PROTEOGLYCAN Sodium TAUROCHOLATE cotransporting POLYPEPTIDE
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Dication-accelerated anion transport inside micropores for the rapid decontamination of pertechnetate 被引量:1
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作者 Peng Zhang Yi-Zhi Chen +5 位作者 Han-Qin Weng Zi-Fang Guo Jia-Liang Chen Xing Zhao Guo-An Ye Ming-Zhang Lin 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2022年第4期19-32,共14页
Over 70%of the treated contaminated water at the Fukushima Daiichi Nuclear Power Station contains radionuclides beyond the regulatory standard for discharge that need to be re-purified.Technetium-99(^(99)Tc),mainly in... Over 70%of the treated contaminated water at the Fukushima Daiichi Nuclear Power Station contains radionuclides beyond the regulatory standard for discharge that need to be re-purified.Technetium-99(^(99)Tc),mainly in the form of pertechnetate Tc(VII)O_(4)^(-),is one of the main sources of long-term radiotoxicity that jeopardizes the environment and human health.Herein,we used a series of dicationic pyridinium(DCP)derivative groups(–Py^(+)C_(n)H_(2n)N^(+)Me_(3),n=2,3,and 5)to modify commercial Reillex 425 resins containing tertiary pyridyl groups to improve the adsorption performance of rhenium(Re,an analog of radioactive Tc)and Tc.As the quaternary pyridinium and ammonium sites in one DCP group can adsorb ReO_(4)^(-) simultaneously,DCP-modified Reillex 425(Reillex-Cn)exhibited high maximum adsorption capacities for Re under neutral conditions.Adsorption capacities reached 344.8,416.7,and 588.2 mg g^(-)1 for Reillex 425-C2,Reillex 425-C3,and Reillex 425-C5,respectively.Intraparticle diffusion of ReO_(4)^(-)/TcO_(4)^(-) in Reillex 425-Cn was verified to be the rate-limiting step of adsorption.However,adsorption can be adjusted by the length of the alkyl spacers between the two positively charged N sites in DCP.–Py^(+)C_(2)H_(4)N^(+)Me_(3) significantly enhanced intraparticle diffusion compared to–Py^(+)C_(5)H_(10)N^(+)Me_(3).The two positive sites in–Py^(+)C_(2)H_(4)N^(+)Me_(3) would be laterally distributed,leading to a smaller steric hindrance for ReO_(4)–/TcO_(4)^(-) transport inside the microporous channels.Meanwhile,the longer alkyl spacers in–Py^(+)C_(5)H_(10)N^(+)Me_(3) formed hydrophobic microphases,repulsing the hydrated ReO_(4)–/TcO_(4)^(-) anions.Thus,the adsorptions of both ReO_(4)^(-) and TcO_(4)^(-) on Reillex 425-C2 were faster than those on Reillex 425-C5.Moreover,Reillex 425-Cn exhibited an exothermic nature,good selectivity,excellent reusability,and strong salinity tolerance.This study provides a simple strategy to enhance the Tc removal performance of adsorbents containing abundant micropores,which implies enormous environmental and economic benefits. 展开更多
关键词 Quaternary pyridinium Dicationic pyridyl derivatives PERTECHNETATE Intraparticle diffusion
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Silver Nanowire Electrodes: Conductivity Improvement Without Post-treatment and Application in Capacitive Pressure Sensors 被引量:11
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作者 Jun Wang Jinting Jiu +6 位作者 Teppei Araki Masaya Nogi Tohru Sugahara Shijo Nagao Hirotaka Koga Peng He Katsuaki Suganuma 《Nano-Micro Letters》 SCIE EI CAS 2015年第1期51-58,共8页
Transparent electrode based on silver nanowires(Ag NWs) emerges as an outstanding alternative of indium tin oxide film especially for flexible electronics. However, the conductivity of Ag NWs transparent electrode is ... Transparent electrode based on silver nanowires(Ag NWs) emerges as an outstanding alternative of indium tin oxide film especially for flexible electronics. However, the conductivity of Ag NWs transparent electrode is still dramatically limited by the contact resistance between nanowires at high transmittance. Polyvinylpyrrolidone(PVP) layer adsorbed on the nanowire surface acts as an electrically insulating barrier at wire–wire junctions, and some devastating post-treatment methods are proposed to reduce or eliminate PVP layer, which usually limit the application of the substrates susceptible to heat or pressure and burden the fabrication with high-cost, time-consuming, or inefficient processes. In this work, a simple and rapid pre-treatment washing method was proposed to reduce the thickness of PVP layer from 13.19 to0.96 nm and improve the contact between wires. Ag NW electrodes with sheet resistances of 15.6 and 204 X sq-1have been achieved at transmittances of 90 and 97.5 %, respectively. This method avoided any post-treatments and popularized the application of high-performance Ag NW transparent electrode on more substrates. The improved Ag NWs were successfully employed in a capacitive pressure sensor with high transparency, sensitivity, and reproducibility. 展开更多
关键词 Silver nanowire Pre-treatment Transparent electrode Pressure sensor
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Development of tailored TiO_2 mesocrystals for solar driven photocatalysis 被引量:3
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作者 Peng Zhang Mamoru Fujitsuka Tetsuro Majima 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2016年第6期917-926,共10页
Ordered metal oxides superstructures have attracted much more attention in the fields of fuel generation and environmental purification owing to their unique physiochemical characteristics such as large surface area, ... Ordered metal oxides superstructures have attracted much more attention in the fields of fuel generation and environmental purification owing to their unique physiochemical characteristics such as large surface area, fine pore structure, efficient electronic mobility, and good stability. Very recently, TiOmesocrystals(TMCs) having superstructures self-assembled by TiOnanoparticle building blocks, are of considerable interest in current research and application ranging from UV to visible light attributed to their efficient charge separation and superior photocatalytic activity. In this review, we describe the common procedures to prepare unique TMCs and overview of recent developments of TMCs during last 3 years, especially the structure-related or electronic-effected mechanism in photocatalytic reaction. Further, we introduce the characterization and fundamental properties of modified TMCs by the means of single-particle fluorescence microscopy for unraveling the charge transport and photocatalytic properties of individual TMCs and time-resolved diffuse reflectance spectroscopy(TDR) for monitoring the charge transfer dynamics. Finally, various aspects on TMCs are discussed for the future developments of energy and environmental fields. 展开更多
关键词 TiO2 Mesocrystal PHOTOCATALYST Topotactic transformation DOPING Charge separation CO-CATALYST Electron flow
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Development of picosecond pulse radiolysis system at Waseda University
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作者 T Kuribayashi K Ushida +5 位作者 S Kashiwagi R Kuroda H Hirama M Kawaguchi Y Hama M Washio 《辐射研究与辐射工艺学报》 CAS CSCD 北大核心 2005年第2期69-69,共1页
A compact pulse radiolysis apparatus using a BNL-type s-band photocathode RF gun is now under development at Waseda University.The laser pulse is used for excitation of the photocathode and for generation of white lig... A compact pulse radiolysis apparatus using a BNL-type s-band photocathode RF gun is now under development at Waseda University.The laser pulse is used for excitation of the photocathode and for generation of white light,which is used for analyzing light in the pulse radiolysis. 展开更多
关键词 Pico-second pulse radiolysis system Data deconvolution
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Chemical vapor deposition synthesis of V-doped MoS_(2)
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作者 Yang Yang Qing-Rong Liang +6 位作者 Chun-Li Zhu Guo-Zhong Zheng Jian Zhang Shou-Jun Zheng Yung-Chang Lin De-Zhi Zheng Jia-Dong Zhou 《Rare Metals》 SCIE EI CAS CSCD 2023年第12期3985-3992,共8页
Van der Waals coupling with different stacking configurations can significantly affect the optical and electronic properties of ultrathin two-dimensional(2D)materials,which is an effective way to tune device performan... Van der Waals coupling with different stacking configurations can significantly affect the optical and electronic properties of ultrathin two-dimensional(2D)materials,which is an effective way to tune device performance.Herein,we report a salt-assisted chemical vapor deposition method for the synthesis of bilayer V-doped MoS_(2) with 2H and 3R phases,which are demonstrated by the second harmonic generation and scanning transmission electron microscopy.Notably,the mobility of the 3R phase V-doped MoS_(2) is 6.2%higher than that of the 2H phase.Through first-principles calculations,we further reveal that this particular behavior is attributed to the stronger interlayer coupling of 3R compared to the 2H stacking configuration.This research can be further generalized to other transition metal chalcogenides and will contribute to the development of electronic devices based on 2D materials in the future. 展开更多
关键词 Chemical vapor deposition SYNTHESIS Firstprinciples calculations 2H 3R
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Oxidation-enhanced bonding strength of Cu sinter joints during thermal storage test 被引量:2
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作者 Yue Gao Jinting Jiu +3 位作者 Chuantong Chen Katsuaki Suganuma Rong Sun Zhi-Quan Liu 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2022年第20期251-255,共5页
With the development in next-generation semiconductor power devices,the power devices based on silicon carbide(SiC)and gallium nitride(GaN)are expected to replace the traditional Si-based power devices[1–6].However,t... With the development in next-generation semiconductor power devices,the power devices based on silicon carbide(SiC)and gallium nitride(GaN)are expected to replace the traditional Si-based power devices[1–6].However,the foreseeable harsh operating environment such as heavy thermal-load or extremely temperature cycle required more reliable interconnection technology[4,7-9]. 展开更多
关键词 INTERCONNECTION THERMAL BONDING
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Precise Synthesis of Organometallic Dendrimers 被引量:1
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作者 K. Onitsuka S. Takahashi 《复旦学报(自然科学版)》 CAS CSCD 北大核心 2005年第5期823-824,共2页
关键词 有机金属 树型化合物 乙炔化物 合成方法 光学性质
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Effects of Bi-dopant and co-catalysts upon hole surface trapping on La_(2)Ti_(2)O_(7) nanosheet photocatalysts in overall solar water splitting 被引量:1
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作者 Xiaoyan Cai Liang Mao +4 位作者 Mamoru Fujitsuka Tetsuro Majima Sujan Kasani Nianqiang Wu Junying Zhang 《Nano Research》 SCIE EI CSCD 2022年第1期438-445,共8页
Pristine and Bi-doped lanthanum titanium oxide(La_(2)Ti_(2)O_(7))nanosheets have been synthesized as photocatalysts for overall solar water splitting.The surface hole trap is a critical factor that limits the photocat... Pristine and Bi-doped lanthanum titanium oxide(La_(2)Ti_(2)O_(7))nanosheets have been synthesized as photocatalysts for overall solar water splitting.The surface hole trap is a critical factor that limits the photocatalytic activity of pristine La_(2)Ti_(2)O_(7)-Deposition of cobalt phosphate(Co-Pi)and platinum(Pt)nanoparticles on La_(2)Ti_(2)O_(7) cannot remove the surface traps although they are essential for enabling the oxygen and hydrogen evolution reactions.It is interesting that doping bismuth(Bi)into La_(2)Ti_(2)O_(7) nanosheets has eliminated the surface traps due to surface enrichment of Bi.The Co-Pi/Bi-La_(2)Ti_(2)O_(7)/Pt nanosheets exhibit increasing photocatalytic activity toward overall water splitting with increasing the Bi-dopant level up to 5 at.%.Further increasing the Bi-dopant level leads to the formation of localized states above the valence band,leading to the lifetime reduction of photogenerated charge-carriers,and jeopardizing the photocatalytic activity.This work proposes an effective strategy to address the surface trapping and surface catalysis issues in the nanostructured metal oxide photocatalysts. 展开更多
关键词 photocatalyst water splitting surface trap CO-CATALYST solar fuel
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The relationship between formate adsorption energy and electronic properties: A first principles density functional theory study
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作者 MORIKAWA Yoshitada NAKAMURA Junji 《Science China Chemistry》 SCIE EI CAS 2009年第9期1427-1433,共7页
First principles density functional theory calculations have been performed for the chemisorption of formate adsorption on some metal surfaces. For the most stable adsorption site of short-bridge, the calculated forma... First principles density functional theory calculations have been performed for the chemisorption of formate adsorption on some metal surfaces. For the most stable adsorption site of short-bridge, the calculated formate adsorption energy follows the order of Au(110) < Ag(110) < Cu(110) < Pd(110) < Pt(110) < Ni(110) < Rh(110) < Fe(100) < Mo(100), and a clear linear correlation exists between the adsorption energy and the corresponding heat of formation of metal oxides. Moreover, it has been found that the formate adsorption energy for the transition metals can be correlated well with its d-band center (εd), and the IB Group metals can be described by the coupling matrix element square (Vad2). 展开更多
关键词 FORMATE metal DFT-GGA SLAB model adsorption energy d-band CENTER
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Fabrication of Silver Nanowire Transparent Electrodes at Room Temperature 被引量:39
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作者 Takehiro Tokuno Masaya Nogi Makoto Karakawa Jinting Jiu Thi Thi Nge Yoshio Aso Katsuaki Suganuma 《Nano Research》 SCIE EI CAS CSCD 2011年第12期1215-1222,共8页
Silver nanowires (AgNWs) surrounded by insulating poly(vinylpyrrolidone) have been synthesized by a polyol process and employed as transparent electrodes. The AgNW transparent electrodes can be fabricated by heatt... Silver nanowires (AgNWs) surrounded by insulating poly(vinylpyrrolidone) have been synthesized by a polyol process and employed as transparent electrodes. The AgNW transparent electrodes can be fabricated by heattreatment at about 200 ℃ which forms connecting junctions between AgNWs. Such a heating process is, however, one of the drawbacks of the fabrication of AgNW electrodes on heat-sensitive substrates. Here it has been demonstrated that the electrical conductivity of AgNW electrodes can be improved by mechanical pressing at 25 MPa for 5 s at room temperature. This simple process results in a low sheet resistance of 8.6 Ω/square and a transparency of 80.0%, equivalent to the properties of the AgNW electrodes heated at 200 ℃. This technique makes it possible to fabricate AgNW transparent electrodes on heat-sensitive substrates. The AgNW electrodes on poly(ethylene terephthalate) films exhibited high stability of their electrical conductivities against the repeated bending test. In addition, the surface roughness of the pressed AgNW electrodes is one-third of that of the heat-treated electrode because the AgNW junctions are mechanically compressed. As a result, an organic solar cell fabricated on the pressed AgNW electrodes exhibited a power conversion as much as those fabricated on indium tin oxide electrodes. These findings enable continuous roll-to-roll processing at room temperature, resulting in relatively simple, inexpensive, and scalable processing that is suitable for forthcoming technologies such as organic solar cells, flexible displays, and touch screens. 展开更多
关键词 Silver nanowire transparent electrode room temperature FLEXIBILITY organic solar cell
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Facile fabrication of stretchable Ag nanowire/polyurethane electrodes using high intensity pulsed light 被引量:11
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作者 Yang Yang1 Su Ding +6 位作者 Teppei Araki Jinting Jiu Tohru Sugahara Jun Wang Jan Vanfleteren Tsuyoshi Sekitani Katsuaki Suganuma 《Nano Research》 SCIE EI CAS CSCD 2016年第2期401-414,共14页
Silver nanowires (AgNWs) have emerged as a promising nanomaterial for next generation stretchable electronics. However, until now, the fabrication of AgNW- based components has been hampered by complex and time-cons... Silver nanowires (AgNWs) have emerged as a promising nanomaterial for next generation stretchable electronics. However, until now, the fabrication of AgNW- based components has been hampered by complex and time-consuming steps. Here, we introduce a facile, fast, and one-step methodology for the fabrication of highly conductive and stretchable AgNW/polyurethane (PU) composite electrodes based on a high-intensity pulsed light (HIPL) technique. HIPL simultaneously improved wire-wire junction conductivity and wire-substrate adhesion at room temperature and in air within 50 μs, omitting the complex transfer-curing-implanting process. Owing to the localized deformation of PU at interfaces with AgNWs, embedding of the nanowires was rapidly carried out without substantial substrate damage. The resulting electrode retained a low sheet resistance (high electrical conductivity) of 〈10 Ω/sq even under 100% strain, or after 1,000 continuous stretching-relaxation cycles, with a peak strain of 60%. The fabricated electrode has found immediate application as a sensor for motion detection. Furthermore, based on our electrode, a light emitting diode (LED) driven by integrated stretchable AgNW conductors has been fabricated. In conclusion, our present fabrication approach is fast, simple, scalable, and cost- efficient, making it a good candidate for a future roll-to-roll process. 展开更多
关键词 silver nanowires stretchable electrode photonic sintering nanofabrication
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Mechanism of improved electromigration reliability using Fe-Ni UBM in wafer level package 被引量:3
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作者 Li-Yin Gao Hao Zhang +2 位作者 Cai-Fu Li Jingdong GUO Zhi-Quan Liu 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2018年第8期1305-1314,共10页
Fe-Ni films with compositions of 73 wt% of Ni and 45 wt% of Ni were used as under bump metallization (UBM) in wafer level chip scale package, and their reliability was evaluated through electromigration (EM) test ... Fe-Ni films with compositions of 73 wt% of Ni and 45 wt% of Ni were used as under bump metallization (UBM) in wafer level chip scale package, and their reliability was evaluated through electromigration (EM) test compared with commercial Cu UBM. For Sn3.SAg0.7Cu(SAC)]Cu solder joints, voids had initiated at Cu cathode after 300 h and typical failures of depletion of Cu cathode and cracks were detected after 1000 h EM. While the SAC]Fe-Ni solder joints kept at a perfect condition without any failures after 1000 h EM. Moreover, the characteristic lifetime calculated by Weibull analysis for Fe-73Ni UBM (2121 h), Fe-45Ni UBM (2340 h) were both over three folds to Cu UBM's (698 h). The failure modes for Fe-Ni solder joints varied with the different growth behavior of intermetallic compounds (IMCs), which can all be classified as the crack at the cathodic interface between solder and outer IMC layer. The atomic fluxes concerned cathode dissolution and crack initiation were analyzed. When Fe-Ni UBM was added, cathode dissolution was suppressed due to the low diffusivity of IMCs and opposite transferring direction to electron flow of Fe atoms. The smaller EM flux within solder material led a smaller vacancy flux in Fe-Ni solder joints, which can explain the delay of solder voids and cracks as well as the much longer lifetime under EM. 展开更多
关键词 Fe-Ni under bump metallization (UBM) Intermetallic compounds (IMCs) Electromigration (EM) Diffusion Vacancy formation
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Van der Waals epitaxy of ultrathin crystalline PbTe nanosheets with high near-infrared photoelectric response 被引量:3
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作者 Xinxin Zhao Qing Yin +8 位作者 Hao Huang Qiang Yu Bo Liu Jie Yang Zhuo Dong Zhenjiang Shen Benpeng Zhu Lei Liao Kai Zhang 《Nano Research》 SCIE EI CAS CSCD 2021年第6期1955-1960,共6页
Lead telluride(PbTe)is one of the reliable candidates for infrared(IR)optoelectronics with optimum band-gap as well as excellent photoelectric properties.Great interests had been paid on the growth and device applicat... Lead telluride(PbTe)is one of the reliable candidates for infrared(IR)optoelectronics with optimum band-gap as well as excellent photoelectric properties.Great interests had been paid on the growth and device applications with PbTe for the development of high-performance IR photodetectors especially those working in the near-infrared regime.Although a great deal of effort had been made to prepare PbTe nanostructures for miniaturized detectors,it is difficult to synthesize high-quality two-dimensional(2D)PbTe crystals due to its rock-salt non-layered structure.Herein,a facile strategy for controllable synthesis of ultrathin crystalline PbTe nanosheets by van der Waals epitaxy is reported.With an optimized growth temperature,which determines the morphology transit from triangular pyramid islands to regular square 2D planars,PbTe nanosheets in lateral size of tens of microns with thickness down to~7 nm are achieved.Meanwhile,ultrasensitive near-infrared detectors(NIRDs)based on the as-grown 2D PbTe nanosheets have been demonstrated with an ultrahigh responsivity exceeding 3,847 A/W at the wavelength of 1,550 nm under room temperature.Our approach demonstrates that 2D PbTe nanosheets have great latent capacity of developing high-performance miniaturized IR optoelectronic devices. 展开更多
关键词 two-dimensional materials van der Waals epitaxy lead telluride NEAR-INFRARED PHOTODETECTOR
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Development of anti-oxidation Ag salt paste for large-area(35×35 mm^(2))Cu-Cu bonding with ultra-high bonding strength 被引量:1
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作者 Bowen Zhang Chuantong Chen +3 位作者 Takuya Sekiguchi Yang Liu Caifu Li Katsuaki Suganuma 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2022年第18期261-270,共10页
In this paper,by proposing a novel and low-cost Ag salt paste,a robustly and large-area(35×35 mm^(2))bare Cu to Cu bonding was realized under a low sintering pressure of 0.8 MPa and a low sintering temperature of... In this paper,by proposing a novel and low-cost Ag salt paste,a robustly and large-area(35×35 mm^(2))bare Cu to Cu bonding was realized under a low sintering pressure of 0.8 MPa and a low sintering temperature of 300℃ in air atmospheric conditions.The relationship between the bonding strength and microstructure changes of sintered Ag under various bonding conditions was investigated in detail.The large-area bonded plate exhibits low porosity about 10%and low percentage of voids,which result in ultra-high bonding strength over 58 MPa.More importantly,the introduction of reducing agent formic acid(CH_(2)O_(2))and the low porosity successfully improve the anti-oxidation of novel Ag salt paste during sintering process,result in pure Cu-Ag-Cu bonding.The cross-section of the Ag joints was obtained to explain the bonding pattern,in which Cu was oxidized only at the edge of the sintering interface,and no Cu oxide generated in middle bonding section.The development of novel Ag salt paste successfully addresses the energy-intensive process and low bonding strength faced by large-scale sintering,which greatly promotes the high-temperature applications of power device. 展开更多
关键词 Large-area bonding ANTI-OXIDATION Cu-cu joint Ag salt paste Bonding strength
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Ambipolar device simulation based on the drift-diffusion model in ion-gated transition metal dichalcogenide transistors 被引量:1
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作者 Akiko Ueda Yijin Zhang +2 位作者 Nobuyuki Sano Hiroshi Imamura Yoshihiro Iwasa 《npj Computational Materials》 SCIE EI CSCD 2020年第1期1446-1454,共9页
Ionic gating is known as a powerful tool for investigation of electronic functionalities stemming from low voltage transistor operation to gate-induced electronic phase control including superconductivity.Two-dimensio... Ionic gating is known as a powerful tool for investigation of electronic functionalities stemming from low voltage transistor operation to gate-induced electronic phase control including superconductivity.Two-dimensional(2D)material is one of the archetypal channel materials which exhibit a variety of gate-induced phenomena.Nevertheless,the device simulations on such iongated transistor devices have never been reported,despite its importance for the future design of device structures.In this paper,we developed a drift-diffusion(DD)model on a 2D material,WSe2 monolayer,attached with an ionic liquid,and succeeded in simulating the transport properties,potential profile,carrier density distributions in the transistor configuration. 展开更多
关键词 TRANSISTOR BIPOLAR diffusion
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