Interactive holography offers unmatched levels of immersion and user engagement in the field of future display.Despite of the substantial progress has been made in dynamic meta-holography,the realization of real-time,...Interactive holography offers unmatched levels of immersion and user engagement in the field of future display.Despite of the substantial progress has been made in dynamic meta-holography,the realization of real-time,highly smooth interactive holography remains a significant challenge due to the computational and display frame rate limitations.In this study,we introduced a dynamic interactive bitwise meta-holography with ultra-high computational and display frame rates.To our knowledge,this is the first reported practical dynamic interactive metasurface holographic system.We spa-tially divided the metasurface device into multiple distinct channels,each projecting a reconstructed sub-pattern.The switching states of these channels were mapped to bitwise operations on a set of bit values,which avoids complex holo-gram computations,enabling an ultra-high computational frame rate.Our approach achieves a computational frame rate of 800 kHz and a display frame rate of 23 kHz on a low-power Raspberry Pi computational platform.According to this methodology,we demonstrated an interactive dynamic holographic Tetris game system that allows interactive gameplay,color display,and on-the-fly hologram creation.Our technology presents an inspiration for advanced dynamic meta-holography,which is promising for a broad range of applications including advanced human-computer interaction,real-time 3D visualization,and next-generation virtual and augmented reality systems.展开更多
Multispectral and polarized focusing and imaging are key functions that are vitally important for a broad range of optical applications.Conventional techniques generally require multiple shots to unveil desired optica...Multispectral and polarized focusing and imaging are key functions that are vitally important for a broad range of optical applications.Conventional techniques generally require multiple shots to unveil desired optical information and are implemented via bulky multi-pass systems or mechanically moving parts that are difficult to integrate into compact and integrated optical systems.Here,a design of ultra-compact transversely dispersive metalens capable of both spectrum and polarization ellipticity recognition and reconstruction in just a single shot is demonstrated with both coherent and incoherent light.Our design is well suited for integrated and high-speed optical information analysis and can significantly reduce the size and weight of conventional devices while simplifying the process of collecting optical information,thereby promising for various applications,including machine vision,minimized spectrometers,material characterization,remote sensing,and other areas which require comprehensive optical analysis.展开更多
Self-accelerating beams have the unusual ability to remain diffraction-free while undergo the transverse shift during the free-space propagation.We theoretically identify that the transverse optical field distribution...Self-accelerating beams have the unusual ability to remain diffraction-free while undergo the transverse shift during the free-space propagation.We theoretically identify that the transverse optical field distribution of 2D self-accelerating beam is determined by the selection of the transverse Cartesian coordinates,when the caustic method is utilized for its trajectory design.Based on the coordinate-rotation method,we experimentally demonstrate a scheme to flexibly manipulate the rotation of transverse optical field for 2D self-accelerating beams under the condition of a designated trajectory.With this scheme,the transverse optical field can be rotated within a range of 90 degrees,especially when the trajectory of 2D self-accelerating beams needs to be maintained for free-space photonic interconnection.展开更多
Tin (Sn) metal foil is a promising anode for next-generation high-energy–density lithium-ion batteries (LIBs) due to its high capacity and easy processibility. However, the pristine Sn foil anode suffers nonuniform a...Tin (Sn) metal foil is a promising anode for next-generation high-energy–density lithium-ion batteries (LIBs) due to its high capacity and easy processibility. However, the pristine Sn foil anode suffers nonuniform alloying/dealloying reaction with lithium (Li) and huge volume variation, leading to electrode pulverization and inferior electrochemical performance. Herein, we proposed that reduced grain size and elaborate porosity design of Sn foil can circumvent the nonuniform alloy reaction and buffer the volume change during the lithiation/delithiation cycling. Experimentally, we designed a three-dimensional interconnected porous Sn (3DIP-Sn) foil by a facile chemical alloying/dealloying approach, which showed improved electrochemical performance. The enhanced structure stability of the as-fabricated 3DIP-Sn foil was verified by chemo-mechanical simulations and experimental investigation. As expected, the 3DIP-Sn foil anode revealed a long cycle lifespan of 4400 h at 0.5 mA cm^(−2) and 1 mAh cm^(−2) in Sn||Li half cells. A 3DIP-Sn||LiFePO_(4) full cell with LiFePO_(4) loading of 7.1 mg cm^(−2) exhibited stable cycling for 500 cycles with 80% capacity retention at 70 mA g^(−1). Pairing with high-loading commercial LiNi0.6Co0.2Mn0.2O_(2) (NCM622, 18.4 mg cm^(−2)) cathode, a 3DIP-Sn||NCM622 full cell delivered a high reversible capacity of 3.2 mAh cm^(−2). These results demonstrated the important role of regulating the uniform alloying/dealloying reaction and circumventing the localized strain/stress in improving the electrochemical performance of Sn foil anodes for advanced LIBs.展开更多
Optical vortex arrays,with their unique wavefront structures,find extensive applications in fields such as optical communications,trapping,imaging,metrology,and quantum.The methods used to generate these vortex beam a...Optical vortex arrays,with their unique wavefront structures,find extensive applications in fields such as optical communications,trapping,imaging,metrology,and quantum.The methods used to generate these vortex beam arrays are crucial for their applications.In this review,we begin with introducing the fundamental concepts of optical vortex beams.Subsequently,we present three methods for generating them,including diffractive optical elements,metasurfaces,and integrated optical devices.We then explore the applications of optical vortex beam arrays in five different domains.Finally,we conclude with a summary and outlook for the research on optical vortex beam arrays.展开更多
High-performance infrared(IR)photodetectors made by low dimensional materials promise a wide range of applications in communication,security and biomedicine.Moreover,light-harvesting effects based on novel plasmonic m...High-performance infrared(IR)photodetectors made by low dimensional materials promise a wide range of applications in communication,security and biomedicine.Moreover,light-harvesting effects based on novel plasmonic materials and their combinations with two-dimensional(2 D)materials have raised tremendous interest in recent years,as they may potentially help the device complement or surpass currently commercialized IR photodetectors.Graphene is a particularly attractive plasmonic material because graphene plasmons are electrically tunable with a high degree of electromagnetic confinement in the mid-infrared(mid-IR)to terahertz regime and the field concentration can be further enhanced by forming nanostructures.Here,we report an efficient mid-IR room-temperature photodetector enhanced by plasmonic effect in graphene nanoresonators(GNRs)/graphene heterostructure.The plasmon polaritons in GNRs are size-dependent with strong field localization.Considering that the size and density of GNRs are controllable by chemical vapor deposition method,our work opens a cost-effective and scalable pathway to fabricate efficient IR optoelectronic devices with wavelength tunability.展开更多
The photovoltaic(PV)market is currently dominated by silicon based solar cells.However technological diversification is essential to promote competition,which is the driving force for technological growth.Historically...The photovoltaic(PV)market is currently dominated by silicon based solar cells.However technological diversification is essential to promote competition,which is the driving force for technological growth.Historically,the choice of PV materials has been limited to the three-dimensional(3D)compounds with a high crystal symmetry and direct band gap.However,to meet the strict demands for sustainable PV applications,material space has been expanded beyond 3D compounds.In this perspective we discuss the potential of low-dimensional materials(2D,1D)for application in PVs.We present unique features of low-dimensional materials in context of their suitability in the solar cells.The band gap,absorption,carrier dynamics,mobility,defects,surface states and growth kinetics are discussed and compared to 3D counterparts,providing a comprehensive view of prospects of low-dimensional materials.Structural dimensionality leads to a highly anisotropic carrier transport,complex defect chemistry and peculiar growth dynamics.By providing fundamental insights into these challenges we aim to deepen the understanding of low-dimensional materials and expand the scope of their application.Finally,we discuss the current research status and development trend of solar cell devices made of low-dimensional materials.展开更多
Metamaterial structure based on cascaded split ring resonators (CSRR) is proposed in order to produce a negative refractive index in terahertz regime at near-infrared range. We have incident light horizontally instead...Metamaterial structure based on cascaded split ring resonators (CSRR) is proposed in order to produce a negative refractive index in terahertz regime at near-infrared range. We have incident light horizontally instead of incidenting it perpendicular. We have measured the negative refractive index, permeability and permittivity by using the S-parameter analysis. Furthermore, it is found out that negative refractive index, permeability and permittivity are dependent upon the width of the wire and the gap between resonators at near-infrared range. This work will be helpful for the fabrication and design of double negative metamaterials structure having negative permeability, permittivity and negative refractive index for in plane applications.展开更多
Explosive growth in demand for data traffic has prompted exploration of the spatial dimension of lightwaves, which provides a degree of freedom to expand data transmission capacity. Various techniques basedon bulky op...Explosive growth in demand for data traffic has prompted exploration of the spatial dimension of lightwaves, which provides a degree of freedom to expand data transmission capacity. Various techniques basedon bulky optical devices have been proposed to tailor light waves in the spatial dimension. However, theirinherent large size, extra loss, and precise alignment requirements make these techniques relativelydifficult to implement in a compact and flexible way. In contrast, three-dimensional (3D) photonic chips withcompact size and low loss provide a promising miniaturized candidate for tailoring light in the spatialdimension. Significantly, they are attractive for chip-assisted short-distance spatial mode optical interconnectsthat are challenging to bulky optics. Here, we propose and fabricate femtosecond laser-inscribed 3D photonicchips to tailor orbital angular momentum (OAM) modes in the spatial dimension. Various functions on theplatform of 3D photonic chips are experimentally demonstrated, including the generation, (de)multiplexing,and exchange of OAM modes. Moreover, chip-chip and chip–fiber–chip short-distance optical interconnectsusing OAM modes are demonstrated in the experiment with favorable performance. This work paves the wayto flexibly tailor light waves on 3D photonic chips and offers a compact solution for versatile opticalinterconnects and other emerging applications with spatial modes.展开更多
Optical beating is the usual approach to generation of microwave signals.However,the highest frequency achievable for microwave signals is limited by the bandwidths of optoelectronic devices.To maximize the microwave ...Optical beating is the usual approach to generation of microwave signals.However,the highest frequency achievable for microwave signals is limited by the bandwidths of optoelectronic devices.To maximize the microwave frequency with a limited bandwidth of a photodetector(PD)and relieve the bandwidth bottleneck,we propose to generate microwave signals with the single sideband(SSB)format by beating a continuous wave(CW)light with an optical SSB signal.By simply adjusting the frequency diference between the CW light and the carrier of the optical SSB signal,the frequency of the generated microwave SSB signal is changed correspondingly.In the experiment,amplitude shift keying(ASK)microwave signals with the SSB format are successfully generated with diferent carrier frequencies and coding bit rates,and the recovered coding information agrees well with the original pseudo random binary sequence(PRBS)of 2^(7)−1 bits.The proposed approach can signifcantly relieve the bandwidth restriction set by optoelectronic devices in high-speed microwave communication systems.展开更多
Nano-3D printing has obtained widespread attention owing to its capacity to manufacture end-use components with nano-scale features in recent years.Multiphoton lithography(MPL)is one of the most promising 3D nanomanuf...Nano-3D printing has obtained widespread attention owing to its capacity to manufacture end-use components with nano-scale features in recent years.Multiphoton lithography(MPL)is one of the most promising 3D nanomanufacturing technologies,which has been widely used in manufacturing micro-optics,photonic crystals,microfluidics,meta-surface,and mechanical metamaterials.Despite of tremendous potential of MPL in laboratorial and industrial applications,simultaneous achievement of high throughput,high accuracy,high design freedom,and a broad range of material structuring capabilities remains a long-pending challenge.To address the issue,we propose an acousto-optic scanning with spatial-switching multispots(AOSS)method.Inertia-free acousto-optic scanning and nonlinear swept techniques have been developed for achieving ultrahigh-speed and aberration-free scanning.Moreover,a spatial optical switch concept has been implemented to significantly boost the lithography throughput while maintaining high resolution and high design freedom.An eight-foci AOSS system has demonstrated a record-high 3D printing rate of 7.6×10^(7)voxel s^(-1),which is nearly one order of magnitude higher than earlier scanning MPL,exhibiting its promise for future scalable 3D nanomanufacturing.展开更多
The complex Maxwell stress tensor theorem has been developed to relate the imaginary optical force,reactive strength of canonical momentum and total optical force of a nanoparticle,which is essential to perfect optica...The complex Maxwell stress tensor theorem has been developed to relate the imaginary optical force,reactive strength of canonical momentum and total optical force of a nanoparticle,which is essential to perfect optical force efficiency.展开更多
Scintillators are widely utilized in high-energy radiation detection in view of their high light yield and short fluorescence decay time.However,constrained by their current shortcomings,such as complex fabrication pr...Scintillators are widely utilized in high-energy radiation detection in view of their high light yield and short fluorescence decay time.However,constrained by their current shortcomings,such as complex fabrication procedures,high temperature,and difficulty in the large scale,it is difficult to meet the increasing demand for costeffective,flexible,and environment-friendly X-ray detection using traditional scintillators.Perovskite-related cesium copper halide scintillators have recently received multitudinous research due to their tunable emission wavelength,high photoluminescence quantum yield(PLQY),and excellent optical properties.Herein,we demonstrated a facile solution-synthesis route for indium-doped all-inorganic cesium copper iodide(Cs_(3)Cu_(2)I_(5))powders and a high scintillation yield flexible film utilizing indium-doped Cs_(3)Cu_(2)I_(5)powders.The large area flexible films achieved a PLQY as high as 90.2%by appropriately adjusting the indium doping concentration,much higher than the undoped one(73.9%).Moreover,benefiting from low self-absorption and high PLQY,the Cs_(3)Cu_(2)I_(5):In films exhibited ultralow detection limit of 56.2 n Gy/s,high spatial resolution up to 11.3 lp/mm,and marvelous relative light output with strong stability,facilitating that Cs_(3)Cu_(2)I_(5):In films are excellent candidates for X-ray medical radiography.Our work provides an effective strategy for developing environment-friendly,low-cost,and efficient scintillator films,showing great potential in the application of highperformance X-ray imaging.展开更多
Perovskite-based optoelectronic devices,espe-cially perovskite light-emitting diodes(PeLEDs)and perovskite solar cells,have recently attracted considerable attention.The National Renewable Energy Laboratory(NREL)chart...Perovskite-based optoelectronic devices,espe-cially perovskite light-emitting diodes(PeLEDs)and perovskite solar cells,have recently attracted considerable attention.The National Renewable Energy Laboratory(NREL)chart inspires us to develop a counterpart for PeLEDs.In this study,we collect the record performance of PeLEDs including several new entries to address their latest external quantum efficiency(EQE),highest lumi-nance,and stability status.We hope that these performance tables and future updated versions will show the frontiers of PeLEDs,assist researchers in capturing the overview of this field,identify the remaining challenges,and predict the promising research directions.展开更多
Preparation of high-quality films plays an important role to achieve high-performance nonfullerene (NF) organic solar cells. NF active layer films are typically fabricated by spin coating. Novel fabrication methods to...Preparation of high-quality films plays an important role to achieve high-performance nonfullerene (NF) organic solar cells. NF active layer films are typically fabricated by spin coating. Novel fabrication methods to process the NF active layer are desirable to be compatible with large-area production. Herein, we report on the fabrication of NF active layer films via a water transfer printing method.This method delivers a uniform film with controllable film thicknesses. NF active layers of PDBD-T:ITIC and PBDB-T-2F:IT-4F were fabricated via the method to validate its effectiveness. Solar cells with the water transfer-printed active layers show comparable performance (up to 11.7%) to the cells with spin-coated active layers. Furthermore, NF solar modules containing 4-sub cells with the active area of 3.2 cm2 are also fabricated via the method. The module shows VOC of up to 3.4 V and a power conversion efficiency of 8.1% with the PBDB-T-2F:IT-4F active layer.展开更多
Niobium nitride superconducting nanowire single-photon detectors were fabricated on thermally oxidized silicon substrates with large active areas of 30 μm× 30 μm.To achieve non-constricted detectors,we improved...Niobium nitride superconducting nanowire single-photon detectors were fabricated on thermally oxidized silicon substrates with large active areas of 30 μm× 30 μm.To achieve non-constricted detectors,we improved the film growth and electron beam lithography process to fabricate uniform 100-nm wide Nb N nanowires with a fill factor of 50%.The devices showed 72.4% system detection efficiency(SDE) at 100-Hz dark count rate(DCR) and 74-ps timing jitter,measured at the fiber communication wavelength of 1550 nm.The highest SDE which is 81.2% when the DCR is ～ 700 c/s appears at the wavelength of 1650 nm.展开更多
Metamaterial structure based on split ring resonators (SRR) is proposed in order to produce a negative refractive index. For this structure we have used a new approach, instead of applying light perpendicularly incide...Metamaterial structure based on split ring resonators (SRR) is proposed in order to produce a negative refractive index. For this structure we have used a new approach, instead of applying light perpendicularly incident. We apply horizontally incident input waves. A model of SRR is used to understand the behavior and its affects. We calculate the S-parameters using S-parameter analysis and the results for transmission, refractive index, permeability and permittivity of the structure is induced. The negative refractive index is found to be significantly dependent upon the width of the continuous wire as well as gap between resonators. Moreover, we study the effect of lattice constant on the electromagnetic response of the structure. It is expected that this work will provide useful information for design and fabrication of metamaterials with negative refractive index for in-plane applications.展开更多
While the spatial mode of photons is widely used in quantum cryptography, its potential for quantum computation remains largely unexplored. Here, we showcase the use of the multi-dimensional spatial mode of photons to...While the spatial mode of photons is widely used in quantum cryptography, its potential for quantum computation remains largely unexplored. Here, we showcase the use of the multi-dimensional spatial mode of photons to construct a series of high-dimensional quantum gates, achieved through the use of diffractive deep neural networks (D2NNs). Notably, our gates demonstrate high fidelity of up to 99.6(2)%, as characterized by quantum process tomography. Our experimental implementation of these gates involves a programmable array of phase layers in a compact and scalable device, capable of performing complex operations or even quantum circuits. We also demonstrate the efficacy of the D2NN gates by successfully implementing the Deutsch algorithm and propose an intelligent deployment protocol that involves self-configuration and self-optimization. Moreover, we conduct a comparative analysis of the D2NN gate’s performance to the wave-front matching approach. Overall, our work opens a door for designing specific quantum gates using deep learning, with the potential for reliable execution of quantum computation.展开更多
基金supports from National Natural Science Foundation of China (Grant No.62205117,52275429)National Key Research and Development Program of China (Grant No.2021YFF0502700)+3 种基金Young Elite Scientists Sponsorship Program by CAST (Grant No.2022QNRC001)West Light Foundation of the Chinese Academy of Sciences (Grant No.xbzg-zdsys-202206)Knowledge Innovation Program of Wuhan-Shuguang,Innovation project of Optics Valley Laboratory (Grant No.OVL2021ZD002)Hubei Provincial Natural Science Foundation of China (Grant No.2022CFB792).
文摘Interactive holography offers unmatched levels of immersion and user engagement in the field of future display.Despite of the substantial progress has been made in dynamic meta-holography,the realization of real-time,highly smooth interactive holography remains a significant challenge due to the computational and display frame rate limitations.In this study,we introduced a dynamic interactive bitwise meta-holography with ultra-high computational and display frame rates.To our knowledge,this is the first reported practical dynamic interactive metasurface holographic system.We spa-tially divided the metasurface device into multiple distinct channels,each projecting a reconstructed sub-pattern.The switching states of these channels were mapped to bitwise operations on a set of bit values,which avoids complex holo-gram computations,enabling an ultra-high computational frame rate.Our approach achieves a computational frame rate of 800 kHz and a display frame rate of 23 kHz on a low-power Raspberry Pi computational platform.According to this methodology,we demonstrated an interactive dynamic holographic Tetris game system that allows interactive gameplay,color display,and on-the-fly hologram creation.Our technology presents an inspiration for advanced dynamic meta-holography,which is promising for a broad range of applications including advanced human-computer interaction,real-time 3D visualization,and next-generation virtual and augmented reality systems.
基金We are grateful for financial supports from National Key Research and Development Program of China(Grant No.2021YFF0502700)National Natural Science Foundation of China(Grant Nos.52275429,62205117,61835008)+1 种基金Knowledge Innovation Program of Wuhan-Shuguang,Innovation project of Optics Valley Laboratory(Grant No.OVL2021ZD002)Hubei Provincial Natural Science Foundation of China(Grant Nos.2020CFA004,2022CFB792).
文摘Multispectral and polarized focusing and imaging are key functions that are vitally important for a broad range of optical applications.Conventional techniques generally require multiple shots to unveil desired optical information and are implemented via bulky multi-pass systems or mechanically moving parts that are difficult to integrate into compact and integrated optical systems.Here,a design of ultra-compact transversely dispersive metalens capable of both spectrum and polarization ellipticity recognition and reconstruction in just a single shot is demonstrated with both coherent and incoherent light.Our design is well suited for integrated and high-speed optical information analysis and can significantly reduce the size and weight of conventional devices while simplifying the process of collecting optical information,thereby promising for various applications,including machine vision,minimized spectrometers,material characterization,remote sensing,and other areas which require comprehensive optical analysis.
基金supports from National Key R&D Program of China(Grant No.2018YFB1801001)the National Natural Science Foundation of China(Grant No.61875061)the Program for Guangdong Introducing Innovative and Entrepreneurial Teams.
文摘Self-accelerating beams have the unusual ability to remain diffraction-free while undergo the transverse shift during the free-space propagation.We theoretically identify that the transverse optical field distribution of 2D self-accelerating beam is determined by the selection of the transverse Cartesian coordinates,when the caustic method is utilized for its trajectory design.Based on the coordinate-rotation method,we experimentally demonstrate a scheme to flexibly manipulate the rotation of transverse optical field for 2D self-accelerating beams under the condition of a designated trajectory.With this scheme,the transverse optical field can be rotated within a range of 90 degrees,especially when the trajectory of 2D self-accelerating beams needs to be maintained for free-space photonic interconnection.
基金This work is financially supported by the National Natural Science Foundation of China(Grant Nos.52072137,51802105).
文摘Tin (Sn) metal foil is a promising anode for next-generation high-energy–density lithium-ion batteries (LIBs) due to its high capacity and easy processibility. However, the pristine Sn foil anode suffers nonuniform alloying/dealloying reaction with lithium (Li) and huge volume variation, leading to electrode pulverization and inferior electrochemical performance. Herein, we proposed that reduced grain size and elaborate porosity design of Sn foil can circumvent the nonuniform alloy reaction and buffer the volume change during the lithiation/delithiation cycling. Experimentally, we designed a three-dimensional interconnected porous Sn (3DIP-Sn) foil by a facile chemical alloying/dealloying approach, which showed improved electrochemical performance. The enhanced structure stability of the as-fabricated 3DIP-Sn foil was verified by chemo-mechanical simulations and experimental investigation. As expected, the 3DIP-Sn foil anode revealed a long cycle lifespan of 4400 h at 0.5 mA cm^(−2) and 1 mAh cm^(−2) in Sn||Li half cells. A 3DIP-Sn||LiFePO_(4) full cell with LiFePO_(4) loading of 7.1 mg cm^(−2) exhibited stable cycling for 500 cycles with 80% capacity retention at 70 mA g^(−1). Pairing with high-loading commercial LiNi0.6Co0.2Mn0.2O_(2) (NCM622, 18.4 mg cm^(−2)) cathode, a 3DIP-Sn||NCM622 full cell delivered a high reversible capacity of 3.2 mAh cm^(−2). These results demonstrated the important role of regulating the uniform alloying/dealloying reaction and circumventing the localized strain/stress in improving the electrochemical performance of Sn foil anodes for advanced LIBs.
基金financially supported by the National Natural Science Foundation of China(NSFC)(Nos.62125503,62261160388,and 62101198)the Natural Science Foundation of Hubei Province of China(Nos.2021CFB011 and 2023AFA028)+2 种基金the Key R&D Program of Hubei Province of China(Nos.2020BAB001 and 2021BAA024)the Shenzhen Science and Technology Program(No.JCYJ20200109114018750)the Innovation Project of Optics Valley Laboratory(Nos.OVL2021BG004 and OVL2023ZD004)。
文摘Optical vortex arrays,with their unique wavefront structures,find extensive applications in fields such as optical communications,trapping,imaging,metrology,and quantum.The methods used to generate these vortex beam arrays are crucial for their applications.In this review,we begin with introducing the fundamental concepts of optical vortex beams.Subsequently,we present three methods for generating them,including diffractive optical elements,metasurfaces,and integrated optical devices.We then explore the applications of optical vortex beam arrays in five different domains.Finally,we conclude with a summary and outlook for the research on optical vortex beam arrays.
基金support from the National Key Research&Development Program(No.2016YFA0201902,2018YFA0703200)Shenzhen Nanshan District Pilotage Team Program(LHTD20170006)+4 种基金National Natural Science Foundation of China(61974099 and 61604102,51773041,61890940)Shanghai Committee of Science and Technology in China(18ZR1404900)Natural Science Research Project for Anhui Universities(Grant No.KJ2019A0596)Youth Project of Provincial Natural Science Foundation of Anhui(Grant No.2008085QF319)Australian Research Council(ARC,FT150100450 and IH150100006)。
文摘High-performance infrared(IR)photodetectors made by low dimensional materials promise a wide range of applications in communication,security and biomedicine.Moreover,light-harvesting effects based on novel plasmonic materials and their combinations with two-dimensional(2 D)materials have raised tremendous interest in recent years,as they may potentially help the device complement or surpass currently commercialized IR photodetectors.Graphene is a particularly attractive plasmonic material because graphene plasmons are electrically tunable with a high degree of electromagnetic confinement in the mid-infrared(mid-IR)to terahertz regime and the field concentration can be further enhanced by forming nanostructures.Here,we report an efficient mid-IR room-temperature photodetector enhanced by plasmonic effect in graphene nanoresonators(GNRs)/graphene heterostructure.The plasmon polaritons in GNRs are size-dependent with strong field localization.Considering that the size and density of GNRs are controllable by chemical vapor deposition method,our work opens a cost-effective and scalable pathway to fabricate efficient IR optoelectronic devices with wavelength tunability.
基金supported by the National Natural Science Foundation of China(61725401,61904058,61904058)the National Key R&D Program of China(2016YFA0204000)+1 种基金China Postdoctoral Science Foundation Project(2019M662623)the National Postdoctoral Program for Innovative Talent(BX20190127).
文摘The photovoltaic(PV)market is currently dominated by silicon based solar cells.However technological diversification is essential to promote competition,which is the driving force for technological growth.Historically,the choice of PV materials has been limited to the three-dimensional(3D)compounds with a high crystal symmetry and direct band gap.However,to meet the strict demands for sustainable PV applications,material space has been expanded beyond 3D compounds.In this perspective we discuss the potential of low-dimensional materials(2D,1D)for application in PVs.We present unique features of low-dimensional materials in context of their suitability in the solar cells.The band gap,absorption,carrier dynamics,mobility,defects,surface states and growth kinetics are discussed and compared to 3D counterparts,providing a comprehensive view of prospects of low-dimensional materials.Structural dimensionality leads to a highly anisotropic carrier transport,complex defect chemistry and peculiar growth dynamics.By providing fundamental insights into these challenges we aim to deepen the understanding of low-dimensional materials and expand the scope of their application.Finally,we discuss the current research status and development trend of solar cell devices made of low-dimensional materials.
文摘Metamaterial structure based on cascaded split ring resonators (CSRR) is proposed in order to produce a negative refractive index in terahertz regime at near-infrared range. We have incident light horizontally instead of incidenting it perpendicular. We have measured the negative refractive index, permeability and permittivity by using the S-parameter analysis. Furthermore, it is found out that negative refractive index, permeability and permittivity are dependent upon the width of the wire and the gap between resonators at near-infrared range. This work will be helpful for the fabrication and design of double negative metamaterials structure having negative permeability, permittivity and negative refractive index for in plane applications.
基金This work was supported by the National Natural Science Foundation of China(Grant Nos.62125503 and 62261160388)the Key R&D Program of Hubei Province of China(Grant Nos.2020BAB001 and 2021BAA024)+2 种基金the Key R&D Program of Guangdong Province(Grant No.2018B030325002)the Shenzhen Science and Technology Program(Grant No.JCYJ20200109114018750)the Innovation Project of Optics Valley Laboratory(Grant No.OVL2021BG004).
文摘Explosive growth in demand for data traffic has prompted exploration of the spatial dimension of lightwaves, which provides a degree of freedom to expand data transmission capacity. Various techniques basedon bulky optical devices have been proposed to tailor light waves in the spatial dimension. However, theirinherent large size, extra loss, and precise alignment requirements make these techniques relativelydifficult to implement in a compact and flexible way. In contrast, three-dimensional (3D) photonic chips withcompact size and low loss provide a promising miniaturized candidate for tailoring light in the spatialdimension. Significantly, they are attractive for chip-assisted short-distance spatial mode optical interconnectsthat are challenging to bulky optics. Here, we propose and fabricate femtosecond laser-inscribed 3D photonicchips to tailor orbital angular momentum (OAM) modes in the spatial dimension. Various functions on theplatform of 3D photonic chips are experimentally demonstrated, including the generation, (de)multiplexing,and exchange of OAM modes. Moreover, chip-chip and chip–fiber–chip short-distance optical interconnectsusing OAM modes are demonstrated in the experiment with favorable performance. This work paves the wayto flexibly tailor light waves on 3D photonic chips and offers a compact solution for versatile opticalinterconnects and other emerging applications with spatial modes.
基金the National Natural Science Foundation of China(Grant No.61975249)the National Key Research and Development Program of China(Nos.2018YFB2201700 and 2018YFA0704403)the Program for HUST Academic Frontier Youth Team(No.2018QYTD08).
文摘Optical beating is the usual approach to generation of microwave signals.However,the highest frequency achievable for microwave signals is limited by the bandwidths of optoelectronic devices.To maximize the microwave frequency with a limited bandwidth of a photodetector(PD)and relieve the bandwidth bottleneck,we propose to generate microwave signals with the single sideband(SSB)format by beating a continuous wave(CW)light with an optical SSB signal.By simply adjusting the frequency diference between the CW light and the carrier of the optical SSB signal,the frequency of the generated microwave SSB signal is changed correspondingly.In the experiment,amplitude shift keying(ASK)microwave signals with the SSB format are successfully generated with diferent carrier frequencies and coding bit rates,and the recovered coding information agrees well with the original pseudo random binary sequence(PRBS)of 2^(7)−1 bits.The proposed approach can signifcantly relieve the bandwidth restriction set by optoelectronic devices in high-speed microwave communication systems.
基金National Key Research and Development Program of China(2021YFF0502700)National Natural Science Foundation of China(52275429,62205117)+4 种基金Innovation project of Optics Valley Laboratory(OVL2021ZD002)Hubei Provincial Natural Science Foundation of China(2022CFB792)Young Elite Scientists Sponsorship Program by CAST(2022QNRC001)West Light Foundation of the Chinese Academy of Sciences(xbzg-zdsys-202206)Knowledge Innovation Program of Wuhan-Shuguang。
文摘Nano-3D printing has obtained widespread attention owing to its capacity to manufacture end-use components with nano-scale features in recent years.Multiphoton lithography(MPL)is one of the most promising 3D nanomanufacturing technologies,which has been widely used in manufacturing micro-optics,photonic crystals,microfluidics,meta-surface,and mechanical metamaterials.Despite of tremendous potential of MPL in laboratorial and industrial applications,simultaneous achievement of high throughput,high accuracy,high design freedom,and a broad range of material structuring capabilities remains a long-pending challenge.To address the issue,we propose an acousto-optic scanning with spatial-switching multispots(AOSS)method.Inertia-free acousto-optic scanning and nonlinear swept techniques have been developed for achieving ultrahigh-speed and aberration-free scanning.Moreover,a spatial optical switch concept has been implemented to significantly boost the lithography throughput while maintaining high resolution and high design freedom.An eight-foci AOSS system has demonstrated a record-high 3D printing rate of 7.6×10^(7)voxel s^(-1),which is nearly one order of magnitude higher than earlier scanning MPL,exhibiting its promise for future scalable 3D nanomanufacturing.
文摘The complex Maxwell stress tensor theorem has been developed to relate the imaginary optical force,reactive strength of canonical momentum and total optical force of a nanoparticle,which is essential to perfect optical force efficiency.
基金National Natural Science Foundation of China(52275562)National Key Research and Development Program of China(2019YFB1503200)。
文摘Scintillators are widely utilized in high-energy radiation detection in view of their high light yield and short fluorescence decay time.However,constrained by their current shortcomings,such as complex fabrication procedures,high temperature,and difficulty in the large scale,it is difficult to meet the increasing demand for costeffective,flexible,and environment-friendly X-ray detection using traditional scintillators.Perovskite-related cesium copper halide scintillators have recently received multitudinous research due to their tunable emission wavelength,high photoluminescence quantum yield(PLQY),and excellent optical properties.Herein,we demonstrated a facile solution-synthesis route for indium-doped all-inorganic cesium copper iodide(Cs_(3)Cu_(2)I_(5))powders and a high scintillation yield flexible film utilizing indium-doped Cs_(3)Cu_(2)I_(5)powders.The large area flexible films achieved a PLQY as high as 90.2%by appropriately adjusting the indium doping concentration,much higher than the undoped one(73.9%).Moreover,benefiting from low self-absorption and high PLQY,the Cs_(3)Cu_(2)I_(5):In films exhibited ultralow detection limit of 56.2 n Gy/s,high spatial resolution up to 11.3 lp/mm,and marvelous relative light output with strong stability,facilitating that Cs_(3)Cu_(2)I_(5):In films are excellent candidates for X-ray medical radiography.Our work provides an effective strategy for developing environment-friendly,low-cost,and efficient scintillator films,showing great potential in the application of highperformance X-ray imaging.
基金supported by the National Key R&D Program of China(No.2016YFB070700702)the National Natural Science Foundation of China(Grant No.51761145048)+1 种基金the Fundamental Research Funds for the Central Universities(HUST:2019421JYCXJJ004)the Innovation Funds of Wuhan National Laboratory for Optoelectronics(WNLO).
文摘Perovskite-based optoelectronic devices,espe-cially perovskite light-emitting diodes(PeLEDs)and perovskite solar cells,have recently attracted considerable attention.The National Renewable Energy Laboratory(NREL)chart inspires us to develop a counterpart for PeLEDs.In this study,we collect the record performance of PeLEDs including several new entries to address their latest external quantum efficiency(EQE),highest lumi-nance,and stability status.We hope that these performance tables and future updated versions will show the frontiers of PeLEDs,assist researchers in capturing the overview of this field,identify the remaining challenges,and predict the promising research directions.
基金supported by the National Natural Science Foundation of China (Grant nos. 21474035, 51773072)the HUST Innovation Research Fund (Grant nos. 2016JCTD111, 2017KFKJXX012)+1 种基金the Science and Technology Program of Hubei Province (2017AHB040)China Postdoctoral Science Foundation funded project (2016M602289)
文摘Preparation of high-quality films plays an important role to achieve high-performance nonfullerene (NF) organic solar cells. NF active layer films are typically fabricated by spin coating. Novel fabrication methods to process the NF active layer are desirable to be compatible with large-area production. Herein, we report on the fabrication of NF active layer films via a water transfer printing method.This method delivers a uniform film with controllable film thicknesses. NF active layers of PDBD-T:ITIC and PBDB-T-2F:IT-4F were fabricated via the method to validate its effectiveness. Solar cells with the water transfer-printed active layers show comparable performance (up to 11.7%) to the cells with spin-coated active layers. Furthermore, NF solar modules containing 4-sub cells with the active area of 3.2 cm2 are also fabricated via the method. The module shows VOC of up to 3.4 V and a power conversion efficiency of 8.1% with the PBDB-T-2F:IT-4F active layer.
文摘Niobium nitride superconducting nanowire single-photon detectors were fabricated on thermally oxidized silicon substrates with large active areas of 30 μm× 30 μm.To achieve non-constricted detectors,we improved the film growth and electron beam lithography process to fabricate uniform 100-nm wide Nb N nanowires with a fill factor of 50%.The devices showed 72.4% system detection efficiency(SDE) at 100-Hz dark count rate(DCR) and 74-ps timing jitter,measured at the fiber communication wavelength of 1550 nm.The highest SDE which is 81.2% when the DCR is ～ 700 c/s appears at the wavelength of 1650 nm.
文摘Metamaterial structure based on split ring resonators (SRR) is proposed in order to produce a negative refractive index. For this structure we have used a new approach, instead of applying light perpendicularly incident. We apply horizontally incident input waves. A model of SRR is used to understand the behavior and its affects. We calculate the S-parameters using S-parameter analysis and the results for transmission, refractive index, permeability and permittivity of the structure is induced. The negative refractive index is found to be significantly dependent upon the width of the continuous wire as well as gap between resonators. Moreover, we study the effect of lattice constant on the electromagnetic response of the structure. It is expected that this work will provide useful information for design and fabrication of metamaterials with negative refractive index for in-plane applications.
基金supported by the National Natural Science Foundation of China(62125503,62261160388,62001182,62371202)the Natural Science Foundation of Hubei Province of China(2023AFA028,2023AFB814)+2 种基金the Key R&D Program of Guangdong Province(2018B030325002)the Key R&D Program of Hubei Province of China(2021BAA024,2020BAB001)the Innovation Project of Optics Valley Laboratory(OVL2021BG004).
文摘While the spatial mode of photons is widely used in quantum cryptography, its potential for quantum computation remains largely unexplored. Here, we showcase the use of the multi-dimensional spatial mode of photons to construct a series of high-dimensional quantum gates, achieved through the use of diffractive deep neural networks (D2NNs). Notably, our gates demonstrate high fidelity of up to 99.6(2)%, as characterized by quantum process tomography. Our experimental implementation of these gates involves a programmable array of phase layers in a compact and scalable device, capable of performing complex operations or even quantum circuits. We also demonstrate the efficacy of the D2NN gates by successfully implementing the Deutsch algorithm and propose an intelligent deployment protocol that involves self-configuration and self-optimization. Moreover, we conduct a comparative analysis of the D2NN gate’s performance to the wave-front matching approach. Overall, our work opens a door for designing specific quantum gates using deep learning, with the potential for reliable execution of quantum computation.
